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The crystal structure and the magnetism of BaMn$_2$O$_3$ have been studied by thermodynamic and by diffraction techniques using large single crystals and powders. BaMn$_2$O$_3$ is a realization of a $S = 5/2$ spin ladder as the magnetic…

Strongly Correlated Electrons · Physics 2015-05-20 M. Valldor , O. Heyer , A. C. Komarek , A. Senyshyn , M. Braden , T. Lorenz

An $S=1/2$ ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain model is investigated in connection to its realization compound: (CH$_3$)$_2$CHNH$_3$Cu(Cl$_x$Br$_{1-x}$)$_3$. The exchange interaction…

Disordered Systems and Neural Networks · Physics 2009-11-10 Tota Nakamura

Spin correlations in metallic and insulating phases of $V_2O_3$ and its derivatives are investigated using magnetic neutron scattering. Metallic samples have incommensurate spin correlations varying little with hole doping. Paramagnetic…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , C. Broholm , G. Aeppli , P. Dai , J. M. Honig , P. Metcalf

A possibility of the uniform antiferromagnetic order is pointed out in an S=1/2 ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain compound: (CH_3)_2 CHNH_3 Cu(Cl_x Br_{1-x})_3. The system possesses…

Statistical Mechanics · Physics 2009-11-07 Tota Nakamura

The phase diagrams of the spin-$3/2$ Blume-Capel model with competing short and long-range interactions were studied through the free energy density obtained by analytical methods. The competition emerges when positive short-range…

We present a detailed powder and single crystal neutron diffraction study of the spin chain compound Ca3Co2O6. Below 25 K, the system orders magnetically with a modulated partially disordered antiferromagnetic structure. We give a…

Strongly Correlated Electrons · Physics 2008-09-17 S. Agrestini , L. C. Chapon , A. Daoud-Aladine , J. Schefer , A. Gukasov , C. Mazzoli , M. R. Lees , O. A. Petrenko

Magnetic properties and magnetic structure of the Ba$_{2}$Mn(PO$_{4}$)$_{2}$ antiferromagnet featuring frustrated zigzag chains of $S=\frac{5}{2}$ Mn$^{2+}$ ions are reported based on neutron diffraction, density-functional band-structure…

Strongly Correlated Electrons · Physics 2018-04-10 Arvind Yogi , A. K. Bera , Ashwin Mohan , Ruta Kulkarni , S. M. Yusuf , A. Hoser , A. A. Tsirlin , A. Thamizhavel

Large-spin two-dimensional magnets are generally expected to develop conventional long-range order once the dominant exchange scale becomes appreciable. The layered spin-$3/2$ maple-leaf compound Na$_2$Mn$_3$O$_7$ defies this expectation:…

Strongly Correlated Electrons · Physics 2026-02-27 Hari Borutta , Tobias Müller , Ronny Thomale , Harald O. Jeschke , Yasir Iqbal

Using powder neutron diffraction we have discovered an unusual magnetic order-order transition in the Ising spin chain compound Ca3Co2O6. On lowering the temperature an antiferromagnetic phase with propagation vector k=(0.5,-0.5,1) emerges…

Strongly Correlated Electrons · Physics 2011-05-17 S. Agrestini , C. L. Fleck , L. C. Chapon , C. Mazzoli , A. Bombardi , M. R. Lees , O. A. Petrenko

Spin-spin correlations and microscopic origin of net magnetization in the spin-1 trimer chain compound CaNi3P4O14 have been investigated by powder neutron diffraction. The present study reveals a 3D long-range magnetic ordering below 16 K…

Strongly Correlated Electrons · Physics 2016-05-27 A. K. Bera , S. M. Yusuf , Amit Kumar , M. Majumder , K. Ghoshray , L. Keller

A neutron scattering investigation of the magnetoelectric coupling in PbFe_{1/2}Nb_{1/2}O_{3} (PFN) has been undertaken. Ferroelectric order occurs below 400 K, as evidenced by the softening with temperature and subsequent recovery of the…

