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We have studied the dielectric properties of the ferromagnetic spinel CdCr$_2$S$_4$ from first principles. Zone-center phonons and Born effective charges were calculated by frozen-phonon and Berry phase techniques within LSDA+U. We find…

Materials Science · Physics 2009-11-11 Craig J. Fennie , Karin M. Rabe

A magneto-optical survey was conducted for HgCr$_2$O$_4$ powder samples under pulsed high magnetic fields of up to 55 T. Intensity changes in magnetic fields observed for the exciton-magnon-phonon optical transition spectra coincide well…

Materials Science · Physics 2015-05-14 Daisuke Nakamura , Atsuhiko Miyata , Hiroaki Ueda , Shojiro Takeyama

The interplay between different degrees of freedom such as charge, spin, orbital, and lattice has received a great deal of interest due to its potential to engineer materials properties and their functionalities for device applications. In…

Materials Science · Physics 2021-10-26 Bommareddy Poojitha , Ankit Kumar , Anjali Rathore , Devesh Negi , Surajit Saha

The interplay between spin dynamics and lattice vibration has been suggested as an important part of the puzzle of high-temperature superconductivity. Here we report the strong interaction between spin fluctuation and phonon in SmFeAsO, a…

Superconductivity · Physics 2010-10-29 L. Zhang , P. F. Guan , D. L. Feng , X. H. Chen , S. S. Xie , M. W. Chen

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

Strongly Correlated Electrons · Physics 2012-05-01 Pradeep Kumar , A. Bera , D. V. S. Muthu , S. N. Shirodkar , R. Saha , A. Shireen , A. Sundaresan , U. V. Waghmare , A. K. Sood , C. N. R. Rao

The observation of strongly coupled lattice and spin dynamics in altermagnet CoF$_2$ is reported. On the background of the expected spin-phonon interaction leading to renormalization of all phonons at the Neel temperature an additional…

Materials Science · Physics 2024-05-14 M. A. Prosnikov , M. Bal , R. V. Pisarev , P. C. M. Christianen , A. M. Kalashnikova

The crystal and magnetic structures of stoichiometric ZnCr2Se4 have been investigated using synchrotron X-ray and neutron powder diffraction, muon spin relaxation (muSR) and inelastic neutron scattering. Synchrotron X-ray diffraction shows…

Strongly Correlated Electrons · Physics 2017-04-12 P. Zajdel , W-Y. Li , W. Van Beek , A. Lappas , A. Ziolkowska , S. Jaskiewicz , C. Stock , M. A. Green

We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

Materials Science · Physics 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

We have investigated the dielectric anomalies associated with spin ordering transitions in the tetragonal spinel Mn$_3$O$_4$, using thermodynamic, magnetic, and dielectric measurements. We find that two of the three magnetic ordering…

Materials Science · Physics 2007-10-16 R. Tackett , G. Lawes , B. C. Melot , M. Grossman , E. S. Toberer , R. Seshadri

The $T$-dependence (2- 400 K) of the electron paramagnetic resonance (EPR), magnetic susceptibility, $\chi (T)$, and specific heat, $C_{v}(T)$, of the $normal$ antiferromagnetic (AFM) spinel ZnCr$_{2}$O$_{4}$ and the spin-glass (SG)…

First-principles calculations reveal large zone-center spin-phonon coupling and magnetically-driven phonon anisotropy in cubic perovskites Sr$M$O$_3$ ($M$=V,Cr,Mn,Fe,Co). In particular, the frequency and splitting of the polar Slater mode…

Strongly Correlated Electrons · Physics 2012-09-10 Jun Hee Lee , Karin M. Rabe

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

We present an elaborate electron-spin resonance study of the low-energy dynamics and magnetization in the ordered phase of the magnetically frustrated spinel ZnCr$_2$O$_4$. We observe several resonance modes corresponding to different…

Strongly Correlated Electrons · Physics 2010-11-29 V. N. Glazkov , A. M. Farutin , V. Tsurkan , H. -A. Krug von Nidda , A. Loidl

Cs2CoBr4 is a triangular-lattice antiferromagnet which can be viewed as weakly interacting spin chains due to spatially anisotropic frustrating exchange couplings. The spin-orbit interaction in Co(2+) spin-3/2 ions leads to a strong…

Strongly Correlated Electrons · Physics 2023-09-06 T. A. Soldatov , A. I. Smirnov , A. V. Syromyatnikov

Low-temperature magnetic resonance study of the quasi-two-dimensional antiferromagnet Cu(en)(H$_2$O)$_2$SO$_4$ (en = C$_2$H$_8$N$_2$) was performed down to 0.45~K. This compound orders antiferromagnetically at 0.9K. The analysis of the…

Strongly Correlated Electrons · Physics 2020-02-19 V. N. Glazkov , Yu. V. Krasnikova , I. K. Rodygina , J. Chovan , R. Tarasenko , A. Orendáčová

Two-dimensional (2D) van der Waals (vdW) magnets with spin-phonon coupling are crucial for next-generation spintronics. Among them, Fe3GaTe2 has attracted widespread attention due to above-room-temperature intrinsic ferromagnetism and large…

Materials Science · Physics 2024-12-02 Gaojie Zhang , Hao Wu , Li Yang , Wen Jin , Bichen Xiao , Wenfeng Zhang , Haixin Chang

Ultrasound and magnetization studies of bond-frustrated ZnCr2S4 spinel are performed in static magnetic fields up to 18 T and in pulsed fields up to 62 T. At temperatures below the antiferromagnetic transition at T_N1 14 K the sound…

Strongly Correlated Electrons · Physics 2015-03-19 V. Tsurkan , S. Zherlitsyn , V. Felea , S. Yasin , Yu. Skourski , J. Deisenhofer , H. -A. Krug von Nidda , P. Lemmens , J. Wosnitza , A. Loidl

We present a comparative far-infrared reflection spectroscopy study of phonons, phase transitions, spin-phonon and electron-phonon interactions in isostructural multiferroic iron borates of gadolinium and terbium. The behavior of phonon…

Strongly Correlated Electrons · Physics 2016-03-02 S. A. Klimin , A. B. Kuzmenko , M. A. Kashchenko , M. N. Popova

In this letter we investigated the temperature-dependent Raman spectra of CaMn7O12 helimagnet from room temperature down to 10 K. The temperature dependence of the Raman mode parameters show remarkable anomalies for both antiferromagnetic…

Recently, unconventional antiferromagnets that enable the splitting of electronic spins have been theoretically proposed and experimentally realized, where the magnetic sublattices containing moments pointing at different directions are…