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Related papers: Self-interaction correction in the LDA+U method

200 papers

Methods based on the combination of the usual density functional theory (DFT) codes with the Hubbard models are widely used to investigate the properties of strongly correlated materials. Using first-principle calculations we study the…

Materials Science · Physics 2015-08-04 Christos Tsirogiannis , Iosif Galanakis

We provide a straightforward and efficient procedure to combine LDA+U total energy functional with the full potential linearized augmented plane wave method. A detailed derivation of the LDA+U Kohn-Sham type equations is presented for the…

Strongly Correlated Electrons · Physics 2009-10-31 A. B. Shick , A. I. Liechtenstein , W. E. Pickett

Combining the density functional theory (DFT) and the Gutzwiller variational approach, a LDA+Gutzwiller method is developed to treat the correlated electron systems from {\it ab-initio}. All variational parameters are self-consistently…

Strongly Correlated Electrons · Physics 2009-11-13 XiaoYu Deng , Xi Dai , Zhong Fang

First-principles calculations within the Local Density Approximation (LDA) or Generalized Gradient Approximation (GGA), though very successful, are known to underestimate redox potentials, such as those at which lithium intercalates in…

Materials Science · Physics 2009-11-10 Fei Zhou , Matteo Cococcioni , Chris A. Marianetti , Dane Morgan , G. Ceder

In effective single-electron theories, self-interaction manifests itself through the unphysical dependence of the energy of an electronic state as a function of its occupation, which results in important deviations from the ideal Koopmans…

Materials Science · Physics 2009-01-20 I. Dabo , M. Cococcioni , N. Marzari

To accurately describe the energetics of transition metal systems, density functional approximations (DFAs) must provide a balanced description of s- and d- electrons. One measure of this is the sd transfer error, which has previously been…

Chemical Physics · Physics 2025-01-13 Rohan Maniar , Priyanka B. Shukla , J. Karl Johnson , Koblar A. Jackson , John P. Perdew

A general reformulation of the exchange energy of $5f$-shell is applied in the analysis of the magnetic structure of various actinides compounds in the framework of LDA+U method. The calculations are performed in an efficient scheme with…

Strongly Correlated Electrons · Physics 2016-08-14 Fredrik Bultmark , Francesco Cricchio , Oscar Grånäs , Lars Nordström

DFT+U provides a convenient, cost-effective correction for the self-interaction error (SIE) that arises when describing correlated electronic states using conventional approximate density functional theory (DFT). The success of a DFT+U(+J)…

Calculations of various corrections to the g factor of Li-like ions are presented, which result in a significant improvement of the theoretical accuracy in the region Z = 6-92. The configuration-interaction Dirac-Fock method is employed for…

Atomic Physics · Physics 2007-05-23 D. A. Glazov , V. M. Shabaev , I. I. Tupitsyn , A. V. Volotka , V. A. Yerokhin , G. Plunien , G. Soff

The LDA-1/2 method for self-energy correction is a powerful tool for calculating accurate band structures of semiconductors, while keeping the computational load as low as standard LDA. Nevertheless, controversies remain regarding the…

Computational Physics · Physics 2024-09-17 Kan-Hao Xue , Jun-Hui Yuan , Leonardo R. C. Fonseca , Xiang-Shui Miao

A recently proposed extension of the interaction flow method is applied to exemplary cases of selected physical and methodical parameters for the two-dimensional Hubbard model away from half-filling and perfect nesting. In this scheme, the…

Strongly Correlated Electrons · Physics 2022-02-15 Daniel Rohe

We describe the behavior of the Perdew-Zunger self-interaction-corrected local density approximation (SIC-LDA) functional when implemented in a plane-wave pseudopotential formalism with Wannier functions. Prototypical semiconductors and…

Other Condensed Matter · Physics 2011-03-03 Massimiliano Stengel , Nicola A. Spaldin

Dynamical correlations and non-local contributions beyond static mean-field theories are of fundamental importance for describing the electronic structure of correlated metals. Their effects are usually described with many-body approaches…

Strongly Correlated Electrons · Physics 2023-09-22 Marco Vanzini , Nicola Marzari

The Gutzwiller technique has long been known as a method to include correlations in electronic structure calculations. Here we implement an ab-initio Gutzwiller+LDA calculation, and apply it to a classic problem, the ferromagnetism of bulk…

Strongly Correlated Electrons · Physics 2013-07-23 Giovanni Borghi , Michele Fabrizio , Erio Tosatti

In this article we introduce a generalization of the popular DFT+U method based on the extended Hubbard model that includes on-site and inter-site electronic interactions. The novel corrective Hamiltonian is designed to study systems for…

Strongly Correlated Electrons · Physics 2015-05-13 Vivaldo Leiria Campo , Matteo Cococcioni

Effects of electron correlation on the electronic structure and magnetic properties of the Gd(0001) surface are investigated using of the full-potential linearized augmented plane wave implementation of correlated band theory ("LDA+U"). The…

Strongly Correlated Electrons · Physics 2009-10-31 A. B. Shick , W. E. Pickett , C. S. Fadley

We unify the Perdew-Zunger self-interaction correction (PZSIC) to approximate density functional theory (DFT), the Hubbard correction DFT+U, and Rung 3.5 functionals within the Adiabatic Projection formalism. We modify the Kohn-Sham…

Chemical Physics · Physics 2023-05-16 Benjamin G. Janesko

We present an accurate implementation of total energy calculations into the local density approximation plus dynamical mean-field theory (LDA+DMFT) method. The electronic structure problem is solved through the full potential linear…

Strongly Correlated Electrons · Physics 2009-03-16 I. Di Marco , J. Minár , S. Chadov , M. I. Katsnelson , H. Ebert , A. I. Lichtenstein

The most widely-used density functionals for the exchange-correlation energy are inexact for one-electron systems. Their self-interaction errors can be severe in some applications. The problem is not only to correct the self-interaction…

Chemical Physics · Physics 2009-11-10 Stephan Kümmel , John P. Perdew

In this paper we have investigated the electronic properties of Fe(OH)2 hydroxide by using the LSDA+U as well as the generalized gradient approximation. Our calculations for the iron-hydroxide show that the LSDA results are greatly at…

Materials Science · Physics 2013-05-29 Mansoureh Pashangpour , Khadijeh Imani , Amir Abbas Sabouri-Dodaran , Nasser Nafari