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The detailed temperature dependence of the infrared-active mode in Fe$_{1.03}$Te ($T_N\simeq 68$ K) and Fe$_{1.13}$Te ($T_N\simeq 56$ K) has been examined, and the position, width, strength, and asymmetry parameter determined using an…

Strongly Correlated Electrons · Physics 2016-05-18 C. C. Homes , Y. M. Dai , J. Schneeloch , R. D. Zhong , G. D. Gu

We perform thermodynamic and inelastic neutron scattering (INS) measurements to study the lattice dynamics (phonons) of a cubic collinear antiferromagnet Cu$_3$TeO$_6$ which hosts topological spin excitations (magnons). While the specific…

An investigation of possibilities for superconductivity mediated by spin fluctuations in some elementary metals is motivated by the recent discovery of superconductivity in the hcp high-pressure phase of iron. The electronic structure, the…

Superconductivity · Physics 2016-08-31 T. Jarlborg

We perform a low temperature Raman scattering study of phononic and collective spin excitations in the orthogonal dimers compound SrCu_2(BO_3)_2, focussing on the symmetry and the effects of external fields on the magnetic modes. The zero…

Strongly Correlated Electrons · Physics 2009-11-11 A. Gozar , B. S. Dennis , H. Kageyama , G. Blumberg

The ScAu$_2$Al superconducting Heusler-type compound was recently characterized to have the highest critical temperature of $T_c = 5.12$ K and the strongest electron-phonon coupling among the Heusler family. In this work, the electronic…

Superconductivity · Physics 2023-12-04 Gabriel Kuderowicz , Bartlomiej Wiendlocha

We have studied the influence of magnetic order on the optical phonons of the geometrically frustrated spinel ZnCr$_2$O$_4$ from first-principles. By mapping the first-principles phonon calculations onto a Heisenberg-like model, we…

Materials Science · Physics 2009-11-11 Craig J. Fennie , Karin M. Rabe

MnCr2O4 that exhibits spin frustration and complex spiral spin order is of great interest from both fundamental as well as application-oriented perspectives. Unlike CoCr2O4 whose ground state presents the coexistence of commensurate spiral…

Low-dimensional frustrated magnetic square networks feature a variety of unconventional phases with novel emergent excitations. Often these excitations are intertwined and manifest into intriguing phenomena, an area that has remained…

Materials Science · Physics 2024-01-10 Shalini Badola , Aprajita Joshi , Akriti Singh , Surajit Saha

We report structural, magnetic, and Raman studies of the disordered double perovskite GdSrCoMnO$_{6}$~(GSCM). DC magnetization shows a ferromagnetic transition at $T_{C} \approx 153$~K. The inverse susceptibility exhibits a downturn above…

We have measured polarized Raman scattering spectra of the Fe$_{1-x}$Co$_{x}$Sb$_{2}$ and Fe$_{1-x}$Cr$_{x}$Sb$_{2}$ (0$\leq x\leq $0.5) single crystals in the temperature range between 15 K and 300 K. The highest energy $B_{1g}$ symmetry…

Strongly Correlated Electrons · Physics 2016-09-20 N. Lazarević , Z. V. Popović , Rongwei Hu , C. Petrovic

We performed small-angle neutron scattering (SANS) measurements on the helimagnetic spinel compound ZnCr2Se4. The ground state of this material is a multi-domain spin-spiral phase, which undergoes domain selection in a magnetic field and…

Strongly Correlated Electrons · Physics 2016-03-15 A. S. Cameron , Y. V. Tymoshenko , P. Y. Portnichenko , J. Gavilano , V. Tsurkan , V. Felea , A. Loidl , S. Zherlitsyn , J. Wosnitza , D. S. Inosov

We report on bifurcations effect mediated by the electron-phonon coupling in a concentrated rare-earth-containing antiferromagnet, observed in the spectra of coupled $4f$-electron-phonon modes under the influence of an external magnetic…

The canting angles and fluctuation of the magnetic ion spins of spinel oxide MnCr${}_2$O${}_4$ were studied by nuclear magnetic resonance (NMR) at low temperatures, which has a collinear ferrimagnetic order below $T_C$ and a ferrimagnetic…

Strongly Correlated Electrons · Physics 2015-05-19 Dong Young Yoon , Soonchil Lee , Yoon Seok Oh , Kee Hoon Kim

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

Strongly Correlated Electrons · Physics 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

The strength of the electron-phonon coupling parameter and its evolution throughout a solid's phase diagram often determines phenomena such as superconductivity, charge- and spin-density waves. Its experimental determination relies on the…

The temperature dependent ac and dc magnetization and heat capacity data of Ca$_3$CoIrO$_6$, a spin-chain compound crystallizing in a K$_4$CdCl$_6$-derived rhombohedral structure, show the features due to magnetic ordering of a…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

We provide a theoretical demonstration of controllable non-relativistic spin splitting in both electronic and magnonic bands via targeted structural distortions tied to specific phonon modes. Using MnF$_2$ as a model system, we identify a…

Materials Science · Physics 2025-09-11 Subhadeep Bandyopadhyay , Anoop Raj , Philippe Ghosez , Sumiran Pujari , Sayantika Bhowal

We performed Raman spectroscopy measurements under temperature changes from 10 K up to 850 K to probe the phonon-spin coupling in Y$_2$NiMnO$_6$. The spin-phonon coupling was observed as a softening of the stretching mode, indicating this…

Using Raman spectroscopy to study the correlated 4$d$-electron metal Sr$_2$RhO$_4$, we observe pronounced excitations at 220 meV and 240 meV with $A_\mathrm{1g}$ and $B_\mathrm{1g}$ symmetries, respectively. We identify them as transitions…

We measured two magnetic modes with finite and discrete energies in an antiferromagnetic ordered phase of a geometrically frustrated magnet MgCr2O4 by single-crystal inelastic neutron scattering, and clarified the spatial spin correlations…

Strongly Correlated Electrons · Physics 2008-10-22 K. Tomiyasu , H. Suzuki , M. Toki , S. Itoh , M. Matsuura , N. Aso , K. Yamada
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