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A new mechanism is proposed to explain the origin of negative differential resistance (NDR) in a strongly coupled single molecule-metal junction. A first-principles quantum transport calculation in a Fe-terpyridine linker molecule…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Ranjit Pati , Mike McClain , Anirban Bandyopadhyay

Combining insights from quantum chemistry calculations with master equations, we discuss a mechanism for negative differential resistance (NDR) in molecular junctions, operated in the regime of weak tunnel coupling. The NDR originates from…

Mesoscale and Nanoscale Physics · Physics 2013-01-10 Martin Leijnse , Wei Sun , Mogens Brøndsted Nielsen , Per Hedegård , Karsten Flensberg

Using self-consistent calculations based on Non-Equilibrium Green's Function (NEGF) formalism, the origin of negative differential resistance (NDR) in molecular junctions and quantum wires is investigated. Coupling of the molecule to…

Mesoscale and Nanoscale Physics · Physics 2008-08-21 Hosein Cheraghchi , Keivan Esfarjani

We have observed tunable negative differential resistance (NDR) in scanning tunneling spectroscopy measurements of a double layer of C60 molecules on a metallic surface. Using a simple model we show that the observed NDR behavior is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Grobis , A. Wachowiak , R. Yamachika , M. F. Crommie

We unravel the critical role of vibrational mode softening in single-molecule electronic devices at high bias. Our theoretical analysis is carried out with a minimal model for molecular junctions, with mode softening arising due to…

Mesoscale and Nanoscale Physics · Physics 2020-08-18 Junjie Liu , Dvira Segal

Multipeak negative differential resistance (NDR) molecular devices are designed from first principles. The effect of NDR is associated with the non-linear Stark shifts and the electron localization within the conductive region and contacts.…

Mesoscale and Nanoscale Physics · Physics 2015-01-07 Mikolaj Sadek , Malgorzata Wierzbowska , Michal F. Rode , Andrzej L. Sobolewski

Nonlinear electrical properties, such as negative differential resistance (NDR), are essential in numerous electrical circuits, including memristors. Several physical origins have been proposed to lead to the NDR phenomena in semiconductor…

The conductance-voltage spectrum of molecular nanostructures measured by scanning tunneling spectroscopy (STS) is generally assumed to reflect the local density of states of the molecule. This excludes the possibility of observing negative…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Yongqiang Xue , Supriyo Datta , Seunghun Hong , R. Reifenberger , Jason I. Henderson , Cliff P. Kubiak

We determine the conditions in which negative differential resistance (NDR) appears in the C$_{60}$-based molecular device of [Phys. Rev. Lett. {\bf 100}, 036807 (2008)] by means of ab-initio electron-transport simulations. Our calculations…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Frederico D. Novaes , Manuel Cobian , Alberto Garcia , Pablo Ordejon , Hiromu Ueba , Nicolas Lorente

We investigate the atomic-scale tunneling characteristics of bilayer graphene on silicon carbide using the scanning tunneling microscopy. The high-resolution tunneling spectroscopy reveals an unexpected negative differential resistance…

Field effect transistors with channels made of graphene layer(s) were explored. The graphene layer(s) contacted a distributed array of well-separated semiconductor quantum dots (QDs). The dots were embedded in nano-structured hole-array;…

Mesoscale and Nanoscale Physics · Physics 2013-07-26 Samarth Trivedi , Haim Grebel

We have carried out calculations of electron transport through a metal-molecule-metal junction with metal nanoclusters taking the part of electrodes. We show that negative differential resistance peaks could appear in the current-voltage…

Materials Science · Physics 2008-10-22 Natalya A. Zimbovskaya , Mark R. Pederson

Negative differential resistivity (NDR) in a (3+1)-dimensional quantum system of strongly correlated charge carriers is theoretically reproduced by using the AdS/CFT correspondence. Our system is microscopically defined, and the analysis…

High Energy Physics - Theory · Physics 2011-09-19 Shin Nakamura

Current-controlled (also known as "S-type") negative differential resistance (NDR) is of crucial importance to many emerging applications including neuromorphic computing and high-density memristors integration. However, the experimental…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Miao Wang , Chengyu Wang , Chenchen Wu , Qiao Li , Chen Pan , Cong Wang , Shi-Jun Liang , Feng Miao

Both experiments and theoretical studies have demonstrated that the interaction between the current carrying electrons and the induced polarization charge in single-molecule junctions leads to a strong renormalization of molecular charging…

Mesoscale and Nanoscale Physics · Physics 2013-11-22 K. Kaasbjerg , K. Flensberg

We demonstrate, based on low-temperature scanning tunneling microscopy (STM) and spectroscopy, a pronounced negative differential resistance (NDR) in spin-crossover (SCO) molecular devices, where a Fe$^{\text{II}}$ SCO molecule is deposited…

We theoretically investigate negative differential resistance (NDR) of massless and massive Dirac Fermions in double barrier resonant tunneling diodes based on sufficiently short and wide graphene strips. The current-voltage characteristics…

Mesoscale and Nanoscale Physics · Physics 2013-03-12 Yu Song , Han-Chun Wu , Yong Guo

One of the ultimate goals of molecular electronics is to create technologies that will complement - and eventually supersede - Si-based microelectronics technologies. To reach this goal, electronic properties that mimic at least some of the…

Mesoscale and Nanoscale Physics · Physics 2015-06-26 Bingqian Xu , Yonatan Dubi

A negative differential resistance (NDR) in the nanotransport is often ascribed to electron correlations. We present a simple example which demonstrates that finite electrode bandwidths and energy dependent electrode density of states are…

Mesoscale and Nanoscale Physics · Physics 2010-05-12 Ioan Baldea , Horst Koppel

Reaction currents in chemical networks usually increase when increasing their driving affinities. But far from equilibrium the opposite can also happen. We find that such negative differential response (NDR) occurs in reaction schemes of…

Statistical Mechanics · Physics 2019-07-24 Gianmaria Falasco , Tommaso Cossetto , Emanuele Penocchio , Massimiliano Esposito
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