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We analyze a model problem representing a multi-electronic molecule sitting on a metal surface. Working with a reduced configuration interaction Hamiltonian, we show that one can extract very accurate ground state wavefunctions as compared…

Chemical Physics · Physics 2020-09-24 Junhan Chen , Zuxin Jin , Wenjie Dou , Joseph Subotnik

We study the electronic and magnetic structure of carbon and nitrogen impurities and interstitials in rutile TiO${_2}$. To this end we perform \textit{ab-initio} calculations of a 48-atom supercell employing the VASP code. In order to…

Materials Science · Physics 2015-01-22 Jacqueline Atanelov , Christoph Gruber , Peter Mohn

We present the results of self-consistent calculations of the electronic shell and supershell structure for clusters having up to 6000 valence electrons. The ionic background is described in terms of a homogeneous jellium. The calculations…

Condensed Matter · Physics 2009-10-28 Erik Koch , Olle Gunnarsson

Phosphorene, a single atomic layer of black phosphorus, has recently emerged as a new twodimensional (2D) material that holds promise for electronic and photonic technology. Here we experimentally demonstrate that the electronic structure…

The electronic structure of the poly-pyridine conjugated polymer has been investigated by resonant and nonresonant inelastic X-ray scattering and X-ray absorption spectroscopies using synchrotron radiation. The measurements were made for…

We study numerically self-trapped (polaron) states of quasiparticles (electrons, holes or excitons) in a deformable nanotube formed by a hexagonal lattice, wrapped into a cylinder (carbon- and boron nitride-type nanotube structures). We…

Other Condensed Matter · Physics 2007-05-23 L. Bratek , L. Brizhik , A. Eremko , B. Piette , M. Watson , W. Zakrzewski

We investigate the mechanical properties of $\pi$-conjugated polymeric materials composed of regioregular poly(3-hexylthiophene) (P3HT) and fullerene C$_{60}$ using coarse-grained molecular dynamics simulations. Specifically, we perform…

Materials Science · Physics 2021-01-11 Yuta Yoshimoto , Sou Sugiyama , Shuntaro Shimada , Toshihiro Kaneko , Shu Takagi , Ikuya Kinefuchi

Considering C$_{60}$ as a model system for describing field emission from the extremity of a carbon nanotip, we explore electron emission from this fullerene excited by an intense, near-infrared, few-cycle laser pulse…

Atomic and Molecular Clusters · Physics 2016-03-23 Cong-Zhang Gao , Phuong Mai Dinh , Peter Kluepfel , Chris Meier , Paul-Gerhard Reinhard , Eric Suraud

Materials with optimized band gap are needed in many specialized applications. In this work, we demonstrate that Hellmann-Feynman forces associated with the gap states can be used to find atomic coordinates with a desired electronic density…

Materials Science · Physics 2015-06-16 Kiran Prasai , Parthapratim Biswas , D. A. Drabold

Investigations of clathrate structures have gained a new impetus with the recent discovery of room-temperature superconductivity in metal hydrides. Here we report the finding, through density functional theory calculations, of a clathrate…

Materials Science · Physics 2021-08-02 Jorge Laranjeira , Leonel Marques , Manuel Melle-Franco , Karol Strutynski , Manuel Barroso

Recent experiments have shown that C60 can be positively field-doped. In that state, fullerene exhibits a higher resistivity and a higher superconducting temperature than the corresponding negatively doped state. A strong intramolecular…

Superconductivity · Physics 2009-11-07 Nicola Manini , Andrea Dal Corso , Michele Fabrizio , Erio Tosatti

We investigate the electronic structure of Ca1-xSrxVO3 using careful state-of-the-art experiments and calculations. Photoemission spectra using synchrotron radiation reveal a hitherto unnoticed polarization dependence of the photoemission…

Strongly Correlated Electrons · Physics 2016-08-31 Kalobaran Maiti , U. Manju , Sugata Ray , Priya Mahadevan , I. H. Inoue , C. Carbone , D. D. Sarma

The properties of hydrogen at warm dense matter (WDM) conditions are of high importance for the understanding of astrophysical objects and technological applications such as inertial confinement fusion. In this work, we present extensive…

Plasma Physics · Physics 2023-06-12 Tobias Dornheim , Maximilian Böhme , Zhandos Moldabekov , Jan Vorberger

We discuss physical properties of strongly correlated electron states for a linear chain obtained with the help of the recently proposed new method combining the exact diagonalization in the Fock space with an ab initio readjustment of the…

Strongly Correlated Electrons · Physics 2007-05-23 Adam Rycerz , Jozef Spalek

The electronic structure and structural evolution of hydrogenated graphene are investigated by Raman spectroscopy with multiple excitations. The excitation energy dependent saturation effect on the ratio of integrated intensities of D and G…

Materials Science · Physics 2010-12-06 Zhiqiang Luo , Ting Yu , Zhenhua Ni , Sanhua Lim , Jingzhi Shang , Hailong Hu , Lei Liu , Zexiang Shen , Jianyi Lin

We review the electronic properties of bilayer graphene, beginning with a description of the tight-binding model of bilayer graphene and the derivation of the effective Hamiltonian describing massive chiral quasiparticles in two parabolic…

Mesoscale and Nanoscale Physics · Physics 2013-04-23 Edward McCann , Mikito Koshino

We investigate the stability of boron fullerene sets B76, B78 and B82. We evaluate the ground state energies, nucleus-independent chemical shift (NICS), the binding energies per atom and the band gap values by means of first-principles…

Materials Science · Physics 2017-09-13 Serkan Polad , Mete Ozay

We investigate the formation of fullerene-like structures from hot Carbon gas using classical molecular dynamics, employing Brenner's potential. In particular we examine the influence of different annealing strategies on fullerene yield,…

Materials Science · Physics 2009-12-22 Klaus Lichtenegger , Wolfgang von der Linden

Shell structure in the single particle spectrum of deformed harmonic oscillator potentials when a term proportional to $(\vec L)^2$ is added is analyzed for a large particle number. A scaling law which gives a dividing line between regular…

Condensed Matter · Physics 2009-10-30 W. D. Heiss , R. G. Nazmitdinov

Over many years, computational simulations based on Density Functional Theory (DFT) have been used extensively to study many different materials at the atomic scale. However, its application is restricted by system size, leaving a number of…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Carlos Romero-Muñiz , Ayako Nakata , Pablo Pou , David R. Bowler , Tsuyoshi Miyazaki , Rubén Pérez