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The orbital shapes and charge disproportionations at nominal Mn$^{3+}$ and Mn$^{4+}$ sites for the charge- and orbital-ordered phases have been studied on half-doped manganites Pr(Sr$_{0.1}$Ca$_{0.9}$)$_2$Mn$_2$O$_7$ and…

Strongly Correlated Electrons · Physics 2009-10-17 D. Okuyama , Y. Tokunaga , R. Kumai , Y. Taguchi , T. Arima , Y. Tokura

We report a synchrotron x-ray scattering study of the magnetoresistive manganite La_0.875Sr_0.125MnO_3. At low temperatures, this material undergoes an x-ray induced structural transition at which charge ordering of Mn^3+ and Mn^4+ ions…

Strongly Correlated Electrons · Physics 2009-10-31 V. Kiryukhin , Y. J. Wang , F. C. Chou , M. A. Kastner , R. J. Birgeneau

We report x-ray scattering studies of nanoscale structural correlations in the paramagnetic phases of the perovskite manganites La$_{0.75}$(Ca$_{0.45}$Sr$_{0.55}$)$_{0.25}$MnO$_3$, La$_{0.625}$Sr$_{0.375}$MnO$_3$, and…

Condensed Matter · Physics 2009-11-10 V. Kiryukhin , T. Y. Koo , H. Ishibashi , J. P. Hill , S-W. Cheong

Charge-order-driven ferroelectrics are an emerging class of functional materials, distinct from conventional ferroelectrics, where electron-dominated switching can occur at high frequency. Despite their promise, only a few systems…

Materials Science · Physics 2020-02-19 Se Young Park , Karin M. Rabe , Jeffrey B. Neaton

Investigation of the magnetism of Cu$_3$Mo$_2$O$_9$ single crystal, which has antiferromagnetic (AF) linear chains interacting with AF dimers, reveals an AF second-order phase transition at $T_{\rm N} = 7.9$ K. Although weak…

Strongly Correlated Electrons · Physics 2009-11-13 Tomoaki Hamasaki , Tomoyuki Ide , Haruhiko Kuroe , Tomoyuki Sekine , Masashi Hase , Ichiro Tsukada , Toshiro Sakakibara

The low temperature phase of single crystals of Nd$_{0.5}$Ca$_{0.5}$MnO$_3$ and Gd$_{0.5}$Ca$_{0.5}$MnO$_3$ manganites is investigated by squid magnetometry. Nd$_{0.5}$Ca$_{0.5}$MnO$_3$ undergoes a charge-ordering transition at…

Materials Science · Physics 2016-08-31 R. Mathieu , P. Nordblad , A. R. Raju , C. N. R. Rao

Systematic studies of magnetic properties of LaSr2Mn2O7 as a function of crystalline grain size provide information on how the crystalline grain size affects the magnetic and charge ordering in this compound. The half-doped bi-layered…

Materials Science · Physics 2014-09-16 M. E. Ehsani , M. E. Ghazi , P. Kameli , F. S. Razavi

We report a comprehensive investigation of La0.2Pr0.4Ca0.4MnO3 to clarify the micrometre scale phase separation phenomenon in the mixed valent manganite (La,Pr,Ca)MnO3. The compound shows multiple magnetic transitions, in which the…

Materials Science · Physics 2020-03-18 Deepak Kumar , Ashwin A. Tulapurkar , C. V. Tomy

Since the discovery of charge disproportionation in the FeO$_2$ square-lattice compound Sr$_3$Fe$_2$O$_7$ by M\"ossbauer spectroscopy more than fifty years ago, the spatial ordering pattern of the disproportionated charges has remained…

The interplay of charge, spin, and lattice degrees of freedom in matter leads to various forms of ordered states through phase transitions. An important subclass of these phenomena of complex materials is charge ordering (CO), mainly driven…

Strongly Correlated Electrons · Physics 2018-08-15 Arvind Yogi , C. I. Sathish , Hasung Sim , Matthew J. Coak , Y. Noda , Je-Geun Park

