English

Enhancement of optical switching parameter and third-order optical nonlinearities in embedded Si nanocrystals: a theoretical assessment

Materials Science 2016-08-17 v1

Abstract

Third-order bound-charge electronic nonlinearities of Si nanocrystals (NCs) embedded in a wide band-gap matrix representing silica are theoretically studied using an atomistic pseudopotential approach. Nonlinear refractive index, two-photon absorption and optical switching parameter are examined from small clusters to NCs up to a size of 3 nm. Compared to bulk values, Si NCs show higher third-order optical nonlinearities and much wider two-photon absorption threshold which gives rise to enhancement in the optical switching parameter.

Keywords

Cite

@article{arxiv.0804.2581,
  title  = {Enhancement of optical switching parameter and third-order optical nonlinearities in embedded Si nanocrystals: a theoretical assessment},
  author = {Hasan Yıldırım and Ceyhun Bulutay},
  journal= {arXiv preprint arXiv:0804.2581},
  year   = {2016}
}

Comments

8 pages, 3 figures, to be published in Optics Communications