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Although not an intrinsic superconductor, it has been long--known that, when intercalated with certain dopants, graphite is capable of exhibiting superconductivity. Of the family of graphite--based materials which are known to superconduct,…

Superconductivity · Physics 2016-08-16 Gabor Csányi , P. B. Littlewood , A. H. Nevidomskyy , Chris J. Pickard , B. D. Simons

We use first-principles calculation within the density functional theory (DFT) to explore the electronic properties on stage-1 Li- and Li+-graphite-intercalation compounds (GIC) for different concentrations, LiCx/Li+Cx with x= 6,12,18,24,32…

Materials Science · Physics 2020-06-24 Wei-Bang Li , Shih-Yang Lin , Ngoc Thanh Thuy Tran , Kuang-I Lin , Ming-Fa Lin

Intercalation of epitaxial graphene on SiC(0001) with Sn results in a well-ordered Sn $(1\times1)$ structure on the SiC surface with quasi-freestanding graphene on top. While the electronic properties of the individual layers have been…

Using the tight-binding model of graphite, incorporating all Slonczewski-Weiss-McClure parameters, we compute the spectrum of two-dimensional states of electrons bound to a stacking fault in Bernal graphite. We find that those bands retain…

Mesoscale and Nanoscale Physics · Physics 2024-12-10 Patrick Johansen Sarsfield , Sergey Slizovskiy , Mikito Koshino , Vladimir Fal'ko

This work introduces a new class of two-dimensional crystals with the structure AC$_8$XC$_8$, consisting of two layers of graphene, a chalcogen (X = O, S, Se, Te) intercalation layer, and an alkaline earth (A = Be, Ca, Mg, Sr, Ba) adlayer.…

Mesoscale and Nanoscale Physics · Physics 2025-03-11 Tommy Li

The unusual transport properties of graphene are the direct consequence of a peculiar bandstructure near the Dirac point. We determine the shape of the pi bands and their characteristic splitting, and the transition from a pure 2D to…

Materials Science · Physics 2007-05-23 Taisuke Ohta , Aaron Bostwick , J. L. McChesney , Thomas Seyller , Karsten Horn , Eli Rotenberg

First-principles calculations of the electronic structure and vibrational modes, in a system of graphene bilayers and trilayers intercalated with alkaline earth atoms, are resented. It is found that, in similarity to the case of…

Superconductivity · Physics 2011-07-12 R. A. Jishi , D. M. Guzman , H. M. Alyahyaei

Intercalation is an established technique for tailoring the electronic structure of epitaxial graphene. Moreover, it enables the synthesis of otherwise unstable two-dimensional (2D) layers of elements with unique physical properties…

Mesoscale and Nanoscale Physics · Physics 2022-06-29 Bharti Matta , Philipp Rosenzweig , Olaf Bolkenbaas , Kathrin Küster , Ulrich Starke

Various bandstructure engineering methods have been studied to improve the performance of graphitic transparent conductors; however none demonstrated an increase of optical transmittance in the visible range. Here we measure in situ optical…

We present detailed multi frequency resonant Raman measurements of potassium graphite intercalation compounds (GICs). From a well controlled and consecutive in-situ intercalation and high temperature de-intercalation approach the response…

Materials Science · Physics 2013-10-25 J. C. Chacon-Torres , L. Wirtz , T. Pichler

A flat energy dispersion of electrons at the Fermi level of a material leads to instabilities in the electronic system and can drive phase transitions. Here we introduce a method to induce a flat band in two-dimensional (2D) materials. We…

Mesoscale and Nanoscale Physics · Physics 2019-12-16 N. Ehlen , M. Hell , G. Marini , E. H. Hasdeo , R. Saito , G. Di Santo , L. Petaccia , G. Profeta , A. Grüneis

We find experimentally that the optical sheet conductance of graphite per graphene layer is very close to $(\pi/2)e^2/h$, which is the theoretically expected value of dynamical conductance of isolated monolayer graphene. Our calculations…

Strongly Correlated Electrons · Physics 2009-11-13 A. B. Kuzmenko , E. van Heumen , F. Carbone , D. van der Marel

The essential properties of graphite-based 3D systems are thoroughly investigated by the first-principles method. Such materials cover a simple hexagonal graphite, a Bernal graphite, and the stage-1 to stage-4 Li/Li$^+$ graphite…

Materials Science · Physics 2018-10-29 Shih-Yang Lin , Wei-Bang Li , Ngoc Thanh Thuy Tran , Wen-Dung Hsu , Hsin-Yi Liu , Ming Fa-Lin

Electrons in isolated graphene layers are a two-dimensional gas of massless Dirac Fermions. In realistic devices, however, the electronic properties are modified by elastic deformations, interlayer coupling and substrate interaction. Here…

The high pressure phase diagram of CsC8 graphite intercalated compound has been investigated at ambient temperature up to 32 GPa. Combining X-ray and neutron diffraction, Raman and X- ray absorption spectroscopies, we report for the first…

Using density functional theory calculations, we have investigated the structural, energetic, and electronic properties of ternary graphite intercalation compounds (GICs) containing alkali atoms (AM) and normal alkylamine molecules (nC$x$),…

Materials Science · Physics 2017-09-20 Gum-Chol Ri , Chol-Jun Yu , Jin-Song Kim , Song-Nam Hong , Un-Gi Jong , Mun-Hyok Ri

We have performed photoemission studies of the electronic structure in LiC$_6$ and KC$_8$, a non-superconducting and a superconducting graphite intercalation compound, respectively. We have found that the charge transfer from the…

Superconductivity · Physics 2011-05-20 Z. -H. Pan , J. Camacho , M. H. Upton , A. V. Fedorov , C. A. Howard , M. Ellerby , T. Valla

Modeling layered intercalation compounds from first principles poses a problem, as many of their properties are determined by a subtle balance between van der Waals interactions and chemical or Madelung terms, and a good description of van…

Materials Science · Physics 2014-10-30 E. Hazrati , G. A. de Wijs , G. Brocks

Quantum transport properties in molecularly thin perovskite/graphene heterostructure are experimentally investigated by Shubnikov-de Hass (SdH) oscillation and photo-resistance spectroscopy. We find an efficient charge transfer between the…

Mesoscale and Nanoscale Physics · Physics 2023-12-22 Yan Sun , C. Morice , D. Garrot , R. Weil , K. Watanabe , T. Taniguchi , M. Monteverde , A. D. Chepelianskii

Intercalation at the graphene/SiC interface provides a controlled route to stabilize atomically thin layers with properties distinct from their bulk counterparts. In this platform, the structure and stability of the intercalated phase…

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