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BaCuSi$_2$O$_6$, a $S=1/2$ quantum antiferromagnet with a double-layer structure of Cu$^{2+}$ ions in a distorted planar-rectangular coordination and with a dimerized spin singlet ground state, is studied by means of the electron…

Other Condensed Matter · Physics 2019-09-20 S. A. Zvyagin , J. Wosnitza , J. Krzystek , R. Stern , M. Jaime , Y. Sasago , K. Uchinokura

We use neutron spectroscopy to determine the nature of the magnetic excitations in superconducting BaFe$_{1.9}$Ni$_{0.1}$As$_{2}$ ($T_{c}=20$ K). Above $T_{c}$ the excitations are gapless and centered at the commensurate antiferromagnetic…

We report detailed inelastic neutron scattering measurements on single crystals of the frustrated two-leg ladder BiCu2PO6, whose ground state is described as a spin liquid phase with no long-range order down to 6 K. Two branches of steeply…

Strongly Correlated Electrons · Physics 2013-08-09 K. W. Plumb , Zahra Yamani , M. Matsuda , G. J. Shu , B. Koteswararao , F. C. Chou , Young-June Kim

Building on recent neutron and NMR experiments, we investigate the field-induced exotic criticality observed in the frustrated spin-1/2 dimer compound BaCuSi2O6 using a frustrated model with two types of bilayers. A semiclassical treatment…

Strongly Correlated Electrons · Physics 2009-02-16 Nicolas Laflorencie , Frederic Mila

We performed inelastic neutron scattering experiments on Cu$_2$$^{114}$Cd$^{11}$B$_2$O$_6$ powder. The magnetic excitations at low temperatures are similar to those of the interacting spin-1/2 tetramers in the ordered state. The weak…

Strongly Correlated Electrons · Physics 2015-12-09 Masashi Hase , Kenji Nakajima , Seiko Ohira-Kawamura , Yukinobu Kawakita , Tatsuya Kikuchi , Masashige Matsumoto

The geometrically frustrated double perovskite Ba2YMoO6 is characterized by quantum s=1/2 spins at the Mo5+ sites of an undistorted face-centered cubic (FCC) lattice. Previous low-temperature characterization revealed an absence of static…

Magnetic excitations of the effective spin $S$=1/2 dimerized magnet Ba$_2$CoSi$_2$O$_6$Cl$_2$ have been probed directly via inelastic neutron scattering experiments at temperatures down to 4 K. We observed five types of excitation at 4.8,…

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

Unlike most quantum systems which rapidly become incoherent as temperature is raised, strong correlations persist at elevated temperatures in $S=1/2$ dimer magnets, as revealed by the unusual asymmetric lineshape of their excitations at…

Strongly Correlated Electrons · Physics 2016-07-20 E. S. Klyushina , A. C. Tiegel , B. Fauseweh , A. T. M. N. Islam , J. T. Park , B. Klemke , A. Honecker , G. S. Uhrig , S. R. Manmana , B. Lake

The compound BaCuSi2O6 is a quantum magnet with antiferromagnetic dimers of S = 1/2 moments on a quasi-2D square lattice. We have investigated its spin dynamics by inelastic neutron scattering experiments on single crystals with an energy…

Strongly Correlated Electrons · Physics 2008-04-24 Ch. Rüegg , D. F. McMorrow , B. Normand , H. M. Ronnow , S. E. Sebastian , I. R. Fisher , C. D. Batista , S. Gvasaliya , Ch. Niedermayer , J. Stahn

We present results of magnetisation and electron paramagnetic resonance experiments on the spin-dimer system BaCuSi2O6. Evidence indicates that the origin of anisotropic terms in the spin Hamiltonian is from magnetic dipolar interactions.…

We present a numerical study of the spin-1/2 bilayer Heisenberg antiferromagnet with random interlayer dimer dilution. From the temperature dependence of the uniform susceptibility and a scaling analysis of the spin correlation length we…

Disordered Systems and Neural Networks · Physics 2009-11-07 O. P. Vajk , M. Greven

Thermodynamic properties and elementary excitations in $S=1/2$ one-dimensional Heisenberg antiferromagnet KCuGaF$_6$ were investigated by magnetic susceptibility, specific heat and ESR measurements. Due to the Dzyaloshinsky-Moriya…

Strongly Correlated Electrons · Physics 2009-11-13 Rieko Morisaki , Toshio Ono , Hidekazu Tanaka , Hiroyuki Nojiri

We report on terahertz spectroscopic measurements of quantum spin dynamics on single crystals of a spin-1/2 frustrated spin-ladder antiferromagnet BiCu$_2$PO$_6$ as a function of temperature, polarization, and applied external magnetic…

We investigate the zero-temperature and the finite-temperature properties of the two-dimensional antiferromagnetic quantum spin system composed of the s=1/2 and s=1 spins. The spin excitation spectrum as well as the thermodynamic quantities…

Strongly Correlated Electrons · Physics 2009-10-31 Y. Takushima , A. Koga , N. Kawakami

The magnetic properties of NiTa$_2$O$_6$ were investigated by magnetic susceptibility, specific heat, electron paramagnetic resonance, neutron powder diffraction and pulse field magnetization measurements. Accompanying \textit{ab initio}…

Strongly Correlated Electrons · Physics 2015-06-18 J. M. Law , H. -J. Koo , M. -H. Whangbo , E. Bruecher , V. Pomjakushin , R. K. Kremer

Magnetic excitations in a weakly coupled spin dimers and chains compound Cu2Fe2Ge4O13 are measured by inelastic neutron scattering. Both structure factors and dispersion of low energy excitations up to 10 meV energy transfer are well…

Strongly Correlated Electrons · Physics 2009-11-11 T. Masuda , A. Zheludev , B. Sales , S. Imai , K. Uchinokura , S. Park

We report the magnetic excitation spectrum as measured by inelastic neutron scattering for a polycrystalline sample of Sr$_3$CuPtO$_6$. Modeling the data by the 2+4 spinon contributions to the dynamical susceptibility within the chains, and…

We report magnetization and heat capacity measurements of single crystal samples of the spin gap compound Sr$_2$Cu(BO$_3$)$_2$. Low-field data show that the material has a singlet ground state comprising dimers with intradimer coupling J =…

Strongly Correlated Electrons · Physics 2011-12-08 Suchitra E. Sebastian , D. Yin , P. Tanedo , G. A. Jorge , N. Harrison , M. Jaime , Y. Mozharivskyj , G. Miller , J. Krzystek , S. A. Zvyagin , I. R. Fisher

We present an inelastic neutron scattering (INS) study of the excitation spectrum of a model S = 1/2 equilateral Heisenberg trimer, Cu_3(O_2C_16H_23)_6.1.2C_6H_12. Earlier measurements were interpreted on the basis of a spin ground state…

Strongly Correlated Electrons · Physics 2007-05-23 M. B. Stone , F. Fernandez-Alonso , D. T. Adroja , N. S. Dalal , D. Villagran , F. A. Cotton , S. E. Nagler
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