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We calculate low-frequency Raman scattering from the confined acoustic phonon modes of CdS1-xSex nanoparticles embedded in borosilicate glass. The calculation of the Raman scattering by acoustic phonons in nanoparticles has been performed…

Mesoscale and Nanoscale Physics · Physics 2009-04-16 Sanjeev K. Gupta , Prafulla K. Jha , Satyaprakash Sahoo , A. K. Arora , Y. M. Azhniuk

Strong light-matter coupling gives rise to polaritons -- quasiparticles that combine both photonic and material characteristics. Here, we show that polar nanocrystals exhibit structure- and environment-dependent Raman scattering, enabled by…

We have found that the polarization dependence of Raman scattering in organic crystals at finite temperatures can only be described by a fourth-rank formalism. This generalization of the second-rank Raman tensor $\mathcal{R}$ stems from the…

We use polarization-resolved Raman scattering to study lattice dynamics in NaFe$_{0.53}$Cu$_{0.47}$As single crystals. We identify 4 $A_{1g}$ phonon modes at 125, 172, 183 and 197 cm$^{-1}$, and 4 $B_{3g}$ phonon modes at 101, 138, 173, 226…

Superconductivity · Physics 2018-09-19 W. -L. Zhang , Y. Song , W. -Y. Wang , C. -D. Cao , P. -C. Dai , G. Blumberg

A new numerical method is introduced for calculating the polarizability of an arbitrary dielectric object with position dependent complex permittivity. Three separate numerical approaches are provided to calculate the dipole moment of a…

Materials Science · Physics 2022-03-18 Daniel B. Murray , Caleb H. Netting , Robin D. Mercer , Lucien Saviot

In our recent paper [Phys. Rev. B 65, 075316 (2002)], the selection rules for the Raman scattering in spherical nanocrystals are analyzed. Here we show, that a physically expedient choice of the coordinate system, related to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 E. P. Pokatilov , S. N. Klimin , V. M. Fomin , J. T. Devreese , F. W. Wise

Confined acoustic and optical phonons in Si nanoclusters embedded in sapphire, synthesized using ion-beam implantation are investigated using Raman spectroscopy. The l = 0 and l = 2 confined acoustic phonons, found at low Raman shift, are…

Materials Science · Physics 2008-09-10 Satyaprakash Sahoo , S. Dhara , S. Mahadevan , A. K. Arora

Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ is one of the simplest representatives of the class of lead relaxors and often serves as a model system for more complicated compounds. In this paper we analyse both polarized and depolarized Raman scattering…

Materials Science · Physics 2009-11-10 Oleksiy Svitelskiy , Jean Toulouse , Z. -G. Ye

Multi-phonon Raman scattering in semiconductor nanocrystals is treated taking into account both adiabatic and non-adiabatic phonon-assisted optical transitions. Because phonons of various symmetries are involved in scattering processes,…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 E. P. Pokatilov , S. N. Klimin , V. M. Fomin , J. T. Devreese , F. W. Wise

Raman scattering on phonon--plasmon coupled modes in high magnetic fields is considered theoretically. The calculations of the dielectric function were performed in the long-wave approximation for the semiclassical and ultra-quantum…

Materials Science · Physics 2007-05-23 L. A. Falkovsky

Phonon modes found in low frequency Raman scattering from $CdS_{1-x}Se_x$ nanocrystals embedded in borosilicate glass arising from confined acoustic phonons are investigated. In addition to the breathing modes and quadrupolar modes, two…

Materials Science · Physics 2008-03-10 Sanjeev K. Gupta , Satyaprakash Sahoo , Prafulla K. Jha , A. K. Arora , Y. M. Azhniuk

Optical properties of the lead halide perovskites nanocrystals are controlled by confined excitons and rich spectrum of confined acoustic and optical phonons. We study experimentally and theoretically the exciton-phonon interaction in…

We demonstrate the determination of anharmonic acoustic phonon properties via second-order Raman scattering exemplarily on copper iodide single crystals. The origin of multi-phonon features from the second-order Raman spectra was assigned…

Extending the idea of optical microcavities to sound waves, we propose a {\it phonon cavity} consisting of two semiconductor superlattices enclosing a spacer with thickness determined by the acoustic wavelength at the center of the first…

Condensed Matter · Physics 2009-11-07 M. Trigo , A. Bruchhausen , A. Fainstein , B. Jusserand , V. Thierry-Mieg

An experimental study of optical phonon modes, both normal and interface (IF) phonons, in bilayer strain-coupled InAs/GaAs_(1-x)Sb_x quantum dot heterostructures has been presented by means of low-temperature polarized Raman scattering. The…

Mesoscale and Nanoscale Physics · Physics 2024-09-17 Priyesh Kumar , Sudip Kumar Deb , Subhananda Chakrabarti , Jhuma Saha

The scattering of lattice excitations (phonons) with the photoexcited charge carriers is of a major concern in optoelectronic devices. Here, the resonant Raman scattering will be utilized to study an exciton-phonon interaction in GaN…

A modified phonon confinement model considering the size distribution, an improved phonon dispersion curve and a confinement function is developed for the calculation of size dependent Raman spectra of the silicon (Si) nanocrystals. The…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Sanjeev K. Gupta , Prafulla K. Jha

There is still a gap in understanding phonons scattering by geometrical defects at the nanoscale, and it remains a significant challenge for heat transfer management in nanoscale devices and systems. In this study, we aim to explore the…

Mesoscale and Nanoscale Physics · Physics 2024-03-19 Mykola Isaiev , Nataliia Kyrychenko , Vasyl Kuryliuk , David Lacroix

Low-frequency Raman scattering spectra are presented for gold nanocrystals with diameters 3.5 and 13 nm. The frequencies of the Raman peaks but also their number are shown to vary with the nanocrystal size. These results are analyzed using…

Mesoscale and Nanoscale Physics · Physics 2012-02-09 Lucien Saviot , Nicolas Combe , Adnen Mlayah

Polarized Raman scattering measurements have been performed on Na0.5CoO2 single crystal from 8 to 305 K. Both the A1g and E1g phonon modes show a softening below Tc1 ~ 83 K. Additionally, the A1g phonon mode, which is forbidden in the…

Strongly Correlated Electrons · Physics 2008-02-07 Q. M. Zhang , M. an , S. K. Yuan , Y. Wu , D. Wu , J. L. Luo , N. L. Wang , W. Bao , Y. N. Wang
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