Related papers: Optical second harmonic generation from Wannier ex…
Light generation through optical harmonics plays a pivotal role in photonics, driving innovations in coherent light sources, biological imaging, and spectroscopy. Traditional methods for tuning optical harmonics, including electrostatic…
We develop a theory of the nonlinear optical responses in superconducting systems in the presence of a dc supercurrent. The optical transitions between particle-hole pair bands across the superconducting gap are allowed in clean…
To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…
We present a microscopic quantum theory of light-matter interaction in pristine sheets of two-dimensional semiconductors coupled to localized electromagnetic resonators such as optical nanocavities or plasmonic particles. The light-matter…
Monolayer C$_3$N is an emerging two-dimensional indirect band gap semiconductor with interesting mechanical, thermal, and electronic properties. In this work we present a description of C$_3$N electronic and dielectric properties, focusing…
We theoretically investigate second harmonic generation that originates from the nonlinear, magnetic Lorentz force term from single and multiple apertures carved on thick, opaque metal substrates. The linear transmission properties of…
Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…
Excitons and their complexes govern optical-related behaviors in semiconductors. Here, using angle-resolved photoemission spectroscopy (ARPES), we have elucidated the light-matter interaction mediated by quasi-steady excitonic complexes…
We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…
We measure the second-harmonic (SH) response of MoS$_2$ in a broad fundamental photon energy range between 0.85 and 1.7 eV, and present a continuous SH spectrum capturing signatures of both the fundamental A and B excitons in addition to…
The energy band structure of excitons is studied in periodic potentials produced by the short-range interaction between the exciton and electrons of Wigner or Moir\'{e} lattices. Treating the exciton as a point-like dipole that interacts…
Second harmonic generation by spherical nanoparticles is a non-local optical process that can also be viewed as the result of the non-linear response of the thin interface layer. The classical electrodynamic description, based e.g. on the…
This paper concerns the scattering problem for a nonlinear medium of compact support, $D$, with second-harmonic generation. Such a medium, when probed with monochromatic light beams at frequency $\omega$, generates additional waves at…
We theoretically investigate harmonic generation in graphene quantum dots under linearly polarized optical pulses, focusing on excitonic effects. Combining the tight-binding model and the single-particle density matrix approach, we derive a…
The photophysics of $\pi$-conjugated polymers has been of considerable interest over the last three decades because of their organic semiconductor properties. Primary photoexcitations, Frenkel excitons, can be probed optically by means of…
Exciton condensation, characterized by uniform phase coherence across macroscopic length scales, has enabled the discovery of a variety of excitonic states, greatly enriching our understanding of correlated many-body physics. More exotic…
The theory of Bloembergen and Pershan for the light waves at the boundary of nonlinear media is extended to a nonlinear two-dimensional atomic crystal, i.e. a single planar atomic lattice, placed in between linear bulk media. The crystal is…
Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…
Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…
Nonlinear optical properties of extracted higher fullerenes - C70, C76, C78, and C84 - are theoretically investigated. Magnitudes of off-resonant third-harmonic-generation are calculated by the intermediate exciton theory. We find that…