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We study the dynamics of optically-induced nuclear spin polarization in a fluorine-doped ZnSe epilayer via time-resolved Kerr rotation. The nuclear polarization in the vicinity of a fluorine donor is induced by interaction with coherently…

Mesoscale and Nanoscale Physics · Physics 2016-02-24 F. Heisterkamp , E. Kirstein , A. Greilich , E. A. Zhukov , T. Kazimierczuk , D. R. Yakovlev , A. Pawlis , M. Bayer

We employ optical pump-probe spectroscopy to investigate the voltage dependence of spontaneous electron and nuclear spin polarizations in hybrid MnAs/n-GaAs and Fe/n-GaAs Schottky diodes. Through the hyperfine interaction, nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. J. Epstein , J. Stephens , M. Hanson , Y. Chye , A. C. Gossard , P. M. Petroff , D. D. Awschalom

We theoretically study the dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. In our prior work [Phys. Rev. Lett. 104, 226807 (2010)] we identified three regimes of long-term dynamics,…

Mesoscale and Nanoscale Physics · Physics 2014-07-28 M. Gullans , J. J. Krich , J. M. Taylor , B. I. Halperin , M. D. Lukin

We demonstrate experimentally that a polarized nuclear spin modifies the dynamic behavior of a neighboring electronic spin. Specifically, an out-of-phase component appears in the electronic spin-echo signal. This component is proportional…

Quantum Physics · Physics 2016-01-20 Paz London , Ran Fischer , Ignacio Alvizu , Jeronimo R. Maze , David Gershoni

A pure spin current is predicted to occur when an external magnetic field and a linearly inhomogeneous spin-only field are appropriately aligned. Under these conditions (such as originate from nuclear contact hyperfine fields that do not…

Mesoscale and Nanoscale Physics · Physics 2022-09-14 Nicholas J. Harmon , Michael E. Flatté

We calculate nuclear-polarization energy shifts for hydrogenlike $^{208}_{~82}$Pb$^{81+}$. A retarded transverse part as well as the Coulomb part is taken into account as the electromagnetic interaction between an electron and the nucleus.…

Nuclear Theory · Physics 2009-11-07 Akihiro Haga , Yataro Horikawa , Yasutoshi Tanaka

Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

In a dynamic nuclear polarization experiment on a 40 mM solution of 4-amino-TEMPO in a 40:60 water/glycerol mixture, we have observed that the bulk dipolar reservoir is cooled to a spin temperature of 15.5 micro-K, following microwave…

Other Condensed Matter · Physics 2009-04-01 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

Dynamic nuclear polarization is widely used to enhance the sensitivity of nuclear magnetic resonance. It is presently the method of choice for enhancing the sensitivity of high-field solid state NMR experiments performed under cryogenic…

Chemical Physics · Physics 2022-02-02 Maria Grazia Concilio , Ilya Kuprov , Lucio Frydman

The nuclear polarization of $\mathrm{H}_2$ molecules formed by recombination of nuclear polarized H atoms on the surface of a storage cell initially coated with a silicon-based polymer has been measured by using the longitudinal double-spin…

Atomic Physics · Physics 2012-08-27 The HERMES collaboration

We discuss the implications of a small indium content (3%) in a GaAs epilayer on the electron- and nuclear-spin relaxation due to enhanced quadrupolar effects induced by the strain. Using the weakly perturbative spin-noise spectroscopy, we…

Mesoscale and Nanoscale Physics · Physics 2022-07-27 C. Rittmann , M. Yu. Petrov , A. N. Kamenskii , K. V. Kavokin , A. Yu. Kuntsevich , Yu. P. Efimov , S. A. Eliseev , M. Bayer , A. Greilich

The intensity and the giant circular polarization of edge luminescence in a longitudinal magnetic field have been measured in nitrogen alloys GaAsN under circularly polarized pumping. It has been found that these dependences are shifted…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 V. K. Kalevich , M. M. Afanasiev , A. Yu. Shiryaev , A. Yu. Egorov

Using a `standard' NMR spin-echo technique we determined the spin polarization of two-dimensional electrons, confined to GaAs quantum wells, from the hyperfine shift of Ga nuclei in the wells. Concentrating on the temperature and magnetic…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 S. Melinte , N. Freytag , M. Horvatic , C. Berthier , L. P. Levy , V. Bayot , M. Shayegan

A theoretical study of spin dynamics in non-relativistic particle beams with interacting angular momenta traversing static, spatially varying magnetic fields is presented. The computational framework evaluates sinusoidal magnetic field…

The nature of the nano-scale environment presents a major challenge for solid-state implementation of spin-based qubits. In this work, a single electron spin in an optically pumped nanometer-sized III-V semiconductor quantum dot is used to…

Nuclear spin polarization induced by hyperfine interaction and the Edelstein effect due to strong spin-orbit interaction is investigated by quantum transport in Bi(111) thin film samples. The Bi(111) films are deposited on mica by van der…

Mesoscale and Nanoscale Physics · Physics 2020-09-09 Zijian Jiang , Victoria Soghomonian , Jean J. Heremans

Enhancement of the electron spin polarization in a correlated two-layer two-dimensional electron system at a total Landau level filling factor of one is reported. Using resistively detected nuclear magnetic resonance, we demonstrate that…

Strongly Correlated Electrons · Physics 2015-04-30 L. Tiemann , W. Wegscheider , M. Hauser

Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots lead to nuclear spin polarization that is qualitatively different from the well known optical orientation phenomena. By carrying out a…

Mesoscale and Nanoscale Physics · Physics 2014-10-03 A. Högele , M. Kroner , C. Latta , M. Claassen , I. Carusotto , C. Bulutay , A. Imamoglu

We demonstrate that the dynamic nuclear polarization (DNP) of phosphorus donors in silicon can be very effective in a magnetic field of 4.6 T and at temperatures below 1 K. The DNP occurs due to the Overhauser effect following a cross…

Dynamic nuclear polarization (DNP) can increase nuclear magnetic resonance (NMR) signals by orders of magnitude. DNP in diamond proceeds through different DNP mechanisms with a possible temperature-dependence. We report on 13C dynamic…