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Counterion distributions and effective electrostatic interactions between spherical macroions in polyelectrolyte solutions are calculated via second-order perturbation (linear response) theory. By modelling the macroions as continuous…

Soft Condensed Matter · Physics 2009-11-10 A. R. Denton

We study the ionic equilibria and interactions of neutral semi-permeable spherical shells immersed in electrolyte solutions, including polyions. Although the shells are uncharged, only one type of ions of the electrolyte can permeate them,…

Soft Condensed Matter · Physics 2012-07-24 Vladimir Lobaskin , Artem N. Bogdanov , Olga I. Vinogradova

The addition of co-solutes to colloidal suspensions is often employed to induce tunable depletion interactions. In this work we investigate effective colloidal interactions arising from binary co-solute mixtures of hard spheres and patchy…

Soft Condensed Matter · Physics 2021-08-25 Philip H. Handle , Emanuela Zaccarelli , Nicoletta Gnan

We have developed a simulation model to describe particle adsorption to and desorption from liquid interfaces. Using this model we formulate a closed interfacial equation of state for repulsive elastic spheres. The effect of a long-range…

Soft Condensed Matter · Physics 2011-02-24 Robert D. Groot , Simeon D. Stoyanov

The screened Coulomb interaction between a pair of infinite parallel planes with spatially varying surface charge is considered in the limit of small electrical potentials for arbitrary Debye lengths. A simple expression for the disjoining…

Classical Physics · Physics 2017-04-12 Sandip Ghosal , John D. Sherwood

We consider a fluid of $d$-dimensional spherical particles interacting via a pair potential $\phi(r)$ which takes a finite value $\epsilon$ if the two spheres are overlapped ($r<\sigma$) and 0 otherwise. This penetrable-sphere model has…

Statistical Mechanics · Physics 2015-06-29 L. Acedo , A. Santos

This paper describes the results of our theoretical and numerical studies of hydrodynamic interactions in a suspension of spherical particles confined between two parallel planar walls, under creeping-flow conditions. We propose a novel…

Soft Condensed Matter · Physics 2009-11-11 S. Bhattacharya , J. Blawzdziewicz , E. Wajnryb

Packing spheres efficiently in large dimension $d$ is a particularly difficult optimization problem. In this paper we add an isotropic interaction potential to the pure hard-core repulsion, and show that one can tune it in order to maximize…

Disordered Systems and Neural Networks · Physics 2018-06-28 Thibaud Maimbourg , Mauro Sellitto , Guilhem Semerjian , Francesco Zamponi

In this paper we study the electrostatic interaction of a heterogeneously charged wall with a neutral semipermeable membrane. The wall consists of periodic stripes, where the charge density varies in one direction. The membrane is in a…

Soft Condensed Matter · Physics 2017-02-08 Salim R. Maduar , Vladimir Lobaskin , Olga I. Vinogradova

The simplicity of hard spheres as a model system is deceptive. Although the particles interact solely through volume exclusion, that nevertheless suffices for a wealth of static and dynamical phenomena to emerge, making the model an…

We introduce a simple spherical model whose structural properties are similar to the ones generated by models with directional interactions, by employing a binary mixture of large and small hard spheres, with a square-well attraction acting…

Disordered Systems and Neural Networks · Physics 2009-11-13 Emanuela Zaccarelli , Francesco Sciortino , Piero Tartaglia

We study discrete solvent effects on the interaction of two parallel charged surfaces in ionic aqueous solution. These effects are taken into account by adding a bilinear non-local term to the free energy of Poisson-Boltzmann theory. We…

Soft Condensed Matter · Physics 2009-10-31 Yoram Burak , David Andelman

In this paper we propose a protocol to suppress double-layer forces between two microspheres immersed in a dielectric medium, being one microsphere metallic at a controlled potential {\psi}M and the other a charged one either metallic or…

Classical Physics · Physics 2018-02-21 D. S. Ether , F. S. S. Rosa , D. M. Tibaduiza , L. B. Pires , R. S. Decca , P. A. Maia Neto

The effective interaction between charged colloidal particles confined between two planar like-charged walls is investigated using computer simulations of the primitive model describing asymmetric electrolytes. In detail, we calculate the…

Soft Condensed Matter · Physics 2016-08-15 E. Allahyarov , I. D'Amico , H. Löwen

The effects of image charges (i.e., induced surface charges of polarization) in spherical geometry and their implication for charged colloidal systems are investigated. We study analytically and exactly a single microion interacting with a…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina

Effective electrostatic interactions between colloidal particles, coated with polyelectrolyte brushes and suspended in an electrolyte solvent, are described via linear response theory. The inner cores of the macroions are modeled as hard…

Soft Condensed Matter · Physics 2009-11-10 Hao Wang , Alan R. Denton

The analytical solution of the recently proposed ideal chain polymer mean-spherical approximation (Yu.Kalyuzhnyi, Mol.Phys., 94, 735(1998)) is presented for the multicomponent mixture of charged hard-sphere linear chain flexible molecules.…

Condensed Matter · Physics 2009-11-07 Yu. V. Kalyuzhnyi , P. T. Cummings

In this paper we study the electrostatic properties of `Janus' spheres with unequal charge densities on both hemispheres. We introduce a method to compare primitive-model Monte Carlo simulations of the ionic double layer with predictions of…

Soft Condensed Matter · Physics 2012-09-18 Joost de Graaf , Niels Boon , Marjolein Dijkstra , René van Roij

The possibility to induce demixing in a colloidal mixture by adding small polymers, or other equivalent depletant agents, is theoretically investigated. By use of Mean Field Theory, suitably generalized to deal with short range effective…

Soft Condensed Matter · Physics 2015-10-28 Alberto Parola , Luciano Reatto

We study the effective interaction between differently charged polyelectrolyte-colloid complexes in electrolyte solutions via Monte Carlo simulations. These complexes are formed when short and flexible polyelectrolyte chains adsorb onto…

Soft Condensed Matter · Physics 2010-05-05 D. Truzzolillo , F. Bordi , F. Sciortino , S. Sennato