Related papers: Quantum Phase Interference in Magnetic Molecular C…
Single-molecule magnets facilitate the study of quantum tunneling of magnetization at the mesoscopic level. The spin-parity effect is among the fundamental predictions that have yet to be clearly observed. It is predicted that quantum…
The oscillation of tunnel splitting are obtained by geometrical analysis of the topological Wess-Zumino phase on the basis of tunneling paths in biaxial nanomagnetic particles with magnetic field along the hard anisotropy axis. This theory…
High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…
We investigate the macroscopic quantum coherence of a spin-1 Rb condensate confined in an anisotropic potential. Under the single-mode approximation, we show that the system can be modeled as a biaxial quantum magnet due to the interplay…
Spin coherent state path integrals with discontinuous semiclassical paths are investigated with special reference to a realistic model for the magnetic degrees of freedom in the Fe8 molecular solid. It is shown that such paths are essential…
Spin splitting in the integer quantum Hall effect is investigated for a series of Al$_{x}$Ga$_{1-x}$As/GaAs heterojunctions and quantum wells. Magnetoresistance measurements are performed at mK temperature to characterize the electronic…
The equal-interval splitting of quantum tunneling observed in simple-Ising-model systems of Ni$_{4}$ (3D) and Mn$_3$ (2D) single-molecule magnets (SMMs) is reported. The splitting is due to the identical exchange coupling in the SMMs, and…
Tunneling between the two lowest energy levels of single molecule magnets with Ising type anisotropy, accompanied by the emission or absorption of phonons, is considered. Quantitatively accurate calculations of the rates for such tunneling…
The point-particle-like Hamiltonian of a biaxial spin particle with external magnetic field along the hard axis is obtained in terms of the potential field description of spin systems with exact spin-coordinate correspondence. The Zeeman…
The macroscopic quantum coherence in a biaxial antiferromagnetic molecular magnet in the presence of magnetic field acting parallel to its hard anisotropy axis is studied within the two-sublattice model. On the basis of instanton technique…
The quantum tunneling of the magnetization vector are studied theoretically in single-domain ferromagnetic nanoparticles placed in an external magnetic field at an arbitrarily directed angle in the $ZX$ plane. We consider the…
A Mn4 single-molecule magnet (SMM), with a well isolated spin ground state of S = 9/2, is used as a model system to study Landau-Zener (LZ) tunneling in the presence of weak intermolecular dipolar and exchange interactions. The anisotropy…
We consider the resonant tunneling through a multi-level system. It is demonstrated that the resonant current displays quantum interference effects due to a possibility of tunneling through different levels. We show that the interference…
Quantum tunneling of the magnetization is a major obstacle to the use of single-molecule magnets (SMMs) as basic constituents of next-generation storage devices. In this context, phonons are often only considered (perturbatively) as…
We present topological interference effects for the tunneling of a single large spin, which are caused by the symmetry of a general class of magnetic anisotropies. The interference originates from spin Berry phases associated with different…
The low temperature spin dynamics of a Fe8 Single-Molecule Magnet was studied under circularly polarized electromagnetic radiation allowing us to establish clearly photon-assisted tunneling. This effect, while linear at low power, becomes…
A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…
The antiferromagnetic molecular wheel Fe18 of eighteen exchange-coupled Fe(III) ions has been studied by measurements of the magnetic torque, the magnetization, and the inelastic neutron scattering spectra. The combined data show that the…
We study Landau-Zener macroscopic quantum transitions in ferromagnetic metal nanoparticles containing on the order of 100 atoms. The model that we consider is described by an effective giant-spin Hamiltonian, with a coupling to a random…
The perfect quenching of spin tunneling that has previously been discussed in terms of interfering instantons, and has recently been observed in the magnetic molecule \Fe8, is treated using a discrete phase integral (or…