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A partially miscible binary liquid mixture, composed of A and B particles, is considered theoretically under conditions for which a stable A-rich liquid phase is in thermal equilibrium with the vapor phase. The B-rich liquid is metastable.…

Soft Condensed Matter · Physics 2021-04-28 Hyojeong Kim , Lothar Schimmele , S. Dietrich

We investigate the phase behaviour of 2D mixtures of bi-functional and three-functional patchy particles and 3D mixtures of bi-functional and tetra-functional patchy particles by means of Monte Carlo simulations and Wertheim theory. We…

We present a quantitative comparison between extensive Monte Carlo simulations and self-consistent field calculations on the phase diagram and wetting behavior of a symmetric, binary (AB) polymer blend confined into a film. The flat walls…

Statistical Mechanics · Physics 2009-10-31 M. Mueller , K. Binder

We deduce the mixing-demixing phase diagram for binary liquid mixtures in an electric field for various electrode geometries and arbitrary constitutive relation for the dielectric constant. By focusing on the behavior of the liquid-liquid…

Soft Condensed Matter · Physics 2013-07-18 Jennifer Galanis , Yoav Tsori

Employing simplified models in computer simulation is on the one hand often enforced by computer time limitations but on the other hand it offers insights into the molecular properties determining a given physical phenomenon. We employ this…

Statistical Mechanics · Physics 2008-04-18 Bortolo Matteo Mognetti , Martin Oettel , Leonid Yelash , Peter Virnau , Wolfgang Paul , Kurt Binder

Specialized Monte Carlo simulations and the moment free energy (MFE) method are employed to study liquid-gas phase equilibria in size-disperse fluids. The investigation is made subject to the constraint of fixed polydispersity, i.e. the…

Soft Condensed Matter · Physics 2009-11-10 Nigel B. Wilding , Moreno Fasolo , Peter Sollich

The liquid and crystal phase of a single-component Fermi gas with dipolar interactions are investigated using quantum Monte Carlo methods in two spatial dimensions and at zero temperature. The dipoles are oriented by an external field…

Quantum Gases · Physics 2013-05-30 N. Matveeva , S. Giorgini

We study a three-dimensional system of particles interacting via spherically-symmetric pair potentials consisting of several discontinuous steps. We show that at certain values of the parameters desribing the potential, the system has three…

Soft Condensed Matter · Physics 2015-06-24 Sergey V. Buldyrev , H. Eugene Stanley

We report a joint simulation and theoretical study of the liquid-vapor phase behaviour of a fluid in which polydispersity in the particle size couples to the strength of the interparticle interactions. Attention is focussed on the case in…

Statistical Mechanics · Physics 2009-11-11 Nigel B. Wilding , Peter Sollich , Moreno Fasolo , Matteo Buzzacchi

The liquid-gas phase diagram for polydisperse dipolar hard-sphere fluid with polydispersity in the hard-sphere size and dipolar moment is calculated using extension of the recently proposed thermodynamic perturbation theory for central…

Soft Condensed Matter · Physics 2012-07-16 Yu. V. Kalyuzhnyi , S. Hlushak , P. T. Cummings

We propose a method for describing a phase behavior of a system consisting of particles of two sorts. The interaction of each species is described by interaction potentials containing the repulsive and attractive components. Asymmetry is…

Statistical Mechanics · Physics 2020-06-19 M. P. Kozlovskii , O. A. Dobush

We describe a Monte Carlo scheme for the grand canonical simulation study of fluid phase equilibria in highly size-asymmetrical binary mixtures. The method utilizes an expanded ensemble in which the insertion and deletion of large particles…

Soft Condensed Matter · Physics 2015-05-18 Douglas J. Ashton , Nigel B. Wilding

Using event driven molecular dynamics simulations, we study a three dimensional one-component system of spherical particles interacting via a discontinuous potential combining a repulsive square soft core and an attractive square well. In…

Soft Condensed Matter · Physics 2009-11-10 A. Skibinsky , S. V. Buldyrev , G. Franzese , G. Malescio , H. E. Stanley

Using Monte Carlo simulation techniques, we calculate the phase diagram for a square shoulder-square well potential in two dimensions that has been previously shown to exhibit liquid anomalies consistent with a metastable liquid-liquid…

Soft Condensed Matter · Physics 2015-06-04 Ahmad M. Almudallal , Sergey V. Buldyrev , Ivan Saika-Voivod

A model of polar fluid is studied theoretically. The interaction potential, in addition to dipole-dipole term, possesses a dispersion contribution of the van der Waals-London form. It is found that when the dispersion force is comparable to…

Soft Condensed Matter · Physics 2009-10-31 Yan Levin , Paulo S. Kuhn , Marcia C. Barbosa

The microscopic approach to the description of the phase behaviour and critical phenomena in binary fluid mixtures is proposed. It is based on the method of collective variables with a reference system. The physical nature of the order…

Condensed Matter · Physics 2009-10-31 O. V. Patsahan

The blinking-checkers model [F. Caupin and M. A. Anisimov, Phys. Rev. Lett, 127,185701 (2021)] is a minimal lattice model which has demonstrated that, in the meanfield approximation, it can reproduce the phenomenon of fluid polyamorphism.…

Statistical Mechanics · Physics 2024-06-18 Sergey V. Buldyrev , Thomas J. Longo , Frederic Caupin , Mikhail A. Anisimov

We formulate the scaled particle theory for a general mixture of hard isosceles triangles and calculate different phase diagrams for the one-component fluid and for certain binary mixtures. The fluid of hard triangles exhibits a complex…

Soft Condensed Matter · Physics 2018-05-16 Yuri Martinez-Raton , Ariel Diaz-De Armas , Enrique Velasco

A previously developed fundamental measure fucntional [J. Chem. Phys. vol.107, 6379 (1997)] is used to study the phase behavior of a system of parallel hard cubes. The single-component fluid exhibits a continuous transition to a solid with…

Soft Condensed Matter · Physics 2009-10-31 Y. Martinez-Raton , J. A. Cuesta

The phase behavior of a system composed of spherical particles with a monomodal size distribution is investigated theoretically within the context of the van der Waals approximation for polydisperse fluids. It is shown how the binodals,…

Statistical Mechanics · Physics 2009-10-31 L. Bellier-Castella , H. Xu , M. Baus