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We present details about an experimental method based on the Landau Zener model which allows to measure very small tunnel splittings $\Delta$ in molecular clusters Fe8. The measurements are performed with an array of micro-SQUIDs. The…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , R. Sessoli , A. Caneschi , D. Gatteschi , A. Cornia , D. Mailly

The Landau Zener method allows to measure very small tunnel splittings \Delta in molecular clusters Fe_8. The observed oscillations of \Delta as a function of the magnetic field applied along the hard anisotropy axis are explained in terms…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , R. Sessoli , A. Caneschi , D. Gatteschi , A. Cornia

Magnetization measurements of a molecular clusters Mn12 with a spin ground state of S = 10 show resonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the magnetic field…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 W. Wernsdorfer , M. Soler , G. Christou , D. N. Hendrickson

Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Wernsdorfer , N. E. Chakov , G. Christou

The tunnel splitting in biaxial antiferromagnetic particles is studied with a magnetic field applied along the hard anisotropy axis. We observe the oscillation of tunnel splitting as a function of the magnetic field due to the quantum phase…

Condensed Matter · Physics 2019-08-17 Yi-Hang Nie , Yan-Hong Jin , J. -Q. Liang , H. J. W. Müller-Kirsten , D. K. Park , F. -C. Pu

Ramsey et al. [Nature Phys. 4, 277-281 (2008)] report the observation of quantum interference associated with tunnelling trajectories between states of different total spin length in a dimeric molecular nanomagnet. They argue that the…

Mesoscale and Nanoscale Physics · Physics 2008-07-07 W. Wernsdorfer

The tunneling splitting in biaxial ferrimagnetic particles at excited states with an explicit calculation of the prefactor of exponent is obtained in terms of periodic instantons which are responsible for tunneling at excited states and is…

Condensed Matter · Physics 2019-08-17 Yi-Hang Nie , Yan-Hong Jin , J. -Q Liang , F. -C Pu

Quantum phase interference and spin-parity effects are studied in biaxial molecular magnets in a magnetic field at an arbitrarily directed angle. The calculations of the ground-state tunnel splitting are performed on the basis of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Hui Hu , Jia-Lin Zhu , Rong Lu , Jia-Jiong Xiong

Renormalized tunnel splitting with a finite distribution in the biaxial spin model for molecular magnets is obtained by taking into account the dipolar interaction of enviromental spins. Oscillation of the resonant tunnel splitting with a…

Strongly Correlated Electrons · Physics 2009-11-07 Zhi-De Chen , J. -Q. Liang , Shun-Qing Shen

The detailed theoretical understanding of quantum spin dynamics in various molecular magnets is an important step on the roadway to technological applications of these systems. Quantum effects in both ferromagnetic and antiferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael N. Leuenberger , Florian Meier , Daniel Loss

We study spin tunneling in magnetic molecules, with special reference to Fe8. The article aims to give a pedagogical discussion of what is meant by the tunneling of a spin, and how tunneling amplitudes or energy level splittings may be…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Anupam Garg

Small ferromagnets and anti-ferromagnets with an easy-plane anisotropy have a ground to first excited state (tunnel) splitting which is quasi-periodic in the magnitude of a field applied perpendicular to a principal anisotropy axis. The…

Condensed Matter · Physics 2007-05-23 S. E. Barnes

Macroscopic quantum coherence and spin-phase interference are studied between excited levels in single-domain ferromagnetic particles in a magnetic field along the hard anisotropy axis. The system has the general structure of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Pan Hui , Rong Lu , Jia-Lin Zhu , Yi Zhou

The quantum interference effects induced by the topological phase are studied analytically in biaxial antiferromagnets with an external magnetic field at an arbitrarily angle. This study provides a nontrivial generalization of the Kramers…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Rong Lu , Hui Pan , Jia-Lin Zhu , Bing-Lin Gu

Two antiferromagnetically coupled tunneling systems is a minimal model exhibiting the effect of quantum-mechanical phase in the Landau-Zener effect. It is shown that the averaged staying probability oscillates vs resonance shift between the…

Statistical Mechanics · Physics 2007-05-23 D. A. Garanin

The spin-phase interference effects are studied analytically in resonant quantum tunneling of the N\'{e}el vector between degenerate excited levels in nanometer-scale single-domain antiferromagnets in the absence of an external magnetic…

Statistical Mechanics · Physics 2015-06-24 Rong Lu , Jia-Lin Zhu , Yi Zhou , Bing-Lin Gu

We show that the dynamic magnetic susceptibility and the superparamagnetic blocking temperature of an Fe8 single molecule magnet oscillate as a function of the magnetic field Hx applied along its hard magnetic axis. These oscillations are…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 E. Burzurí , F. Luis , O. Montero , B. Barbara , R. Ballou , S. Maegawa

We present a quantum interpretation of the heights in hysteresis of $Fe_{8}$ molecule at lower temperatures by treating the crystal as an Ising spin system with the dipolar interaction between spins. Then we apply it to two limit cases :…

Other Condensed Matter · Physics 2009-11-10 Li-Bin Fu , Shi-Gang Chen , Bambi Hu

We analyze the interference between tunneling paths that occurs for a spin system with both fourth-order and second-order transverse anisotropy. Using an instanton approach, we find that as the strength of the second-order transverse…

Mesoscale and Nanoscale Physics · Physics 2009-04-30 M. S. Foss-Feig , Jonathan R. Friedman

Magnetization measurements of a truly axial symmetry Mn12-tBuAc molecular nanomagnet with a spin ground state of S = 10 show resonance tunneling. This compound has the same magnetic anisotropy as Mn12-Ac but the molecules are better…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 W. Wernsdorfer , M. Murugesu , G. Christou
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