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The optical excitations in C$_{60}$ and higher fullerenes, including isomers of C$_{76}$, C$_{78}$, and C$_{84}$, are theoretically investigated. We use a tight binding model with long-range Coulomb interactions, treated by the Hartree-Fock…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya

Nonlinear optical properties of extracted higher fullerenes - C70, C76, C78, and C84 - are theoretically investigated. Magnitudes of off-resonant third-harmonic-generation are calculated by the intermediate exciton theory. We find that…

Condensed Matter · Physics 2008-02-03 K. Harigaya

Effects of Coulomb interactions and lattice fluctuations in the optical absorption spectra of C60 and C70 are theoretically investigated by using a tight binding model with long-range Coulomb interaction and bond disorder. Anisotropy…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya , Shuji Abe

Optical absorption spectra of higher fullerenes (C70 and C76) as well as of C60 are calculated by a tight binding model with a long range Coulomb interaction. A reasonable parameter set gives calculated spectra which are in overall…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya

Molecular exciton effects in the neutral and maximally doped C$_{60}$ (C$_{70}$) are considered using a tight binding model with long-range Coulomb interactions and bond disorder. By comparing calculated and observed optical spectra, we…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya , Shuji Abe

Molecular exciton effects in the neutral and maximally doped C60 (C70) are considered using a tight binding model with long-range Coulomb interactions and bond disorder. By comparing calculated and observed optical spectra, we conclude that…

chem-ph · Physics 2008-02-03 Kikuo Harigaya , Shuji Abe

The third-order nonlinear optical susceptiblity chi(3) of a C60 molecule is calculated by using a free-electron model as well as by taking Coulomb interactions into account. The free-electron model yields chi(3) magnitudes which are in…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya , Shuji Abe

Optical absorption spectra of C60^6- are theoretically investigated in order to analyze the optical properties of alkali metal doped fullerites A6C60. We use a tight binding model with long ranged Coulomb interactions and bond disorder.…

Condensed Matter · Physics 2009-10-22 Kikuo Harigaya

Motivated by the recent experimental report of a possible light-induced superconductivity in A3C60 at high temperature [Mitrano et al., Nature 530, 451 (2016)], we investigate theoretical mechanisms for enhanced superconductivity in A3C60…

Strongly Correlated Electrons · Physics 2016-11-01 Minjae Kim , Yusuke Nomura , Michel Ferrero , Priyanka Seth , Olivier Parcollet , Antoine Georges

The multiplet structure induced by the Coulomb interactions in C$_{60}^{n-}$ ($n = 1 - 12$) is analyzed. The partially ocuppied LUMO gives rise to a set of levels which fill a relatively wide band ( $\approx 2-3$ eV ). A large ($\sim 1$ eV)…

Condensed Matter · Physics 2009-10-22 F. Guinea , J. Gonzalez , M. A. H. Vozmediano

We present a systematic theory of Coulomb interaction effects in the nonlinear optical processes in semiconductors using a perturbation series in the exciting laser field. The third-order dynamical response consists of phase-space filling…

Condensed Matter · Physics 2009-10-31 Th. Oestreich , K. Schoenhammer , L. J. Sham

The optical excitations in $\rug$ and higher fullerenes, including isomers of C$_{76}$, C$_{78}$, and C$_{84}$, are theoretically investigated. We use a tight binding model with long-range Coulomb interactions, treated by the Hartree-Fock…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

A theory of optical excitations by using a tight binding model with long-range Coulomb interactions is developed. The model is applied to a C60 molecule and a cluster, and is treated by the Hartree-Fock approximation followed by a…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya , Shuji Abe

We theoretically investigate optical absorption spectra of $\soc^{6-}$ and $\rug^{6-}$, and discuss relations with the optical properties of alkali metal doped fullerides $A_6\soc$ and $A_6\rug$. This is a valid approach for systems where…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya

We theoretically investigate the nonlinearity of trion-polaritons in a two-dimensional material that arises from Coulomb interaction between quasiparticles. To evaluate the interaction constant, we solve a three-body Wannier equation…

Mesoscale and Nanoscale Physics · Physics 2022-07-08 Kok Wee Song , Salvatore Chiavazzo , Ivan A. Shelykh , Oleksandr Kyriienko

We compute, based on density-functional electronic-structure calculations, the Coulomb couplings in the h_u highest occupied orbital of molecular C60. We obtain a multiplet-averaged Hubbard U ~ 3 eV, and four Hund-rule-like intra-molecular…

Strongly Correlated Electrons · Physics 2016-06-22 Martin Lueders , Andrea Bordoni , Nicola Manini , Andrea Dal Corso , Michele Fabrizio , Erio Tosatti

We demonstrate that in the presence of Coulomb interactions, electrons in graphene behave like a critical system, supporting power law correlations with interaction-dependent exponents. An asymptotic analysis shows that the origin of this…

Strongly Correlated Electrons · Physics 2010-05-04 Jianhui Wang , H. A. Fertig , Ganpathy Murthy

We theoretically investigate the effects of Coulomb interaction, at the level of unscreened Hartree-Fock approximation, on third harmonic generation of undoped graphene in an equation of motion framework. The unperturbed electronic states…

Mesoscale and Nanoscale Physics · Physics 2020-01-01 J. L. Cheng , J. E. Sipe , Chunlei Guo

The polarizability of twisted bilayer graphene, due to the combined effect of electron-hole pairs, plasmons, and acoustic phonons is analyzed. The screened Coulomb interaction allows for the for- mation of Cooper pairs and superconductivity…

Strongly Correlated Electrons · Physics 2021-08-12 Tommaso Cea , Francisco Guinea

Recent fluorescence spectroscopy experiments on single wall carbon nanotubes reveal substantial deviations of observed absorption and emission energies from predictions of noninteracting models of the electronic structure. Nonetheless, the…

Materials Science · Physics 2009-11-10 C. L. Kane , E. J. Mele
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