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Resonant-magnetic x-ray scattering (RMXS) near the vanadium $L_{2,3}$-absorption edges has been used to investigate the low temperature magnetic structure of high quality \bvs\ single crystals. Below $T_N$ = 31 K, the strong resonance…

Strongly Correlated Electrons · Physics 2011-04-27 Ph. Leininger , V. Ilakovac , Y. Joly , E. Schierle , E. Weschke , O. Bunau , H. Berger , J. -P. Pouget , P. Foury-Leylekian

The magnetic properties of the layered oxypnictide LaMnAsO have been revisited using neutron scattering and magnetization measurements. The present measurements identify the N\'{e}el temperature $T_N$ = 360(1) K. Below $T_N$ the critical…

Strongly Correlated Electrons · Physics 2016-02-10 Michael A. McGuire , V. Ovidiu Garlea

We study the resonant x-ray scattering at Si and Al K-edges from chiral materials, $\alpha$-quartz and $\alpha$-berlinite. We derive the general form of the scattering matrix for the dipole transition by summing up the local scattering…

Materials Science · Physics 2012-10-03 Jun-ichi Igarashi , Manabu Takahashi

Using soft-x-ray diffraction at the site-specific resonances in the Fe L23 edge, we find clear evidence for orbital and charge ordering in magnetite below the Verwey transition. The spectra show directly that the (001/2) diffraction peak…

Strongly Correlated Electrons · Physics 2010-01-25 J. Schlappa , C. Schuessler-Langeheine , C. F. Chang , H. Ott , A. Tanaka , Z. Hu , M. W. Haverkort , E. Schierle , E. Weschke , G. Kaindl , L. H. Tjeng

The effective Hamiltonian for perovskite titanates is derived by taking into account the three-fold degeneracy of $t_{2g}$ orbitals and the strong electron-electron interactions. The magnetic and orbital ordered phases are studied in the…

Strongly Correlated Electrons · Physics 2009-11-07 S. Ishihara , T. Hatakeyama , S. Maekawa

Neutron scattering has been used to study the nature of the ferromagnetic transition in a single crystal of the perovskite La0.7Ca0.3MnO3. Diffuse scattering from lattice polarons develops as the Curie temperature is approached from below,…

Strongly Correlated Electrons · Physics 2009-10-31 C. P. Adams , J. W. Lynn , Y. M. Mukovskii , A. A. Arsenov , D. A. Shulyatev

We studied the (001/2) diffraction peak in the low-temperature phase of magnetite (Fe3O4) using resonant soft x-ray diffraction (RSXD) at the Fe-L2,3 and O-K resonance. We studied both molecular-beam-epitaxy (MBE) grown thin films and…

We have studied the field and temperature dependence of the magnetization of single crystals of Sr3NiIrO6. These measurements evidence the presence of an easy axis of anisotropy and two anomalies in the magnetic susceptibility. Neutron…

Orbital degree of freedom of electrons and its interplay with spin, charge and lattice degrees of freedom are one of the central issues in colossal magnetoresistive manganites. The orbital degree of freedom has until recently remained…

Strongly Correlated Electrons · Physics 2009-11-07 Sumio Ishihara , Sadamichi Maekawa

The charge and spin correlations in La$_{1.875}$Ba$_{0.125}$CuO$_4$ (LBCO 1/8) are studied using Cu $L_3$ edge resonant inelastic x-ray scattering (RIXS). The static charge order (CO) is observed at a wavevector of $(0.24,0)$ and its charge…

X-ray resonant scattering at the K-edge of transition metal oxides is shown to measure the orbital order parameter, supposed to accompany magnetic ordering in some cases. Virtual transitions to the 3d-orbitals are quadrupolar in general. In…

Strongly Correlated Electrons · Physics 2009-10-30 Michele Fabrizio , Massimo Altarelli , Maurizio Benfatto

We present an analysis of the dependence of the resonant orbital order and magnetic scattering spectra on the spin configuration. We consider an arbitrary spin direction with respect to the local crystal field axis, thus lowering…

Strongly Correlated Electrons · Physics 2016-08-16 N. Stojić , N. Binggeli , M. Altarelli

Charge-lattice fluctuations are observed in the layered perovskite manganite LaSr2Mn2O7 by Raman spectroscopy as high as 340 K and with decreasing temperature they become static and form a charge ordered (CO) phase below TCO=210 K. In the…

The influence of the A-site ionic radii (<rA>) on the magnetic structure has been investigated in La0.5Ca0.5-xSrxMnO3 compounds (0 .GE. x .LE. 0.5) using neutron diffraction, magnetization, and resistivity techniques. All compounds in the…

Strongly Correlated Electrons · Physics 2009-11-13 Indu Dhiman , A. Das , P. K. Mishra , L. Panicker

We report an experimental study of \nco, a Mott insulator containing chains of edge-sharing CuO$_4$ plaquettes, by polarized x-ray absorption spectroscopy (XAS), resonant magnetic x-ray scattering (RMXS), magnetic susceptibility, and…

Strongly Correlated Electrons · Physics 2010-12-07 Ph. Leininger , M. Rahlenbeck , M. Raichle , B. Bohnenbuck , E. Weschke , E. Schierle , A. Maljuk , C. T. Lin , S. Seki , Y. Tokura , J. W. Freeland , B. Keimer

Through a neutron scattering, charge transport, and magnetization study, the correlated ground state in the bilayer iridium oxide Sr$_3$Ir$_2$O$_7$ is explored. Our combined results resolve scattering consistent with a high temperature…

Successive magnetic phase transitions at $T_{\text{N}}$=12.2 K, $T_{\text{N}}^{\;\prime}$=7.0 K, and $T_{\text{N}}^{\;*}$=5.0 K in EuIrGe$_3$, an intermetallic compound with a body centered tetragonal lattice belonging to a polar space…

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

A weak magnetic order was found in a non-superconducting bilayered-hydrate Na$_{x}$CoO$_{2}\cdot y$H$_{2}$O sample by a Co Nuclear Quadrupole Resonance (NQR) measurement. The nuclear spin-lattice relaxation rate divided by temperature…

Superconductivity · Physics 2009-11-10 Y. Ihara , K. Ishida , C. Michioka , M. Kato , K. Yoshimura , K. Takada , T. Sasaki , H. Sakurai , E. Takayama-Muromachi

We studied the stripe phase of La1.8Sr0.2NiO4 using neutron diffraction, resonant soft x-ray diffraction (RSXD) at the Ni L2,3 edges, and resonant x-ray diffraction (RXD) at the Ni K threshold. Differences in the q-space resolution of the…