English

Nonlinear optical response in higher fullerenes

Condensed Matter 2008-02-03 v1 Chemical Physics Optics

Abstract

Nonlinear optical properties of extracted higher fullerenes - C70, C76, C78, and C84 - are theoretically investigated. Magnitudes of off-resonant third-harmonic-generation are calculated by the intermediate exciton theory. We find that optical nonlinearities of higher fullerenes are a few times larger than those of C60. The magnitudes of nonlinearity tend to increase as the optical gap decreases in higher fullerenes.

Cite

@article{arxiv.cond-mat/9702181,
  title  = {Nonlinear optical response in higher fullerenes},
  author = {K. Harigaya},
  journal= {arXiv preprint arXiv:cond-mat/9702181},
  year   = {2008}
}

Comments

Condensed Matter Theory Group at ETL: http://www.etl.go.jp/Organization/Bussei-kiso/

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