English

Transition from one-dimensional antiferromagnetism to three-dimensional antiferromagnetic order in single-crystalline CuSb$_{2}$O$_{6}$

Strongly Correlated Electrons 2015-06-16 v1

Abstract

Measurements of magnetic susceptibility, heat capacity and thermal expansion are reported for single crystalline CuSb2_{2}O6_{6} in the temperature range 5<T<3505<T<350 K. The magnetic susceptibility exhibits a broad peak centered near 60 K that is typical of one-dimensional antiferromagnetic compounds. Long-range antiferromagnetic order at TNT_N = 8.7 K is accompanied by an energy gap (Δ\Delta = 17.48(6) K). This transition represents a crossover from one- to three-dimensional antiferromagnetic behavior. Both heat capacity and the thermal expansion coefficients exhibit distinct jumps at TNT_N, which are similar to those observed at the normal-superconducting phase transition in a superconductor. This behavior is quite unusual, and is presumably associated with a Spin-Peierls transition occurring as a result of three-dimensional phonons coupling with {\it Jordan-Wigner-transformed} Fermions.

Keywords

Cite

@article{arxiv.1306.3961,
  title  = {Transition from one-dimensional antiferromagnetism to three-dimensional antiferromagnetic order in single-crystalline CuSb$_{2}$O$_{6}$},
  author = {A. Rebello and M. G. Smith and J. J. Neumeier and B. D. White and Yi-Kuo Yu},
  journal= {arXiv preprint arXiv:1306.3961},
  year   = {2015}
}

Comments

Submitted to Physical Review B