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Comprehensive x-ray scattering studies have characterized the smectic ordering of octylcyanobiphenyl (8CB) confined in the hydrogen-bonded silica gels formed by aerosil dispersions. For all densities of aerosil and all measurement…

Soft Condensed Matter · Physics 2009-11-07 R. L. Leheny , S. Park , R. J. Birgeneau , J. -L. Gallani , C. W. Garland , G. S. Iannacchione

The effect on the nematic to smectic-A transition in octylcyanobiphenyl (8CB) due to dispersions of hydrogen-bonded silica (aerosil) particles is characterized with high-resolution x-ray scattering. The particles form weak gels in 8CB…

Soft Condensed Matter · Physics 2009-11-07 S. Park , R. L. Leheny , R. J. Birgeneau , J. -L. Gallani , C. W. Garland , G. S. Iannacchione

The effects of dispersed aerosil nanoparticles on two of the phase transitions of the thermotropic liquid crystal material 4-n-pentylphenylthiol-4'-n-octyloxybenzoate 8barS5 have been studied using high-resolution x-ray diffraction…

Soft Condensed Matter · Physics 2009-11-10 P. S. Clegg , R. J. Birgeneau , S. Park , C. W. Garland , G. S. Iannacchione , R. L. Leheny , M. E. Neubert

We have studied the effects of quenched random disorder created by dispersed aerosil nanoparticle gels on the nematic to smectic-A (N-SmA) and smectic-A to reentrant nematic (SmA- RN) phase transitions of thermotropic liquid crystal…

Soft Condensed Matter · Physics 2009-11-13 M. Ramazanoglu , S. Larochelle , C. W. Garland , R. J. Birgeneau

The short-range order which remains when the isotropic to smectic-A transition is perturbed by a gel of silica nanoparticles (aerosils) has been studied using high-resolution synchrotron x-ray diffraction. The gels have been created…

Soft Condensed Matter · Physics 2009-11-10 M. K. Ramazanoglu , P. S. Clegg , R. J. Birgeneau , C. W. Garland , M. E. Neubert , J. M. Kim

We present a neutron scattering analysis of the structure of the smectic liquid crystal octylcyanobiphenyl (8CB) confined in one-dimensional nanopores of porous silicon films (PS). The smectic transition is completely suppressed, leading to…

Soft Condensed Matter · Physics 2016-08-16 Régis Guégan , Denis Morineau , Claude Loverdo , Wilfried Béziel , Mohammed Guendouz

We report studies of the frequency dependent shear modulus, $G^*(\omega)=G'(\omega)+iG''(\omega)$, of the liquid crystal octylcyanobiphenyl (8CB) confined in a colloidal aerosil gel. With the onset of smectic order, $G'$ grows approximately…

Soft Condensed Matter · Physics 2009-11-11 Ranjini Bandyopadhyay , Dennis Liang , Ralph H. Colby , James L. Harden , Robert L. Leheny

We show that smectic liquid crystals confined in_anisotropic_ porous structures such as e.g.,_strained_ aerogel or aerosil exhibit two new glassy phases. The strain both ensures the stability of these phases and determines their nature. One…

Soft Condensed Matter · Physics 2009-10-31 Brad Jacobsen , Karl Saunders , Leo Radzihovsky , John Toner

Liquid crystals offer many unique opportunities to study various phase transitions with continuous symmetry in the presence of quenched random disorder (QRD). The QRD arises from the presence of porous solids in the form of a random gel…

Soft Condensed Matter · Physics 2009-11-07 Germano S. Iannacchione , Sungil Park , Carl W. Garland , Robert J. Birgeneau , Robert L. Leheny

We present a theory of the elasticity and fluctuations of the Smectic A and C phases in uniaxial, anisotropic disordered environments, e.g., stretched aerogel. We find that, bizarrely, the low-temperature, lower-symmetry Smectic $C$ phase…