Electron microdiffraction study of phase transition in La2/3Ca1/3MnO3 revealed temperature dependent (h+1/2,0,l) diffraction spots. Their intensity peaks at Tc. Quantitative electron diffraction intensity analysis shows that they come from…

Strongly Correlated Electrons · Physics 2009-10-31 J. M. Zuo , J. Tao

The complex lanthanide doping of electron manganites results in enhancement of various phase separation effects in physical properties of these compounds. Selecting Ca0.8Sm0.16Nd0.04MnO3 as a model case we show that the first order…

Strongly Correlated Electrons · Physics 2009-11-10 D. A. Filippov , K. V. Klimov , R. Z. Levitin , A. N. Vasil'Ev , T. N. Voloshok , R Suryanarayanan

Neutron scattering has been used to study the nature of the ferromagnetic transition in a single crystal of the perovskite La0.7Ca0.3MnO3. Diffuse scattering from lattice polarons develops as the Curie temperature is approached from below,…

Strongly Correlated Electrons · Physics 2009-10-31 C. P. Adams , J. W. Lynn , Y. M. Mukovskii , A. A. Arsenov , D. A. Shulyatev

The magnetically ordered states of the A-site ordered perovskite manganites LaBaMn2O6 and YBaMn2O6 have been investigated by muon spin relaxation in zero external magnetic field. Our data reveal striking differences in the nature of the…

Strongly Correlated Electrons · Physics 2015-06-05 Y. Kawasaki , T. Minami , M. Izumi , Y. Kishimoto , T. Ohno , K. H. Satoh , A. Koda , R. Kadono , J. L. Gavilano , H. Luetkens , T. Nakajima , Y. Ueda

We report an interesting reentrant metallic resistivity pattern beyond a characteristic temperature T* which is higher than other such characteristic transition temperatures like T(c)(Curie point), T(N) (Neel point), T(CO) (charge order…

Strongly Correlated Electrons · Physics 2007-05-23 Dipten Bhattacharya , H. S. Maiti

We report an inelastic neutron scattering study of acoustic phonons in the charge and orbitally ordered bilayer manganite LaSr$_2$Mn$_2$O$_7$. For excitation energies less than $15\,\rm{meV}$, we observe an abrupt increase (decrease) of the…

Strongly Correlated Electrons · Physics 2011-12-14 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , H. Zheng , J. F. Mitchell , Y. Chen , Songxue Chi , J. W. Lynn , D. Reznik

Neutron diffraction studies have been carried out on a single crystal of oxygen-deficient perovskite NdBaCo2O5 in the temperature range of 7-370 K. There have been observed, with decreasing temperature T, two magnetic transitions…

Strongly Correlated Electrons · Physics 2009-11-10 Minoru Soda , Yukio Yasui , Masafumi Ito , Satoshi Iikubo , Masatoshi Sato , Kazuhisa Kakurai

Neutron diffraction measurements on multiferroic LuFe2O4 show changes in the antiferromagnetic (AFM) structure characterized by wavevector q = (1/3 1/3 1/2) as a function of electric field cooling procedures. The increase of intensity from…

Strongly Correlated Electrons · Physics 2011-11-09 A. M. Mulders , M. Bartkowiak , J. R. Hester , E. Pomjakushina , K. Conder

We investigated complex magnetic properties of multifunctional LaCrO3-LaFeO3 system. The magnetic measurements substantiate the presence of competing complex magnetic ordering against temperature, showing paramagnetic to ferrimagnetic…

Strongly Correlated Electrons · Physics 2019-08-20 Brajesh Tiwari , Ambesh Dixit , M. S. Ramachandra Rao

In this paper the effect of the chemical pressure induced by the Sr replacement for Ca in the La1.4Sr1.6Mn2O7 lattice is directly probed by means of neutron diffraction as a function of temperature. The results show a progressive change of…

Materials Science · Physics 2007-10-25 Lorenzo Malavasi , Clemens Ritter , M. Cristina Mozzati , Carlo B. Azzoni , Giorgio Flor
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