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We study the elastic properties of a single A/B copolymer chain with a specific sequence. We predict a rich structure in the force extension relations which can be addressed to the sequence. The variational method is introduced to probe…

Soft Condensed Matter · Physics 2009-11-07 Namkyung Lee , Thomas A. Vilgis

We develop a first-principle equation of state of salt-free polyelectrolyte solution in the limit of infinitely long flexible polymer chains in the framework of a field-theoretical formalism beyond the linear Debye-Hueckel theory and…

Soft Condensed Matter · Physics 2015-08-04 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , E. A. Nogovitsyn , M. G. Kiselev

A new analysis of elastic properties of dense hard sphere (HS) fluids is presented, based on the expressions derived by Miller [J. Chem. Phys. {\bf 50}, 2733 (1969)]. Important consequences for HS fluids in terms of sound waves propagation,…

Materials Science · Physics 2019-10-02 Sergey Khrapak

Exact solutions for the elastic and thermodynamic properties for the wormlike chain model are elaborated in terms of Mathieu functions. The smearing of the classical Euler buckling instability for clamped polymers is analyzed for the…

Soft Condensed Matter · Physics 2017-05-10 Christina Kurzthaler , Thomas Franosch

The complex band structure of an isolated polyethylene chain is calculated within Density Functional Theory (DFT). A plane wave basis and ultrasoft pseudopotentials are used. The results are compared with those obtained via a local basis…

Materials Science · Physics 2009-11-10 Fabien Picaud , Alexander Smogunov , Andrea Dal Corso , Erio Tosatti

Crosslinked semi-flexible and flexible filaments that are actively deformed by molecular motors occur in various natural settings, such as the ordered eukaryotic flagellum, and the disordered cytoskeleton. The deformation of these composite…

Biological Physics · Physics 2018-10-02 Arvind Gopinath , Raghunath Chelakkot , L. Mahadevan

In the field of soft dielectric elastomers, the notion electrostriction indicates the dependency of the permittivity on strain. The present paper is aimed at investigating the effects of electrostriction onto the stability behaviour of…

Soft Condensed Matter · Physics 2013-10-02 M. Gei , S. Colonnelli , R. Springhetti

In this paper, we study the truncated two-particle correlation function in particle systems with long range interactions. For Coulombian and soft potentials, we define and give well-posedness results for the equilibrium correlations. In the…

Mathematical Physics · Physics 2018-09-28 Juan J. L. Velázquez , Raphael Winter

We consider the link between fragility and elasticity that follows from analysis of the data for a set of soft-colloid materials consisting of deformable spheres reported by Mattsson et. al., in Nature vol 462, 83 (2009). Fragility index…

Soft Condensed Matter · Physics 2021-04-08 Arijit Mondal , Leishangthem Premkumar , Shankar P. Das

The mechanical properties of a polymeric network containing both crosslinks and sliplinks (entanglements) are studied using a multi-chain Brownian dynamics simulation. We coarse-grain at the level of chain segments connecting consecutive…

Soft Condensed Matter · Physics 2007-05-23 Julian Oberdisse , Giovanni Ianniruberto , Francesco Greco , Guiseppe Marrucci

Compression-induced buckling instability of metal thin films on a compliant base result in surface wrinkles. A stiff thin film, perfectly bonded to an infinitely deep pre-stretched dielectric elastomer (DE) substrate, is considered. Linear…

Computational Physics · Physics 2021-08-24 Abhishek Ghosh

We study a minimal extension of the worm-like chain to describe polypeptides having alpha-helical secondary structure. In this model presence/absence of secondary structure enters as a scalar variable that controls the local chain bending…

Statistical Mechanics · Physics 2009-11-10 Buddhapriya Chakrabarti , Alex J. Levine

Active control of wrinkling in soft film-substrate composites using electric fields is a critical challenge in tunable material systems. Here, we investigate the electro-mechanical instability of a soft dielectric film bonded to a…

Soft Condensed Matter · Physics 2026-04-14 Bin Wu , Linghao Kong , Weiqiu Chen , Davide Riccobelli , Michel Destrade

Biopolymer Networks play an important role in coordinating and regulating collective cellular dynamics via a number of signaling pathways. Here, we investigate the mechanical response of a model biopolymer network due to the active…

Soft Condensed Matter · Physics 2016-11-23 Long Liang , Christopher Jones , Bo Sun , Yang Jiao

We perform extensive molecular dynamics simulations of a charged polymer in a good solvent in the regime where the chain is collapsed. We analyze the dependence of the gyration radius $R_g $ on the reduced Bjerrum length $\ell_B$ and find…

Soft Condensed Matter · Physics 2016-10-05 Anvy Moly Tom , Satyavani Vemparala , R. Rajesh , Nikolai V. Brilliantov

A new formalism is used for a Monte Carlo determination of the elastic constants of a two-dimensional net of fixed connectivity. The net is composed of point-like atoms each of which is tethered to six neighbors by a bond limiting the…

Statistical Mechanics · Physics 2009-10-31 Oded Farago , Yacov Kantor

The behavior of a polyelectrolyte adsorbed on a charged surface of high-dielectric constant is studied by both Monte-Carlo simulation and analytical methods. It is found that in a low ionic strength medium, the transition is first-order…

Soft Condensed Matter · Physics 2007-05-23 Chi-Ho Cheng , Pik-Yin Lai

The equilibrium amorphous solid state -- formed, e.g., by adequately randomly crosslinking the constituents of a macromolecular fluid -- is a heterogeneous state characterized by a universal distribution of particle localization lengths.…

Soft Condensed Matter · Physics 2023-01-04 Boli Zhou , Rafael Hipolito , Paul M. Goldbart

We study the friction between a flat solid surface where polymer chains have been end-grafted and a cross-linked elastomer at low sliding velocity. The contribution of isolated grafted chains' penetration in the sliding elastomer has been…

Soft Condensed Matter · Physics 2015-06-24 Thomas Vilmin , Elie Raphael

The cytoskeleton of eukaryotic cells provides mechanical support and governs intracellular transport. These functions rely on the complex mechanical properties of networks of semiflexible protein filaments. Recent theoretical interest has…

Soft Condensed Matter · Physics 2012-11-01 M. Atakhorrami , G. H. Koenderink , J. F. Palierne , F. C. MacKintosh , C. F. Schmidt