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By means of density functional theory, we investigate the magnetic ground state of edge-sharing CuO_2 spin-chains, as found in the (La,Ca,Sr)_14Cu_24O_41system, for instance. Our data rely on spin-polarized electronic structure calculations…

Strongly Correlated Electrons · Physics 2009-11-13 U. Schwingenschloegl , C. Schuster

Recently the superconductivity has been reported in the copper oxides (Sr,Ca)$_{14}$Cu$_{24}$O$_{41}$ with ladders and edge-sharing chains under pressure. In order to understand the mechanism of the superconductivity, it is crucial to…

Strongly Correlated Electrons · Physics 2009-10-31 Yoshiaki Mizuno , Takami Tohyama , Sadamichi Maekawa

The flurry of theoretical and experimental studies following the report of room-temperature superconductivity at ambient pressure in Cu-substituted lead apatite Cu$_x$Pb$_{10-x}$(PO$_4$)$_6$O (`LK99') have explored whether and how this…

Strongly Correlated Electrons · Physics 2024-01-11 Katherine Inzani , John Vinson , Sinéad M. Griffin

The locally self-consistent real space multiple scattering technique has been applied to calculate the electronic structure and chemical binding for the c(2x2)O/Cu(001) system, as a function of $d_{O-Cu1}$ -- the height of oxygen above the…

Materials Science · Physics 2009-11-07 Sergey Stolbov , Abdelkader Kara , Talat S. Rahman

The temperature dependence of the optical and magnetic properties of CuO were examined by means of hybrid density functional theory calculations. Our work shows that the spin exchange interactions in CuO are neither fully one-dimensional…

Materials Science · Physics 2015-05-13 X. Rocquefelte , M. -H. Whangbo , A. Villesuzanne , S. Jobic , F. Tran , K. Schwarz , P. Blaha

We perform first principles, multiconfiguration calculations on clusters including several CuO$_6$ octahedra and study the ground-state electron distribution and electron--lattice couplings when holes are added to the undoped $d^9 p^6$…

Strongly Correlated Electrons · Physics 2009-11-11 L. Hozoi , S. Nishimoto , A. Yamasaki

Based on density functional calculations, we present a detailed theoretical study of the electronic structure and the magnetic properties of the quasi-one dimensional chain cuprate Li_2ZrCuO_4 (Li_2CuZrO_4). For the relevant ratio of the…

Strongly Correlated Electrons · Physics 2015-05-14 M. Schmitt , J. Malek , S. -L. Drechsler , H. Rosner

Single-crystal neutron diffraction has been used to determine the incommensurate magnetic structure of NaCu2O2, a compound built up of chains of edge-sharing CuO4 plaquettes. Magnetic structures compatible with the lattice symmetry were…

Strongly Correlated Electrons · Physics 2015-05-18 L. Capogna , M. Reehuis , A. Maljuk , R. K. Kremer , B. Ouladdiaf , M. Jansen , B. Keimer

The magnetic structure of the edge sharing cuprate compound Li2CuO2 has been investigated by means of ab initio electronic structure calculations. The first and second neighbor in-chain magnetic interactions are calculated to be -142 K and…

Materials Science · Physics 2007-05-23 Coen de Graaf , Iberio de P. R. Moreira , Francesc Illas , Oscar Iglesias , Amilcar Labarta

We investigated the paramagnetic resonance in single crystals of LiCuVO$_4$ with special attention to the angular variation of the absorption spectrum. To explain the large resonance linewidth of the order of 1 kOe, we analyzed the…

Strongly Correlated Electrons · Physics 2009-11-07 H. -A. Krug von Nidda , L. E. Svistov , M. V. Eremin , R. M. Eremina , A. Loidl , V. Kataev , A. Validov , A. Prokofiev , W. Assmus

CoSe$_2$O$_5$ has a crystal structure consisting of zig-zag chains of edge shared CoO$_6$ octahedra running along the c axis, with the chains separated by Se$_2$O$_5^{2-}$ units. Magnetic susceptibility measurements indicate a transition at…

Materials Science · Physics 2012-02-02 Brent C. Melot , Brian Paden , Ram Seshadri , Ambesh Dixit , Gavin Lawes , Emmanuelle Suard

We study a Heisenberg chain with nearest-neighbor (NN) J1 and next-NN J2 exchange interactions with anisotropies Delta_1 and Delta_2 respectively. We investigate by analytical and numerical methods the region of parameters for which there…

Strongly Correlated Electrons · Physics 2007-05-23 A. A. Aligia

We present a joint experimental and theoretical study of the electronic structure of the cuprate chain systems A_(1-x)CuO_2 (A=Ca,Sr,Ba), as measured using O-K and Cu-L_3 x-ray absorption spectroscopy. The doping-dependent behaviour in…

Strongly Correlated Electrons · Physics 2009-09-25 Z. Hu , S. -L. Drechsler , J. Malek , H. Rosner , R. Neudert , M. Knupfer , M. S. Golden , J. Fink , J. Karpinski , G. Kaindl , C. Hellwig , Ch. Jung

The electronic structure of the $(2\sqrt{2}\times\sqrt{2})R45^{\circ}$ O/Cu(001) system has been calculated using locally self-consistent, real space multiple scattering technique based on first principles. Oxygen atoms are found to perturb…

Materials Science · Physics 2009-11-07 S. Stolbov , T. S. Rahman

The title quasi-1D copper oxides (0=< x =<0.4) were investigated by neutron diffraction and magnetic susceptibility studies. Polyhedral CuO4 units in the compounds were found to comprise linear-chains at inter-chain distance of…

Superconductivity · Physics 2009-11-07 K. Yamaura , Q. Huang , E. Takayama-Muromachi

The optical conductivity sigma(omega) is calculated at finite temperature T for CuO_2 chain clusters within a pd-Hubbard model. Data at T = 300 K for Li_2CuO_2 are reanalyzed within this approach. The relative weights of Zhang-Rice singlet…

Strongly Correlated Electrons · Physics 2009-11-13 J. Malek , S. -L. Drechsler , U. Nitzsche , H. Rosner , H. Eschrig

We report an experimental study of \nco, a Mott insulator containing chains of edge-sharing CuO$_4$ plaquettes, by polarized x-ray absorption spectroscopy (XAS), resonant magnetic x-ray scattering (RMXS), magnetic susceptibility, and…

Strongly Correlated Electrons · Physics 2010-12-07 Ph. Leininger , M. Rahlenbeck , M. Raichle , B. Bohnenbuck , E. Weschke , E. Schierle , A. Maljuk , C. T. Lin , S. Seki , Y. Tokura , J. W. Freeland , B. Keimer

A quantum-mechanical model of Cu-O-Cu-O four-center four-electron part of the copper-oxide plane embedded in a superconducting crystal La$_{2-x}$Sr$% _{x}$CuO$_{4}$ (LSCO) is considered. It is shown that displacing the nearest-neighbor…

Superconductivity · Physics 2020-02-12 Krzysztof A. Meissner , Lucjan Piela

In a recent work devoted to the magnetism of Li$_{2}$CuO$_{2}$, Shu et al. [New J. Phys. 19 (2017) 023026] have proposed a "simplified" unfrustrated microscopic model that differs considerably from the models refined through decades of…

First-principles calculations with the full-potential linearized augmented plane-wave (FP-LAPW) method have been performed to investigate detailed electronic and linear optical properties of Sr$_{2}$CuO$_{2}$Cl$_{2}$, which is a classical…

Strongly Correlated Electrons · Physics 2009-11-11 Hongming Weng , Xiangang Wan , Jian Zhou , Jinming Dong
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