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Electrons in condensed matter may transition into a variety of broken-symmetry phase states due to electron-electron interactions. Applying diverse mean-field approximations to the interaction term is arguably the simplest way to identify…

Strongly Correlated Electrons · Physics 2024-06-17 Maxim Trushin , Liangtao Peng , Gargee Sharma , Giovanni Vignale , Shaffique Adam

Large-bipolaron superconductivity is plausible with carrier densities well below those of conventional metals. Bipolarons form when carriers self-trap in pairs. Coherently moving large-bipolarons require extremely large ratios of static to…

Superconductivity · Physics 2017-05-31 David Emin

We study the interactions between two negatively charged macroscopic surfaces confining positive counterions. A density-functional approach is introduced which, besides the usual mean-field interactions, takes into account the correlations…

Soft Condensed Matter · Physics 2015-06-25 A. Diehl , M. N. Tamashiro , Marcia C. Barbosa , Yan Levin

Effect of ionic solute on a near-critical binary aqueous mixture confined between charged walls with different adsorption preferences is considered within a simple density functional theory. For the near-critical system containing small…

Soft Condensed Matter · Physics 2015-05-28 F. Pousaneh , A. Ciach

We investigate the ion distribution and overcharging at charged interfaces with dielectric inhomogeneities in the presence of asymmetric electrolytes containing polyvalent and monovalent ions. We formulate an effective "dressed counterion"…

Soft Condensed Matter · Physics 2015-03-17 Matej Kanduc , Ali Naji , Jan Forsman , Rudolf Podgornik

In order to better understand the collapse of polyions in poor solvent conditions the effective charge and the solvent quality of the hypothetically uncharged polymer backbone need to be known. In the present work this is achieved by…

The mutual electromagnetic correlations between two spatially separated systems gives rise to Casimir and Casimir-Polder effect. The corresponding forces, which are generally attractive for most vacuum-separated metallic or dielectric…

Mesoscale and Nanoscale Physics · Physics 2016-07-13 Partha Goswami

We consider the interactions between two uncharged planar macroscopic surfaces immersed in an electrolyte solution which are induced by interfacial selectivity. These forces are taken into account by introducing a depletion free-energy…

Soft Condensed Matter · Physics 2009-10-31 M. N. Tamashiro , P. Pincus

The recently developed modified Donnan (mD) model provides a simple and useful description of the electrical double layer in microporous carbon electrodes, suitable for incorporation in porous electrode theory. By postulating an attractive…

Chemical Physics · Physics 2014-01-22 P. M. Biesheuvel , S. Porada , M. Levi , M. Z. Bazant

We investigate the influence of geometric confinement on the free energy of an idealized model for charge-stabilized colloidal suspensions. The mean-field Poisson-Boltzmann formulation for this system predicts pure repulsion among…

Soft Condensed Matter · Physics 2009-11-07 Ajay Gopinathan , Tong Zhou , S. N. Coppersmith , L. P. Kadanoff , David G. Grier

We revisit the role of attractions in liquids and apply these concepts to colloidal suspensions. Two means are used to investigate the structure; the pair correlation function and a recently developed topological method. The latter…

Soft Condensed Matter · Physics 2011-01-11 Jade Taffs , Alex Malins , Stephen R. Williams , C. Patrick Royall

We present further evidence that gelation is an arrested phase separation in attractive colloid-polymer mixtures, based on a method combining confocal microscopy experiments with numerical simulations recently established in {\bf Nature…

Soft Condensed Matter · Physics 2009-11-13 Emanuela Zaccarelli , Peter J. Lu , Fabio Ciulla , David. A. Weitz , Francesco Sciortino

The effective interaction between charged colloidal particles confined between two planar like-charged walls is investigated using computer simulations of the primitive model describing asymmetric electrolytes. In detail, we calculate the…

Soft Condensed Matter · Physics 2016-08-15 E. Allahyarov , I. D'Amico , H. Löwen

When an ionic liquid adsorbs onto a porous electrode, its ionic arrangement is deeply modified due to a screening of the Coulombic interactions by the metallic surface and by the confinement imposed upon it by the electrode's morphology. In…

Within the framework of a Modified Poisson-Boltzmann theory accounting for steric effects of microions, we prove analytically that the effective pair interactions between like-charge colloids immersed in a confined electrolyte are…

Soft Condensed Matter · Physics 2009-10-31 E. Trizac , J-L Raimbault

We study the ionic equilibria and interactions of neutral semi-permeable spherical shells immersed in electrolyte solutions, including polyions. Although the shells are uncharged, only one type of ions of the electrolyte can permeate them,…

Soft Condensed Matter · Physics 2012-07-24 Vladimir Lobaskin , Artem N. Bogdanov , Olga I. Vinogradova

We present some recent theory and simulation results addressing the phenomena of colloidal gelation at both high and low volume fractions, in the presence of short-range attractive interactions. We discuss the ability of mode-coupling…

Soft Condensed Matter · Physics 2009-11-10 M. E. Cates , M. Fuchs , K. Kroy , W. C. K. Poon , A. M. Puertas

Electronic charge carriers in ionic materials can self-trap to form large polarons. Interference between the ionic displacements associated with oppositely charged large polarons increases as they approach one another. Initially this…

Other Condensed Matter · Physics 2018-02-05 David Emin

We predict the nature (attractive or repulsive) and range (exponentially screened or long-range power law) of the electrostatic interactions of oppositely charged and planar plates as a function of the salt concentration and surface charge…

Soft Condensed Matter · Physics 2012-01-31 Dan Ben-Yaakov , Yoram Burak , David Andelman , S. A. Safran

A theory is presented which allows us to accurately calculate the density profile of monovalent and multivalent counterions in suspensions of polarizable colloids or nano-particles. In the case of monovalent ions, we derive a weak-coupling…

Soft Condensed Matter · Physics 2011-09-23 Amin Bakhshandeh , Alexandre Pereira dos Santos , Yan Levin