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A mesoscopic model of a diblock copolymer is used to study the stability of a uniform lamellar phase under a reciprocating shear flow. Approximate viscosity contrast between the microphases is allowed through a linear dependence of the…

Soft Condensed Matter · Physics 2009-11-07 Peilong Chen , Jorge Vinals

We introduce a model constitutive law for the dissipative stress tensor of lamellar phases to account for low frequency and long wavelength flows. Given the uniaxial symmetry of these phases, we argue that the stress tensor must be the same…

Soft Condensed Matter · Physics 2009-11-11 Zhi-Feng Huang , Jorge Vinals

A nonequilibrium molecular dynamics computer simulation on microsegregated solutions of symmetrical diblock copolymers is reported. As the polymer concentration increases, the system undergoes phase transitions in the following order: body…

Soft Condensed Matter · Physics 2007-05-23 Igor Rychkov , Kenichi Yoshikawa

We consider the shear flow of well-aligned one-component smectic phases, such as thermotropic smectics and lamellar diblock copolymers, below the critical region. We show that, as a result of thermal fluctuations of the layers, parallel…

Condensed Matter · Physics 2016-08-31 Mark Goulian , Scott T. Milner

The properties of semidilute polymer solutions are investigated at equilibrium and under shear flow by mesoscale simulations, which combine molecular dynamics simulations and the multiparticle collision dynamics approach. In semidilute…

Soft Condensed Matter · Physics 2015-03-19 Chien-Cheng Huang , Roland G. Winkler , Godehard Sutmann , Gerhard Gompper

In order to address the selection mechanism that is responsible for the unique lamellar orientation observed in block copolymers under oscillatory shears, we use a constitutive law for the dissipative part of the stress tensor that respects…

Soft Condensed Matter · Physics 2009-11-11 Zhi-Feng Huang , Jorge Vinals

The non-linear response of entangled polymers to shear flow is complicated. Its current understanding is framed mainly as a rheological description in terms of the complex viscosity. However, the full picture requires an assessment of the…

Computational Physics · Physics 2018-08-21 Airidas Korolkovas , Philipp Gutfreund , Max Wolff

A mesoscopic model of a diblock copolymer is used to study the motion of a grain boundary separating two regions of perfectly ordered lamellar structures under an oscillatory but uniform shear flow. The case considered is a grain boundary…

Soft Condensed Matter · Physics 2007-05-23 Francois Drolet , Jorge Vinals

We study the dynamics of the phase behavior of a polymer blend in the presence of shear flow. By adopting a two fluid picture and using a generalization of the concept of material derivative, we construct kinetic equations that describe the…

Soft Condensed Matter · Physics 2009-10-30 Tao Sun , Anna C. Balazs , David Jasnow

The mesoscale rheology of a lamellar phase of a block copolymer is modeled as a structured fluid of uniaxial symmetry. The model predicts a viscoelastic response that depends on the angle between the the local lamellar planes and velocity…

Soft Condensed Matter · Physics 2013-01-14 Chi-Deuk Yoo , Jorge Vinals

We develop a theory to describe the reorientation phenomena in the lamellar phase of block copolymer melt under reciprocating shear flow. We show that similar to the steady-shear, the oscillating flow anisotropically suppresses fluctuations…

Soft Condensed Matter · Physics 2009-11-07 A. N. Morozov , J. G. E. M. Fraaije

Cell dynamics simulation is used to investigate the phase behavior of block copolymer/homopolymer mixture subjected to a steady shear flow. Phase transitions occur from transverse to parallel and then to perpendicular lamellar structure…

Soft Condensed Matter · Physics 2015-06-29 Y. Guo , J. Zhang , B. Wang , H. Wu , M. Sun , J. Pan

Uniform Shear Flow is a prototype nonequilibrium state admitting detailed study at both the macroscopic and microscopic levels via theory and computer simulation. It is shown that the hydrodynamic equations for this state have a long…

Condensed Matter · Physics 2009-10-28 Mirim Lee , James W. Dufty , José M. Montanero , Andrés Santos , James F. Lutsko

Shear-flow-induced structure formation in surfactant-water mixtures is investigated numerically using a meshless-membrane model in combination with a particle-based hydrodynamics simulation approach for the solvent. At low shear rates,…

Soft Condensed Matter · Physics 2013-07-02 Hayato Shiba , Hiroshi Noguchi , Gerhard Gompper

The stability of idealized shear flow at long wavelengths is studied in detail. A hydrodynamic analysis at the level of the Navier-Stokes equation for small shear rates is given to identify the origin and universality of an instability at…

Condensed Matter · Physics 2009-10-30 Jose M. Montanero , Andres Santos , Mirim Lee , James W. Dufty , J. F. Lutsko

The dynamics of microphase separation and the orientation of lamellae in diblock copolymers is investigated in terms of a mean-field model. The formation of lamellar structures and their stable states are explored and it is shown that…

Soft Condensed Matter · Physics 2015-06-15 Vanessa Weith , Alexei Krekhov , Walter Zimmermann

We use an off-lattice microscopic model for solutions of equilibrium polymers (EP) in a lamellar shear flow generated by means of a self-consistent external field between parallel hard walls. The individual conformations of the chains are…

Soft Condensed Matter · Physics 2009-10-31 A. Milchev , J. P. Wittmer , D. P. Landau

The shear viscosity in the dilute regime of a model for confined granular matter is studied by simulations and kinetic theory. The model consists on projecting into two dimensions the motion of vibrofluidized granular matter in shallow…

Statistical Mechanics · Physics 2015-06-22 Rodrigo Soto , Dino Risso , Ricardo Brito

We investigate shear-induced crystallization in a very dense flow of mono-disperse inelastic hard spheres. We consider a steady plane Couette flow under constant pressure and neglect gravity. We assume that the granular density is greater…

Soft Condensed Matter · Physics 2009-11-11 Evgeniy Khain , Baruch Meerson

We analyze the linear stability of monoclinal traveling waves on a constant incline, which connect uniform flowing regions of differing depths. The classical shallow-water equations are employed, subject to a general resistive drag term.…

Fluid Dynamics · Physics 2022-05-18 Jake Langham , Andrew J. Hogg
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