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We study electron transport properties of some molecular wires and a unconventional disordered thin film within the tight-binding framework using Green's function technique. We show that electron transport is significantly affected by…

Mesoscale and Nanoscale Physics · Physics 2009-06-29 Santanu K. Maiti

Using first-principles methods we study theoretically the properties of an individual $\{Fe_4\}$ single-molecule magnet (SMM) attached to metallic leads in a single-electron transistor geometry. We show that the conductive leads do not…

Mesoscale and Nanoscale Physics · Physics 2014-07-01 J. F. Nossa , M. Fhokrul Islam , C. M. Canali , M. R. Pederson

One of the important issues of molecular spintronics is the control and manipulation of charge transport and, in particular, its spin polarization through single-molecule junctions. Using $ab$ $initio$ calculations, we explore…

Mesoscale and Nanoscale Physics · Physics 2019-09-04 Dongzhe Li , Yannick J. Dappe , Alexander Smogunov

The change of conductance of single molecule junctions in response to various external stimuli is the fundamental mechanism for single-molecule electronic devices with multiple functionalities. We propose a concept that the conductance of…

Mesoscale and Nanoscale Physics · Physics 2014-12-04 Chengbo Zhu , Xiaolin Wang

Here we describe the design, single-molecule transport measurements, and theoretical modeling of a ferrocene-based organometallic molecular wire, whose bias-dependent conductance shows a clear Lorentzian form with magnitude exceeding 70% of…

The effect of molecular vibrations on electronic transport is investigated with the smallest fullerene C20 bridge, utilizing the Keldysh nonequilibrium Green's function techniques combined with the tight-binding molecular-dynamics method.…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Takahiro Yamamoto , Kazuyuki Watanabe , Satoshi Watanabe

Molecules of bisthiolterthiophene have been adsorbed on the two facing gold electrodes of a mechanically controllable break junction in order to form metal-molecule(s)-metal junctions. Current-voltage (I-V) characteristics have been…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 C. Kergueris , J. -P. Bourgoin , S. Palacin , D. Esteve , C. Urbina , M. Magoga , C. Joachim

Impressive advances in nanoscience permit nowadays to manipulate single molecules and broadly control many of their properties. Still, tuning the molecular charge and vibrational properties of single molecules embedded in nanojunctions in…

Chemical Physics · Physics 2015-09-21 Ioan Baldea

We propose a tight-binding model to investigate electronic transport properties of single helical protein molecules incorporating both the helical symmetry and the possibility of multiple charge transfer pathways. Our study reveals that due…

Mesoscale and Nanoscale Physics · Physics 2016-06-10 Sourav Kundu , S. N. Karmakar

The quantum transport properties of the ultrathin silver nanowires are investigated. For a perfect crystalline nanowire with four atoms per unit cell, three conduction channels are found, corresponding to three $s$ bands crossing the Fermi…

Materials Science · Physics 2009-11-07 Jijun Zhao , Buia Calin , Jie Han , Jian Ping Lu

The effect of vibrational motion on resonant charge transport through single molecule junctions is investigated. The study is based on a combination of first-principles electronic structure calculations to characterize the system and…

Other Condensed Matter · Physics 2007-12-24 Claudia Benesch , Martin Cizek , Jiri Klimes , Michael Thoss , Wolfgang Domcke

We explore electron transport properties in a quantum wire attached to two metallic electrodes. A simple tight-binding model is used to describe the system and the coupling of the wire to the electrodes (source and drain) is treated through…

Mesoscale and Nanoscale Physics · Physics 2010-01-10 Santanu K. Maiti

We report the electronic transport properties of a new photo-addressable molecular switch. The switching process relies on a new concept based on linear {\pi}-conjugated dynamic systems, in which the geometry and hence the electronic…

Mesoscale and Nanoscale Physics · Physics 2017-06-13 S. Lenfant , Y. Viero , C. Krzeminski , D. Vuillaume , D. Demeter , I. Dobra , M. Ocafrain , P. Blanchard , J. Roncali , C. van Dyck , J. Cornil

We investigate charge transport in C$_{60}$-based single-molecule junctions with graphene electrodes employing a combination of density functional theory (DFT) electronic structure calculations and Landauer transport theory. In particular,…

Mesoscale and Nanoscale Physics · Physics 2017-01-12 Susanne Leitherer , Pedro B. Coto , Konrad Ullmann , Heiko B. Weber , Michael Thoss

We consider electronic transport through laterally parallel double open quantum dots embedded in a quantum wire in a perpendicular magnetic field. The coupling modes of the dots are tunable by adjusting the strength of a central barrier and…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Chi-Shung Tang , Wing Wa Yu , Vidar Gudmundsson

We present a theoretical study of spin-dependent transport through molecular wires bridging ferromagnetic metal nanocontacts. We extend to magnetic systems a recently proposed model that provides a em quantitative explanation of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Eldon Emberly , George Kirczenow

We report two examples of transport phenomena based on sharp features in the effective density of states of molecular-scale transistors: Kondo physics in C$_{60}$-based devices, and gate-modulated negative differential resistance (NDR) in…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 L. H. Yu , D. Natelson

By means of electronic transport, we study the transverse magnetic anisotropy of an individual Fe$_4$ single-molecule magnet (SMM) embedded in a three-terminal junction. In particular, we determine in situ the transverse anisotropy of the…

Mesoscale and Nanoscale Physics · Physics 2016-08-10 M. Misiorny , E. Burzurí , R. Gaudenzi , K. Park , M. Leijnse , M. R. Wegewijs , J. Paaske , A. Cornia , H. S. J. van der Zant

This tutorial article gives an introduction to the methods needed to treat interacting electrons in a quantum wire with a single occupied band. Since one-dimensional Fermions cannot be described in terms of noninteracting quasiparticles,…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Hermann Grabert

We investigate coherent control of single particles held in a bipartite optical lattice via a combined high-frequency modulation. Our analytical results show that for the photon resonance case the quantum tunneling and dynamical…

Quantum Physics · Physics 2015-06-16 Kuo Hai , Yunrong Luo , Gengbiao Lu , Wenhua Hai