Materials Science · Physics 2018-07-20 C. Stock , S. R. Dunsiger , R. A. Mole , X. Li , H. Luo

The magnetic correlations in double perovskites La2Mn2-xNixO6 (x = 0.5, 0.75, 1.0, 1.25 and 1.5) have been systematically investigated across macroscopic, mesoscopic, and microscopic length scales using temperature-dependent bulk DC…

Materials Science · Physics 2025-10-14 A. K. Bera , K. S. Chikara , B. Saha , S. M. Yusuf , Mohd. Nasir , S. Sen

Magnetic correlations in all four phases of pure and doped vanadium sesquioxide V_2O_3 have been examined by magnetic thermal neutron scattering. While the antiferromagnetic insulator can be accounted for by a Heisenberg localized spin…

Strongly Correlated Electrons · Physics 2009-10-31 Wei Bao , C. Broholm , G. Aeppli , S. A. Carter , P. Dai , T. F. Rosenbaum , J. M. Honig , P. Metcalf , S. F. Trevino

The structural and magnetic properties of BaMn2Si2O7 have been investigated. The magnetic susceptibility and specific heat, measured using single crystals, suggest that the quasi-one-dimensional magnetism originating from the loosely…

Materials Science · Physics 2015-06-17 J. Ma , C. D. Dela Cruz , T. Hong , W. Tian , A. A. Aczel , Songxue Chi , J. -Q. Yan , Z. L. Dun , H. D. Zhou , M. Matsuda

A recent experiment reported type-II multiferroicity in monolayer (ML) NiI$_{2}$ based on a presumed spiral magnetic configuration (Spiral-B), which is, as we found here, under debate in the ML limit. Freestanding ML NiI$_{2}$ breaks its…

Materials Science · Physics 2024-06-05 Nanshu Liu , Cong Wang , Changlin Yan , Changsong Xu , Jun Hu , Yanning Zhang , Wei Ji

1H nuclear magnetic resonance (NMR) measurements in [YPc2]0, an organic compound formed by radicals stacking along chains, are presented. The temperature dependence of the macroscopic susceptibility, of the NMR shift and of the spin-lattice…

Strongly Correlated Electrons · Physics 2015-05-20 F. Branzoli , P. Carretta , M. Filibian , S. Klyatskaya , M. Ruben

Raman scattering studies of the frustrated spin chain system LiCu$_{2}$O$_{2}$ are reported. Two transitions into a magnetically ordered phase (taken place at temperatures $\sim$ 9 K and $\sim$ 24 K) have been confirmed from the analysis of…

Strongly Correlated Electrons · Physics 2009-11-10 K. -Y. Choi , S. A. Zvyagin , G. Cao , P. Lemmens

This work is devoted to the analysis of orbital patterns and related to them interatomic magnetic interactions in centrosymmetric monoclinic structures of BiMnO$_3$, which have been recently determined experimentally. First, we set up an…

Materials Science · Physics 2008-07-11 I. V. Solovyev , Z. V. Pchelkina

We report magnetic susceptibility, specific heat and muon spin relaxation (muSR) experiments on the triangular antiferromagnet La2Ca2MnO7 which develops a genuine two-dimensional, three-sublattice \sqrt{3} \times \sqrt{3} magnetic order…

Strongly Correlated Electrons · Physics 2015-07-08 P. Dalmas de Réotier , C. Marin , A. Yaouanc , T. Douce , A. Sikora , A. Amato , C. Baines

Measurements of magnetic susceptibility, heat capacity and thermal expansion are reported for single crystalline CuSb$_{2}$O$_{6}$ in the temperature range $5<T<350$ K. The magnetic susceptibility exhibits a broad peak centered near 60 K…

Strongly Correlated Electrons · Physics 2015-06-16 A. Rebello , M. G. Smith , J. J. Neumeier , B. D. White , Yi-Kuo Yu