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We consider capillary condensation transitions occurring in open slits of width $L$ and finite height $H$ immersed in a reservoir of vapour. In this case the pressure at which condensation occurs is closer to saturation compared to that…

Statistical Mechanics · Physics 2017-08-22 Alexandr Malijevský , Andrew O. Parry , Martin Pospíšil

We study the kinetics of the isotropic-smectic phase transition in a colloidal rod/polymer mixture by visualizing individual smectic layers. First, we show that the bulk isotropic-smectic phase transition is preceded by a surface freezing…

Soft Condensed Matter · Physics 2009-11-10 Zvonimir Dogic

We report a detailed account of the phase diagram of a recently introduced model for non-equilibrium wetting in 1+1 dimensions [Phys. Rev. Lett. 79, 2710 (1997)]. A mean field approximation is shown to reproduce the main features of the…

Statistical Mechanics · Physics 2007-05-23 H. Hinrichsen , R. Livi , D. Mukamel , A. Politi

A coupled phase-field and hydrodynamic model is introduced to describe a two-phase, weakly compressible smectic (layered phase) in contact with an isotropic fluid of different density. A non-conserved smectic order parameter is coupled to a…

Soft Condensed Matter · Physics 2022-02-02 Eduardo Vitral , Perry H. Leo , Jorge Viñals

We study the structure and morphological changes of fluids that are in contact with solid composites formed by alternating and microscopically wide stripes of two different materials. One type of the stripes interacts with the fluid via…

Statistical Mechanics · Physics 2019-12-30 Martin Pospíšil , Martin Láska , Alexandr Malijevský

The glass transition can simply be viewed as the point at which the viscosity of a structurally disordered liquid reaches 10^{13} Poise [1]. This definition is operational but it sidesteps fundamental controversies about the glass: Is the…

Statistical Mechanics · Physics 2017-05-10 Ludger Santen , Werner Krauth

A full characterization of the water flow past a silicon superhydrophobic surface with longitudinal micro-grooves enclosed in a microfluidic device is presented. Fluorescence microscopy images of the flow seeded with fluorescent passive…

Fluid Dynamics · Physics 2014-06-13 Guido Bolognesi , Cecile Cottin-Bizonne , Christophe Pirat

The problem of the gas-liquid heterophase fluctuations of a fluid within the critical and supercritical regions is revisited. To describe the thermodynamics and structure of the heterophase fluid, the mesoscopic equation of state is…

Statistical Mechanics · Physics 2015-08-21 A. S. Bakai

We consider the location and order of capillary condensation transitions occurring in deep grooves of width $L$ and depth $D$. For walls that are completely wet by liquid (contact angle $\theta=0$) the transition is continuous and its…

Statistical Mechanics · Physics 2018-04-18 A. Malijevský , A. Parry

An electronically coarse-grained model for water reveals a persistent vestige of the liquid-gas transition deep into the supercritical region. A crossover in the density dependence of the molecular dipole arises from the onset of…

Statistical Mechanics · Physics 2015-09-15 V. P. Sokhan , A. Jones , F. S. Cipcigan , J. Crain , G. J. Martyna

We present a theoretical study of wetting phenomena and interactions between liquid-vapor interfaces based on the density functional theory. The focus is mostly on the impact of long-range van der Waals interactions both within the fluid…

Chemical Physics · Physics 2011-11-10 Arik Yochelis , Len M. Pismen

This is a summarising investigation of the events of the phase transition of the first order that occur in the critical region below the liquid-gas critical point. The grand partition function has been completely integrated in the…

Statistical Mechanics · Physics 2015-01-13 I. R. Yukhnovskii

When a fluid is constrained to a fixed, finite volume, the conditions for liquid-vapor equilibrium are different from the infinite volume or constant pressure cases. There is even a range of densities for which no bubble can form, and the…

Chemical Physics · Physics 2023-09-19 Frédéric Caupin

A phase diagram of argon based upon percolation transition loci determined from literature experimental density-pressure isotherms, and simulation values using a Lennard-Jones model shows three fluid phases. The liquid phase spans all…

Statistical Mechanics · Physics 2012-06-14 Leslie V. Woodcock

We present the first microscopic images of the prewetting transition of a liquid film on a solid surface. Pictures of the local coverage map of a helium film on a cesium metal surface are taken while the temperature is raised through the…

Condensed Matter · Physics 2015-06-24 X. Muller , J. Dupont-Roc

A computational fluid dynamics (CFD) model is developed to simulate the dynamics of meniscus formation and capillary flow between vertical parallel plates. The arbitrary Lagrangian-Eulerian (ALE) approach was employed to predict and…

Fluid Dynamics · Physics 2020-03-12 Mohammad Naghashnejad , Hamidreza Shabgard

An approach based on a lattice version of the Boltzmann kinetic equation for describing multi-phase flows in nano- and micro-corrugated devices is proposed. We specialize it to describe the wetting/dewetting transition of fluids in presence…

Cellular Automata and Lattice Gases · Physics 2007-06-13 R. Benzi , L. Biferale , M. Sbragaglia , S. Succi , F. Toschi

Multicanonical ensemble sampling simulations have been performed to calculate the phase diagram of a Lennard-Jones fluid embedded in a fractal random matrix generated through diffusion limited cluster aggregation. The study of the system at…

Statistical Mechanics · Physics 2015-06-25 V. De Grandis , P. Gallo , M. Rovere

The liquid-vapour phase transition near a weakly attractive surface is studied by simulations of the coexistence curves of water in hydrophobic pores. There is a pronounced gradual density depletion of the liquid phase near the surface…

Statistical Mechanics · Physics 2009-11-10 I. Brovchenko , A. Geiger , A. Oleinikova

This paper presents a numerical analysis of the transition from selective withdrawal to viscous entrainment. In our model problem, an interface between two immiscible layers of equal viscosity is deformed by an axisymmetric withdrawal flow,…

Fluid Dynamics · Physics 2007-05-23 Marko Kleine Berkenbusch , Itai Cohen , Wendy W. Zhang