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We study the phase behavior of mixtures of monodisperse colloidal spheres with a depletion agent which can have arbitrary shape and can possess a polydisperse size or shape distribution. In the low concentration limit, considered here, we…

Soft Condensed Matter · Physics 2009-11-11 C. Grodon , R. Roth

Large-scale Monte Carlo simulations of a phase-separating colloid-polymer mixture are performed and compared to recent experiments. The approach is based on effective interaction potentials in which the central monomers of self-avoiding…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , A. Jusufi , J. Dzubiella , C. N. Likos

Molecular dynamics simulations are used to examine the relationship between water-like anomalies and the liquid-liquid critical point in a family of model fluids with multi-Gaussian, core-softened pair interactions. The core-softened pair…

Soft Condensed Matter · Physics 2015-05-27 Evy Salcedo , Alan B. de Oliveira , Ney M. Barraz , Charusita Chakravarty , Marcia C. Barbosa

Two collective properties distinguishing the thin liquid water vapour interface from the bulk liquid are the anisotropy of the pressure tensor giving rise to surface tension and the orientational alignment of the molecules leading to a…

Soft Condensed Matter · Physics 2020-02-03 Chao Zhang , Michiel Sprik

We study the phase behavior of a symmetric binary polymer blend which is confined into a thin film. The film surfaces interact with the monomers via short range potentials. We calculate the phase behavior within the self-consistent field…

Statistical Mechanics · Physics 2009-10-31 M. Mueller , E. V. Albano , K. Binder

We theoretically investigate the nucleation of liquid droplets from vapor in the presence of a charged spherical particle. Due to field gradients, sufficiently close to the critical point of the vapor--gas system, the charge destabilizes…

Chemical Physics · Physics 2021-11-04 Roni Kroll , Yoav Tsori

The phase behavior of the Baxter adhesive hard sphere fluid has been determined using specialized Monte Carlo simulations. We give a detailed account of the techniques used and present data for the fluid-fluid coexistence curve as well as…

Soft Condensed Matter · Physics 2009-11-10 M. A. Miller , D. Frenkel

We investigate the behaviour of a binary surfactant solution (AOT/water) as it is progressively concentrated in microfluidic evaporators. We observe in time a succession of phase transitions from a dilute solution up to a dense state, which…

Soft Condensed Matter · Physics 2007-05-23 Jacques Leng , Mathieu Joanicot , Armand Ajdari

The one-dimensional triplet contact process with diffusion (TCPD) model has been studied using fast multispin GPU Monte Carlo simulations. In particular, the particle density \rho and the density of pairs of neighboring particles \rho_p…

Statistical Mechanics · Physics 2015-06-15 Raoul D. Schram , Gerard T. Barkema

The solid-solid coexistence of a polydisperse hard sphere system is studied by using the Monte Carlo simulation. The results show that for large enough polydispersity the solid-solid coexistence state is more stable than the single-phase…

Soft Condensed Matter · Physics 2009-11-13 Mingcheng Yang , Hongru Ma

When a fluid that undergoes a vapor to liquid transition in the bulk is confined to a long cylindrical pore, the phase transition is shifted (mostly due to surface effects at the walls of the pore) and rounded (due to finite size effects).…

Statistical Mechanics · Physics 2015-05-19 Alexander Winkler , Dorothea Wilms , Peter Virnau , Kurt Binder

In solution-processing of thin films, the material layer is deposited from a solution composed of several solutes and solvents. The final morphology and hence the properties of the film often depend on the time needed for the evaporation of…

A systematic investigation on vapor-liquid equilibria (VLE) of dipolar and quadrupolar fluids is carried out by molecular simulation to develop a new Helmholtz energy contribution for equations of state (EOS). Twelve two-center…

Chemical Physics · Physics 2009-04-30 Jadran Vrabec , J. Gross

A non-linear model associated with a Landau-Ginzburg-like behavior in mean field approximation forecasts phase transition waves and solitary kinks near the critical point. The behavior of isothermal waves is different of the one of…

Fluid Dynamics · Physics 2008-01-17 Henri Gouin

We compute the fourth virial coefficient of a binary nonadditive hard-sphere mixture over a wide range of deviations from diameter additivity and size ratios. Hinging on this knowledge, we build up a $y$ expansion [B. Barboy and W. N.…

Soft Condensed Matter · Physics 2011-10-25 G. Pellicane , F. Saija , C. Caccamo , P. V. Giaquinta

We present a Monte Carlo method to simulate asymmetric binary mixtures in the grand canonical ensemble. The method is used to study the colloid-polymer model of Asakura and Oosawa. We determine the phase diagram of the fluid-fluid unmixing…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , J. Horbach

We investigate the quantum phases of hard-core bosonic atoms in an extended Hubbard model where particles interact via soft-shoulder potentials in one dimension. Using a combination of field-theoretical methods and strong-coupling…

Quantum Gases · Physics 2015-07-08 M. Dalmonte , W. Lechner , Zi Cai , M. Mattioli , A. M. Läuchli , G. Pupillo

Vapor-liquid menisci of the truncated and shifted Lennard-Jones fluid between parallel planar walls are investigated by molecular dynamics simulation. Thereby, the characteristic energy of the unlike dispersive interaction between fluid…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Martin Horsch , Martina Heitzig , Calin Dan , Jens Harting , Hans Hasse , Jadran Vrabec

When a fluid with a bulk liquid-vapor critical point is placed inside a static external field with spatial periodic oscillations in one direction, the bulk critical point splits into two new critical points and a triple point. This…

Soft Condensed Matter · Physics 2015-05-27 Richard Vink , Tim Neuhaus , Hartmut Loewen

The phase behavior is investigated for systems composed of a large number of macromolecular components N, with N greater or equal to 2. Liquid-liquid phase separation is modelled using a virial expansion up to the second order of the…

Soft Condensed Matter · Physics 2024-05-29 Arjen Bot , Erik van der Linden , Paul Venema
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