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The physics of doping a Mott insulator is investigated in the presence of a solid-vacuum interface. Using the embedding approach for dynamical mean field theory we show that the change in surface spectral evolution in a doped Mott insulator…

Strongly Correlated Electrons · Physics 2011-07-12 Reza Nourafkan , Frank Marsiglio

The Mott insulator LaVO$_3$ is known to become metallic if La is replaced by small concentrations of Ca. Since surface quasi-particle spectra of various perovskites are more strongly correlated than their bulk spectra, the coexistence of a…

Strongly Correlated Electrons · Physics 2007-05-23 A. Liebsch

The spectral weight evolution of the low-dimensional Mott insulator TiOCl upon alkali-metal dosing has been studied by photoelectron spectroscopy. We observe a spectral weight transfer between the lower Hubbard band and an additional peak…

Strongly Correlated Electrons · Physics 2015-05-13 M. Sing , S. Glawion , M. Schlachter , M. R. Scholz , K. Goss , J. Heidler , G. Berner , R. Claessen

The spectral properties of a one-dimensional (1D) single-chain Mott insulator Sr$_2$CuO$_{3}$ have been studied in angle-resolved photoemission and optical spectroscopy, at half filling and with small concentrations of extra charge doped…

Strongly Correlated Electrons · Physics 2008-03-04 T. Valla , T. E. Kidd , P. D. Johnson , K. W. Kim , C. C. Homes , G. D. Gu

Since the discovery of half-filled cuprate to be a Mott insulator, the excitation spectra above the chemical potential for the unoccupied states has attracted many research attentions. There were many theoretical works using different…

Superconductivity · Physics 2017-01-25 Huan-Kuang Wu , Ting-Kuo Lee

We study evolution of metals from Mott insulators in the carrier-doped 2D Hubbard model using a cluster extension of the dynamical mean-field theory. While the conventional metal is simply characterized by the Fermi surface (pole of the…

Strongly Correlated Electrons · Physics 2009-11-13 Shiro Sakai , Yukitoshi Motome , Masatoshi Imada

The filling-controlled metal-insulator transition (MIT) in a two-dimensional Mott-Hubbard system La1.17-xPbxVS3.17 has been studied by photoemission spectroscopy. With Pb substitution x, chemical potential mu abruptly jumps by ~ 0.07 eV…

Strongly Correlated Electrons · Physics 2009-11-10 A. Ino , T. Okane , S. -I. Fujimori , A. Fujimori , T. Mizokawa , Y. Yasui , T. Nishikawa , M. Sato

Unravelling the nature of doping-induced transition between a Mott insulator and a weakly correlated metal is crucial to understanding novel emergent phases in strongly correlated materials. For this purpose, we study the evolution of…

Strongly Correlated Electrons · Physics 2018-03-14 Yao Wang , Brian Moritz , Cheng-Chien Chen , Thomas P. Devereaux , Krzysztof Wohlfeld

In a recent Comment [arXiv:0904.0454] on our Letter [Phys. Rev. Lett. 102, 056404 (2009); arXiv:0809:0950], Phillips criticizes one specific issue discussed in our paper, concerning the spectral weight transfer, among our wide-ranging…

Strongly Correlated Electrons · Physics 2009-04-16 Shiro Sakai , Yukitoshi Motome , Masatoshi Imada

We present experimental photoemission and inverse photoemission spectra of SrTiO$_{3- \delta}$ representing electron doped $d^0$ systems. Photoemission spectra in presence of electron doping exhibit prominent features arising from electron…

Condensed Matter · Physics 2016-08-31 D. D. Sarma , S. R. Barman , H. Kajueter , G. Kotliar

The doping induced insulator-metal transition in $La_{1-x}Sr_{x}TiO_{3}$ is studied using the ab-initio LDA+DMFT method. Combining the LDA bandstructure for the actual, distorted structure found recently with multi-orbital DMFT to treat…

Strongly Correlated Electrons · Physics 2016-08-31 L. Craco , M. S. Laad , S. Leoni , E. Müller-Hartmann

The insulator to metal transition in LaTiO_3 induced by La substitution via Sr is studied within multi-band exact diagonalization dynamical mean field theory at finite temperatures. It is shown that weak hole doping triggers a large…

Strongly Correlated Electrons · Physics 2009-11-13 A. Liebsch

We investigate a hole-doped Mott insulator in a slab geometry using the dynamical cluster approximation. We show that the enhancement of the correlation strength at the surface results in the remarkable evolution of the layer-projected…

Strongly Correlated Electrons · Physics 2025-11-05 Gregorio Staffieri , Michele Fabrizio

We have performed x-ray absorption spectroscopy (XAS) and x-ray photoemission spectroscopy (XPS) studies of single crystal Ba_{1-x}K_{x}BiO_{3} (BKBO) covering the whole composition range $0 \leq x \leq 0.60$. Several features in the oxygen…

Superconductivity · Physics 2009-10-31 K. Kobayashi , T. Mizokawa , A. Ino , J. Matsuno , A. Fujimori , H. Samata , A. Mishiro , Y. Nagata , F. M. F. de Groot

How a Mott insulator develops into a weakly coupled metal upon doping is a central question to understanding various emergent correlated phenomena. To analyze this evolution and its connection to the high-$T_c$ cuprates, we study the…

We have analyzed experimental evidence for an anomalous transfer of spectral weight from high to low energy scales in both electron and hole doped cuprates as a function of doping. X-ray scattering, optical and photoemission spectra are all…

Superconductivity · Physics 2010-12-06 R. S. Markiewicz , Tanmoy Das , A. Bansil

We have studied the critical behaviour of a doped Mott insulator near the metal-insulator transition for the infinite-dimensional Hubbard model using a linearized form of dynamical mean-field theory. The discontinuity in the chemical…

Strongly Correlated Electrons · Physics 2009-11-07 Y. Ono , R. Bulla , A. C. Hewson , M. Potthoff

We investigate the effect of spatial doping of the Mott insulator LaVO$_3$ by inserting a few layers of the correlated metal SrVO$_3$ in multilayer geometries. Using density functional theory in combination with dynamical mean-field theory,…

Strongly Correlated Electrons · Physics 2022-12-22 Sophie Beck , Claude Ederer

The evolution of the electronic structures of strongly correlated insulators with doping has long been a central fundamental question in condensed matter physics; it is also of great practical relevance for applications. We have studied the…

We investigate experimentally the ultrafast changes in the spectral response of the Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl ($\kappa$-Cl) upon photodoping with intense excitation at 1.6 eV and probing with continuum pulses…

Strongly Correlated Electrons · Physics 2023-10-31 Konstantin Warawa , Yassine Agarmani , Harald Schubert , Martin Dressel , Michael Lang , Hartmut G. Roskos , Mark D. Thomson
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