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Inelastic neutron scattering is applied to study the role of magnetism in stabilizing the charge ordered state in \emph{R}$_{1/3}$Sr$_{2/3}$FeO$_{3}$ (\emph{R}SFO) (\emph{R} = La, Pr, and Nd). The ratio of the ferromagnetic exchange energy…

Strongly Correlated Electrons · Physics 2015-05-28 J. Ma , J. -Q. Yan , S. O. Diallo , R. Stevens , A. Llobet , F. Trouw , D. L. Abernathy , M. B. Stone , R. J. McQueeney

In the present work we analyze the influence of the charge-ordering on the magnetocaloric effect of Pr$_{1-x}$Ca$_x$MnO$_3$ manganites. The results for the samples with $x<$0.30 present the usual ferromagnetic behavior, peaking at the Curie…

Materials Science · Physics 2007-05-23 M. S. Reis , V. S. Amaral , J. P. Araujo , P. B. Tavares , A. M. Gomes , I. S. Oliveira

Charge ordering of V4+ and V5+ in NaV2O5 has been studied by an X-ray diffraction technique using anomalous scattering near a vanadium K-absorption edge to critically enhance a contrast between the two ions. A dramatic energy dependence of…

Strongly Correlated Electrons · Physics 2009-10-31 H. Nakao , K. Ohwada , N. Takesue , Y. Fujii , M. Isobe , Y. Ueda , M. v. Zimmermann , J. P. Hill , D. Gibbs , J. C. Woicik , I. Koyama , Y. Murakami

Infrared absorption study has been carried out on a series of half doped manganites, $La_{0.5}Ca_{0.5-x}Sr_{x}MnO_{3}$ $(0.1\leq x\leq0.5)$, with varying magnetic ground state. The charge ordering transition observed in samples with…

Materials Science · Physics 2015-05-20 Indu Dhiman , A. Das , K. R. Priolkar , P. S. R. Murthy

Using resonant soft X-ray techniques we follow the magnetic behavior of a strained epitaxial film of CoCr2O4, a type-II multiferroic. The film is [110]-oriented, such that both the ferroelectric and ferromagnetic moments can coexist in…

Static charge-density wave (CDW) and spin-density wave (SDW) order has been convincingly observed in La-based cuprates for some time. However, more recently it has been suggested by quantum oscillation, transport and thermodynamic…

We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the…

Strongly Correlated Electrons · Physics 2013-04-23 Feng Ye , Songxue Chi , Bryan C. Chakoumakos , Jaime A. Fernandez-Baca , Tongfei Qi , G. Cao

We have investigated cobaltite relatives of the layered perovskite cuprates and nickelates, Pr$_{2-x}$Ca$_x$CoO$_4$ ($0.39 \leq x \leq 0.73$) and La$_{2-x}$Sr$_x$CoO$_4$ ($x = 0.61$), using elastic neutron scattering. We have discovered…

Strongly Correlated Electrons · Physics 2010-07-28 N. Sakiyama , I. A. Zaliznyak , S. -H. Lee , Y. Mitsui , H. Yoshizawa

Spin, charge, and orbital structures in models for doped manganites are studied by a combination of analytic mean-field and numerical relaxation techniques. At realistic values for the electron-phonon and antiferromagnetic $t_{2g}$ spin…

Strongly Correlated Electrons · Physics 2009-10-31 Takashi Hotta , Elbio Dagotto

Soft x-ray resonant scattering at the Ni L2,3 edges is used to test models of magnetic and orbital-ordering below the metal-insulator transition in NdNiO3. The large branching ratio of the L3 to L2 intensities of the (1/2,0,1/2) reflection…

Strongly Correlated Electrons · Physics 2009-11-11 V. Scagnoli , U. Staub , A. M. Mulders , M. Janousch , G. I. Meijer , G. Hammerl , J. M. Tonnerre , N. Stojic

In spinel-type nickelate NiRh$_2$O$_4$, magnetic ordering is observed upon the sample synthesized via kinetically controlled low-temperature solid-state metathesis, as opposed to previously-reported samples obtained through conventional…

Strongly Correlated Electrons · Physics 2023-10-24 Yuya Haraguchi , Daisuke Nishio-Hamane , Hiroko Aruga Katori

We present a formula for the calculation of K-edge resonant inelastic x-ray scattering on transition metal compounds, based on a local interaction between the valence shell electrons and the $1s$ core hole. Extending a previous result, we…

Materials Science · Physics 2017-08-21 T. F. Seman , X. Liu , J. P. Hill , M. van Veenendaal , K. H. Ahn

CoSeO$_4$ has a structure consisting of edge-sharing chains of Co$^{2+}$ octahedra which are held together by SeO$_4^{2-}$ tetrahedra via shared oxygen atoms at the edges of the octahedra. DC magnetization measurements indicate a transition…

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

Superconductivity · Physics 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

In order to determine types of the orbital ordering in manganites, we study theoretically the polarization dependence of the anomalous X-ray scattering which is caused by the anisotropy of the scattering factor. The general formulae of the…

Strongly Correlated Electrons · Physics 2009-10-31 Sumio Ishihara , Sadamichi Maekawa

We performed resonant x-ray diffraction experiments at the $L$ absorption edges for the post-perovskite-type compound CaIrO$_{3}$ with $(t_{2g})^5$ electronic configuration. By observing the magnetic signals, we could clearly see that the…

We report coherent x-ray scattering studies of charge and orbital domains in manganite systems. The experiments were carried out on LaMnO_3 and Pr_{0.6}Ca_{0.4}MnO_3, with the incident photon energy tuned near the Mn K edge. At room…

Strongly Correlated Electrons · Physics 2009-11-07 C. S. Nelson , J. P. Hill , Doon Gibbs , F. Yakhou , F. Livet , Y. Tomioka , T. Kimura , Y. Tokura

By means of first-principles simulations, we unambiguously show that improper ferroelectricity in magnetite in the low-temperature insulating phase is driven by charge-ordering. An accurate comparison between monoclinic ferroelectric Cc and…

Materials Science · Physics 2015-05-13 Kunihiko Yamauchi , Tetsuya Fukushima , Silvia Picozzi

We study theoretically the anomalous X-ray scattering as a new probe to observe the orbital orderings and excitations in perovskite manganites. The scattering matrix is given by the virtual electronic excitations from Mn $1s$ level to…

Strongly Correlated Electrons · Physics 2009-10-30 Sumio Ishihara , Sadamichi Maekawa

Based on the Hamiltonian of small polarons with the strong nearest neighbor repulsion, we have investigated the charge ordering phenomena observed in half-doped manganites R_{1/2}A_{1/2}MnO_3. We have explored possible consequences of the…

Condensed Matter · Physics 2009-10-30 J. D. Lee , B. I. Min
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