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We assess the capabilities of hydrodynamic density functional theory (DFT) to predict mass transfer across vapor-liquid interfaces by studying the response of an initially equilibrated pure component vapor-liquid system to the localized…

Chemical Physics · Physics 2025-07-08 B. Bursik , F. Bender , R. Stierle , G. Bauer , J. Gross

Two-dimensional mixtures of dipolar colloidal particles with different dipole moments exhibit extremely rich self-assembly behaviour and are relevant to a wide range of experimental systems, including charged and super-paramagnetic colloids…

Soft Condensed Matter · Physics 2019-04-16 W. R. C. Somerville , J. L. Stokes , A. M. Adawi , T. S. Horozov , A. J. Archer , D. M. A. Buzza

The origin of the dramatic changes in the behavior of liquids as they approach their vitreous state - increases of many orders of magnitude in transport properties and dynamic time scales - is a major unsolved problem in condensed matter.…

Soft Condensed Matter · Physics 2015-06-23 R. Casalini , D. Fragiadakis , C. M. Roland

We present an extensive treatment of the generalized mode-coupling theory (GMCT) of the glass transition, which seeks to describe the dynamics of glass-forming liquids using only static structural information as input. This theory amounts…

Statistical Mechanics · Physics 2016-07-05 Liesbeth M. C. Janssen , Peter Mayer , David R. Reichman

We review the Random First Order Transition Theory of the glass transition, emphasizing the experimental tests of the theory. Many distinct phenomena are quantitatively predicted or explained by the theory, both above and below the glass…

Disordered Systems and Neural Networks · Physics 2015-06-25 Vassiliy Lubchenko , P. G. Wolynes

Mass transport phenomenon in concrete structures is strongly coupled with their mechanical behavior. The first coupling fabric is the Biot's theory according to which fluid pressure interacts with solid stress state and volumetric…

Computational Engineering, Finance, and Science · Computer Science 2023-12-18 Jan Eliáš , Gianluca Cusatis

Dense or glassy active matter, as a result of its remarkable resemblance to passive glass-forming materials, is enjoying increasing scientific interest. To better grasp the subtle effect of active motion on the process of vitrification, a…

Soft Condensed Matter · Physics 2023-10-20 Vincent E. Debets , Liesbeth M. C. Janssen

We analyze the dynamics of model supercooled liquids in a temperature regime where predictions of mode coupling theory (MCT) are known to be valid qualitatively. In this regime, the Adam-Gibbs (AG) relation, based on an activation picture…

We present a comprehensive theoretical study of finite size effects in the relaxation dynamics of glass-forming liquids. Our analysis is motivated by recent theoretical progress regarding the understanding of relevant correlation length…

Statistical Mechanics · Physics 2012-09-12 Ludovic Berthier , Giulio Biroli , Daniele Coslovich , Walter Kob , Cristina Toninelli

Using molecular dynamics simulations, we study the slow dynamics of supercooled liquids confined in a random matrix of immobile obstacles. We study the dynamical crossover from glass-like to Lorentz-gas-like behavior in terms of the density…

Soft Condensed Matter · Physics 2011-05-30 Kang Kim , Kunimasa Miyazaki , Shinji Saito

The question about the existence of a structural glass transition in two dimensions is studied using mode coupling theory (MCT). We determine the explicit d-dependence of the memory functional of mode coupling for one-component systems.…

Soft Condensed Matter · Physics 2009-11-13 M. Bayer , J. Brader , F. Ebert , E. Lange , M. Fuchs , G. Maret , R. Schilling , M. Sperl , J. P. Wittmer

Hard constraints imposed in statistical mechanics models can lead to interesting thermodynamical behaviors, but may at the same time raise obstructions in the thoroughfare to thermal equilibration. Here we study a variant of Baxter's…

Statistical Mechanics · Physics 2007-11-30 C. Castelnovo , P. Pujol , C. Chamon

We study the role of active coupling on the transport properties of homogeneously charged macromolecules in an infinitely dilute solution. An enzyme becomes actively bound to a segment of the macromolecule, exerting an electrostatic force…

Soft Condensed Matter · Physics 2024-05-24 Tapas Singha , Siao-Fong Li , Murugappan Muthukumar

We analyse the dynamics of a two dimensional system of interacting active dumbbells. We characterise the mean-square displacement, linear response function and deviation from the equilibrium fluctuation-dissipation theorem as a function of…

The correlation-driven Mott transition is commonly characterized by a drop in resistivity across the insulator-metal phase boundary; yet, the complex permittivity provides a deeper insight into the microscopic nature. We investigate the…

Molecular dynamics simulations are performed to study spatially heterogeneous dynamics in a model of viscous silica above and below the critical temperature of the mode coupling theory, $T_{MCT}$. Specifically, we follow the evolution of…

Soft Condensed Matter · Physics 2009-11-10 M. Vogel , S. C. Glotzer

The high-pressure dynamics of a computer-modeled silica melt is studied in the framework of the mode-coupling theory of the glass transition (MCT) using static-structure input from molecular-dynamics (MD) computer simulation. The theory…

Materials Science · Physics 2009-11-13 Th. Voigtmann , J. Horbach

Using molecular dynamics computer simulations we study the dynamics of a molecular liquid by means of a general class of time-dependent correlators S_{ll'}^m(q,t) which explicitly involve translational (TDOF) and orientational degrees of…

Statistical Mechanics · Physics 2009-10-30 Stefan Kammerer , Walter Kob , Rolf Schilling

In the Second Order Theories (SOT) of real relativistic fluids, the non-ideal properties of the flows are described by a new set of dynamical tensor variables. In this work we explore the non-linear dynamics of those variables in a…

High Energy Physics - Theory · Physics 2020-07-14 Nahuel Mirón-Granese , Alejandra Kandus , Esteban Calzetta

Mode coupling theory (MCT) appears to explain several, though not all, aspects of the glass transition in colloids (particularly when short-range attractions are present). Developments of MCT, from rational foundations in statistical…

Soft Condensed Matter · Physics 2007-05-23 M. E. Cates , C. B. Holmes , M. Fuchs , O. Henrich
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