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A key open question in the glass transition field is whether a finite temperature thermodynamic transition to the glass state exists or not. Recent simulations of coupled replicas in atomistic models have found signatures of a static…

Statistical Mechanics · Physics 2015-06-18 Juan P. Garrahan

The aging behavior of polymer glass, poly(methyl methacrylate), has been investigated through the measurement of ac dielectric susceptibility ata fixed frequency after a temperature shift $\Delta T$ ($\le $ 20 K)between two temperatures,…

Soft Condensed Matter · Physics 2009-11-13 Koji Fukao , Sinpei Yamawaki

An infinite hierarchy of layering transitions exists for model polymers in solution under poor solvent or low temperatures and near an attractive surface. A flat histogram stochastic growth algorithm known as FlatPERM has been used on a…

Statistical Mechanics · Physics 2009-11-10 J. Krawczyk , A. L. Owczarek , T. Prellberg , A. Rechnitzer

We study an air-fluidized granular monolayer, composed of plastic spheres which roll on a metallic grid. The air current is adjusted so that the spheres never loose contact with the grid, so that the dynamics may be regarded as pseudo…

Soft Condensed Matter · Physics 2022-11-21 F. Vega Reyes , A. Rodríguez-Rivas , J. F. González-Saavedra , M. A. López-Castaño

Whether the glass transition is caused by an underlying singularity or is a purely kinetic phenomenon is a significant outstanding question. Studying an atomistic glass former, we introduce a sampling method to access temperatures…

Statistical Mechanics · Physics 2017-09-20 Thomas Speck , C. Patrick Royall , Stephen R. Williams

We study by Molecular Dynamics simulation a dense one-component system of particles confined on a spherical substrate. We more specifically investigate the evolution of the structural and dynamical properties of the system when changing the…

Soft Condensed Matter · Physics 2018-05-23 Julien-Piera Vest , Gilles Tarjus , Pascal Viot

Glass-to-glass and liquid-to-liquid phase transitions are observed in bulk and confined water, with or without applied pressure. They result from the competition of two liquid phases separated by an enthalpy difference depending on…

Disordered Systems and Neural Networks · Physics 2017-11-21 Robert F. Tournier

We study the viscoelastic response of amorphous polymers using theory and simulations. By accounting for internal stresses and considering instantaneous normal modes (INMs) within athermal non-affine theory, we make parameter-free…

Conformational phases of a semiflexible off-lattice homopolymer model near an attractive substrate are investigated by means of multicanonical computer simulations. In our polymer-substrate model, nonbonded pairs of monomers as well as…

Computational Physics · Physics 2009-07-20 Monika Möddel , Michael Bachmann , Wolfhard Janke

Thermal conductivity of a model glass-forming system in the liquid and glass states is studied using extensive numerical simulations. We show that near the glass transition temperture, where the structural relaxation time becomes very long,…

Disordered Systems and Neural Networks · Physics 2020-02-26 Pranab Jyoti Bhuyan , Rituparno Mandal , Pinaki Chaudhuri , Abhishek Dhar , Chandan Dasgupta

Molecular dynamics simulations are used to investigate the connection between thermal history and physical aging in polymer glasses, in particular the effects of a temperature square step. Measurements of two-time correlation functions show…

Soft Condensed Matter · Physics 2009-11-13 Mya Warren , Joerg Rottler

The dramatic dynamic slowing down associated with the glass transition is considered by many to be related to the existence of a static length scale that grows when temperature decreases. Defining, identifying and measuring such a length is…

Statistical Mechanics · Physics 2014-05-29 Giulio Biroli , Smarajit Karmakar , Itamar Procaccia

Via large-scale molecular dynamics simulations, we observe the melting of a topological glass of stiff ring polymers by incorporating flexible ring polymers, along an isobaric path. As more flexible ring polymers are introduced, cluster…

Soft Condensed Matter · Physics 2023-05-19 Projesh Kumar Roy , Pinaki Chaudhuri , Satyavani Vemparala

The glass transition is described in terms of thermally activated local structural rearrangements, the secondary relaxations of the glass phase. The interaction between these secondary relaxations leads to a much faster and much more…

Disordered Systems and Neural Networks · Physics 2007-05-23 U. Buchenau

The dynamical behavior of a kind of models with hierarchically constrained dynamics is investigated. The models exhibit many properties resembling real structural glasses. In particular, we focus on the study of time-dependent temperature…

Statistical Mechanics · Physics 2009-11-07 A. Prados , J. J. Brey

We analyze a (1+1)-dimension directed random walk model of a polymer dipped in a medium constituted by two immiscible solvents separated by a flat interface. The polymer chain is heterogeneous in the sense that a single monomer may…

Probability · Mathematics 2007-05-23 Erwin Bolthausen , Giambattista Giacomin

We study the glass transition by exploring a broad class of kinetic rules that can significantly modify the normal dynamics of super-cooled liquids, while maintaining thermal equilibrium. Beyond the usual dynamics of liquids, this class…

Soft Condensed Matter · Physics 2024-06-14 Cristina Gavazzoni , Carolina Brito , Matthieu Wyart

The short- and long-time dynamics of model systems undergoing a glass transition with apparent inversion of Kauzmann and dynamical arrest glass transition lines is investigated. These models belong to the class of the spherical mean-field…

Disordered Systems and Neural Networks · Physics 2016-01-06 Corrado Rainone , Ulisse Ferrari , Matteo Paoluzzi , Luca Leuzzi

An asymmetric generalization of the zero-temperature Glauber model on a lattice is introduced. The dynamics of the particle-density and specially the large-time behavior of the system is studied. It is shown that the system exhibits two…

Statistical Mechanics · Physics 2009-10-31 Mohammad Khorrami , Amir Aghamohammadi

We investigate glassy dynamical properties of one component three-dimensional system of particles interacting via pair repulsive potential by the molecular dynamic simulation in the wide region of densities. The glass state is superfragile…

Soft Condensed Matter · Physics 2013-01-11 R. E. Ryltsev , N. M. Chtchelkatchev , V. N. Ryzhov