Soft Condensed Matter · Physics 2013-05-29 Leiming Chen , John Toner

High-resolution ac-calorimetry has been carried out on dispersions of aerosils in the liquid crystal octyloxycyanobiphenyl (8OCB) as a function of aerosil concentration and temperature spanning the crystal to isotropic phases. The…

Soft Condensed Matter · Physics 2016-08-31 A. Roshi , G. S. Iannacchione , P. S. Clegg , R. J. Birgeneau

We study smectic liquid crystals in random environments, e.g., aerogel. A low temperature analysis reveals that even arbitrarily weak quenched disorder (i.e., arbitrarily low aerogel density) destroys translational (smectic) order. A…

Soft Condensed Matter · Physics 2009-10-31 Leo Radzihovsky , John Toner

We study the smectic AC transition in anisotropic and uniaxial disordered environments, e.g., aerogel with an external field. We find very strange behavior of translational correlations: the low-temperature, lower-symmetry Smectic C phase…

Exactly Solvable and Integrable Systems · Physics 2009-11-10 Leiming Chen , John Toner

High-resolution X-ray scattering studies of the nonpolar thermotropic liquid crystal 4-n-pentylphenylthiol-4'-n-octyloxybenzoate (\bar{8}S5) in aerosil gel nano-networks reveal that the aerosil-induced disorder significantly alters both the…

Soft Condensed Matter · Physics 2015-05-28 B. Freelon , M. Ramazanoglu , P. J. Chung , P. Valdivia , C. W. Garland , R. J. Birgeneau

Confinement in the nanochannels of porous silicon strongly affects the phase behavior of the archetype liquid-crystal 4-n-octyl-4-cyanobiphenyl (8CB). A very striking phenom- enon is the development of a short-range smectic order, which…

Soft Condensed Matter · Physics 2011-06-08 Régis Guégan , Ronan Lefort , Wilfried Béziel , Denis Morineau , Mohammed Guendouz , Bernhard Frick

We report combined optical birefringence and neutron scattering measurements on the liquid crystal 12CB nanoconfined in mesoporous silicon layers. This liquid crystal exhibits strong nematic-smectic coupling responsible for a discontinuous…

Mesoscale and Nanoscale Physics · Physics 2010-05-04 Gilbert Chahine , Andriy V. Kityk , Klaus Knorr , Ronan Lefort , Mohammed Guendouz , Denis Morineau , Patrick Huber

The liquid crystal octylcyanobiphenyl (8CB) was doped with the chiral agent CB15 and spin-coated onto a substrate treated for planar alignment of the director, resulting in a film of thickness several hundred nm in the smectic-A phase. In…

Soft Condensed Matter · Physics 2016-10-02 Ian R. Nemitz , Andrew J. Ferris , Emmanuelle Lacaze , Charles Rosenblatt

We study the smectic $A$-$C$ phase transition in biaxial disordered environments, e.g. fully anisotropic aerogel. We find that both the $A$ and $C$ phases belong to the universality class of the "XY Bragg glass", and therefore have…

Soft Condensed Matter · Physics 2015-06-03 Leiming Chen , John Toner

A high-resolution calorimetric study has been carried out on nano-colloidal dispersions of aerosils in the liquid crystal 4-\textit{n}-pentylphenylthiol-4'-\textit{n}-octyloxybenzoate ($\bar{8}$S5) as a function of aerosil concentration and…

Soft Condensed Matter · Physics 2009-11-11 A. Roshi , G. S. Iannacchione , P. S. Clegg , R. J. Birgeneau , M. E. Neubert

We show that discotics, lying deep in the columnar phase, can exhibit an x-ray scattering pattern which mimics that of a somewhat unusual smectic liquid crystal. This exotic, new glassy phase of columnar liquid crystals, which we call a…

Soft Condensed Matter · Physics 2009-10-31 Karl Saunders , Leo Radzihovsky , John Toner
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