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Here we present a theoretical analysis of inelastic effects on thermoelectric properties of molecular-scale junction in both linear and nonlinear response regimes. Considered device is composed of molecular quantum dot (with discrete energy…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Kamil Walczak

Realistic nucleon-nucleon interaction induce correlations to the nuclear many-body system which lead to a fragmentation of the single-particle strength over a wide range of energies and momenta. We address the question of how this…

Nuclear Theory · Physics 2007-05-23 Arnau Rios , Artur Polls , Angels Ramos , Herbert Müther

Building on a beyond-GW many-body framework that incorporates higher-order vertex effects in the self-energy -- giving rise to T-matrix and second-order exchange contributions -- this approach is extended to now include the vertex derived…

Computational Physics · Physics 2025-05-14 Brian Cunningham

Ab initio many-body perturbation theory within the $GW$ approximation is a Green's function formalism widely used in the calculation of quasiparticle excitation energies of solids. In what has become an increasingly standard approach,…

In this work we include electron-electron interaction beyond Hartree-Fock level in our non-equilibrium Green's function approach by a crude form of GW through the Single Plasmon Pole Approximation. This is achieved by treating all…

Mesoscale and Nanoscale Physics · Physics 2016-05-02 David O. Winge , Martin Franckié , Claudio Verdozzi , Andreas Wacker , Mauro F. Pereira

A nonequilibrium Green's functions (NEGF) approach for spatially inhomogeneous, strongly correlated artificial atoms is presented and applied to compute the time-dependent properties while starting from a (correlated) initial few-electron…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 K Balzer , M Bonitz

We derive the explicit expression of the three self-energies that one encounters in many-body perturbation theory: the well-known $GW$ self-energy, as well as the particle-particle and electron-hole $T$-matrix self-energies. Each of these…

Chemical Physics · Physics 2024-03-01 Roberto Orlando , Pina Romaniello , Pierre-François Loos

We present an ab initio approach to electronic transport in nanoscale systems which includes electronic correlations through the GW approximation. With respect to Landauer approaches based on density-functional theory (DFT), we introduce a…

Mesoscale and Nanoscale Physics · Physics 2010-09-08 Pierre Darancet , Andrea Ferretti , Didier Mayou , Valerio Olevano

We calculate groundstate total energies and single-particle excitation energies of seven pi conjugated molecules described with the semi-empirical Pariser-Parr-Pople (PPP) model using self-consistent many-body perturbation theory at the GW…

Mesoscale and Nanoscale Physics · Physics 2013-11-22 K. Kaasbjerg , K. S. Thygesen

We calculate single-particle excitation energies for a series of 33 molecules using fully selfconsistent GW, one-shot G$_0$W$_0$, Hartree-Fock (HF), and hybrid density functional theory (DFT). All calculations are performed within the…

Materials Science · Physics 2015-05-14 C. Rostgaard , K. W. Jacobsen , K. S. Thygesen

One of the few exact results for the description of the time-evolution of an inhomogeneous, interacting many-particle system is given by the Harmonic Potential Theorem (HPT). The relevance of this theorem is that it sets a tight constraint…

Nuclear Theory · Physics 2019-09-18 S. Zanoli , X. Roca-Maza , G. Colò , S. Shen

A fully analytical approximation for the observable characteristics of many-electron atoms is developed via a complete and orthonormal hydrogen-like basis with a single-effective charge parameter for all electrons of a given atom. The basis…

Quantum Physics · Physics 2017-12-06 O. D. Skoromnik , I. D. Feranchuk , A. U. Leonau , C. H. Keitel

The self-energy embedding theory (SEET), in which the active space self-energy is embedded in the self-energy obtained from a perturbative method treating the non-local correlation effects, was recently developed in our group. In SEET the…

Chemical Physics · Physics 2016-11-15 Tran Nguyen Lan , Alexei A. Kananenka , Dominika Zgid

The total energy and electron addition and removal spectra can in principle be obtained exactly from the one-body Green's function. In practice, the Green's function is obtained from an approximate self-energy. In the framework of many-body…

Strongly Correlated Electrons · Physics 2023-12-08 Abdallah El-Sahili , Francesco Sottile , Lucia Reining

We review the Bethe-Salpeter equation (BSE) approach to the calculation of electronic excitation energies of molecular systems. We recall the general Green's function many-theory formalism and give the working equations of the BSE approach…

Chemical Physics · Physics 2013-04-05 Elisa Rebolini , Julien Toulouse , Andreas Savin

A novel self-consistent implementation of Hedin's GW perturbation theory is introduced. This finite-temperature method uses Hartree-Fock wave functions to represent Green's function. GW equations are solved with full potential linear…

Strongly Correlated Electrons · Physics 2015-05-13 Andrey Kutepov , Sergey Yu. Savrasov , Gabriel Kotliar

Starting from the full many-body Hamiltonian of interacting electrons the effective self-energy acting on electrons residing in a subspace of the full Hilbert space is derived. This subspace may correspond to, for example, partially filled…

Strongly Correlated Electrons · Physics 2010-10-20 F. Aryasetiawan , J. M. Tomczak , T. Miyake , R. Sakuma

In this paper, we propose a generic and systematic approach for study of the electronic structure for atoms or molecules. In particular, we address the issue of single particle states, or orbitals, which should be one of the most important…

Chemical Physics · Physics 2007-05-23 Liqiang Wei

Electron-electron interactions seem to play a surprisingly small role in the description of the integer quantum Hall effect, considering that for just slightly different filling factors the interactions are of utmost importance causing the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Christoph Sohrmann , Rudolf A. Roemer

We present an approach for self-consistent calculations of the many-body Green function in transition metals. The distinguishing feature of our approach is the use of the one-site approximation and the self-consistent quasiparticle wave…

Strongly Correlated Electrons · Physics 2009-11-07 N. E. Zein , V. P. Antropov