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We study the influence of chain stiffness on droplet flow in a nano-channel, coated with semiflexible hydrophobic polymers by means of non-equilibrium molecular-dynamics simulations. The studied system is then a moving droplet in the slit…

Soft Condensed Matter · Physics 2017-10-18 Kevin Speyer , Claudio Pastorino

Semiflexible polymers in concentrated lyotropic solution are studied within a bead-spring model by molecular dynamics simulations, focusing on the emergence of a smectic A phase and its properties. We systematically vary the density of the…

Soft Condensed Matter · Physics 2019-01-28 Andrey Milchev , Arash Nikoubashman , Kurt Binder

Phase separation within polymer networks plays a central role in shaping the structure and mechanics of both synthetic materials and living cells, including the formation of biomolecular condensates within cytoskeletal networks. Previous…

Soft Condensed Matter · Physics 2025-12-01 Takahiro Yokoyama , Yicheng Qiang , David Zwicker , Arash Nikoubashman

Polymer brushes are increasingly used to tailor surface physicochemistry for various applications such as wetting, adhesion of biological objects, implantable devices, etc. We perform Dissipative Particle Dynamics simulations to study the…

Soft Condensed Matter · Physics 2015-10-01 Sofia Biagi , Lorenzo Rovigatti , Francesco Sciortino , Chaouqi Misbah

The non-linear response of entangled polymers to shear flow is complicated. Its current understanding is framed mainly as a rheological description in terms of the complex viscosity. However, the full picture requires an assessment of the…

Computational Physics · Physics 2018-08-21 Airidas Korolkovas , Philipp Gutfreund , Max Wolff

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

Soft Condensed Matter · Physics 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

We use molecular dynamics simulations to study a semidilute, unentangled polymer solution containing well dispersed, weakly attractive nanoparticles (NP) of size ($\sigma_N$) smaller than the polymer radius of gyration $R_g$. We find that…

Soft Condensed Matter · Physics 2018-09-18 Valerio Sorichetti , Virginie Hugouvieux , Walter Kob

We examine the phase transition of polymer adsorption as well as the underlying kinetics of polymer binding from dilute solutions on a structureless solid surface. The emphasis is put on the properties of regular multiblock copolymers,…

Soft Condensed Matter · Physics 2009-09-03 A. Milchev , V. Rostiashvili , S. Bhattacharya , T. Vilgis

We experimentally and theoretically consider highly condensed planar brushes made of charged polymers. Using x-ray reflectivity on polyelectrolytes which are anchored at the water-air interface, it is shown that such strongly stretched…

We propose a new model for the description of complex granular particles and their interaction in molecular dynamics simulations of granular material in two dimensions. The grains are composed of triangles which are connected by deformable…

Materials Science · Physics 2007-05-23 Thorsten Poeschel , Volkhard Buchholtz

The dynamics of structural relaxation in a model polymer glass subject to spatially-homogeneous, time-periodic shear deformation is investigated using molecular dynamics simulations. We study a coarse-grained bead-spring model of short…

Soft Condensed Matter · Physics 2014-01-10 Nikolai V. Priezjev

Using molecular simulations, we study the properties of a polymer brush in contact with an explicit solvent under Couette and Poiseuille flow. The solvent is comprised of chemically identical chains. We present evidence that individual,…

Soft Condensed Matter · Physics 2009-11-13 M. Müller , C. Pastorino

We present molecular dynamics study of a generic (coarse-grained) model for single-polymer diffusion confined in a corrugated cylinder. For a narrow tube, i.e., diameter of the cylinder $\delta < 2.3$, the axial diffusion coefficient…

Soft Condensed Matter · Physics 2015-06-11 A. De Virgiliis , L. Kuban , J. Paturej , D. Mukherji

We study the relaxation dynamics of a coarse-grained polymer chain at different degrees of stretching by both analytical means and numerical simulations. The macromolecule is modelled as a string of beads, connected by anharmonic springs,…

Soft Condensed Matter · Physics 2009-11-13 M. Febbo , A. Milchev , V. Rostiashvili , T. A. Vilgis , D. Dimitrov

The adsorption of a bottle-brush polymer end-grafted with one chain end of its backbone to a flat substrate surface is studied by Monte Carlo simulation of a coarse-grained model, that previously has been characterized in the bulk, assuming…

Soft Condensed Matter · Physics 2010-10-13 Hsiao-Ping Hsu , Wolfgang Paul , Kurt Binder

We analyze the structural behavior of a single polymer chain grafted to an attractive, flexible surface. Our model is composed of a coarse-grained bead-and-spring polymer and a tethered membrane. By means of extensive parallel tempering…

Soft Condensed Matter · Physics 2011-09-26 Steffen Karalus , Wolfhard Janke , Michael Bachmann

When a liquid drop spreads on an adaptive substrate the latter changes its properties what may result in an intricate coupled dynamics of drop and substrate. Here we present a generic mesoscale hydrodynamic model for such processes that is…

Fluid Dynamics · Physics 2020-10-28 Uwe Thiele , Simon Hartmann

The adhesion between a polymer melt and substrate is studied in the presence of chemically attached chains on the substrate surface. Extensive molecular dynamics simulations have been carried out to study the effect of temperature, tethered…

Materials Science · Physics 2016-08-31 Scott W. Sides , Gary S. Grest , Mark J. Stevens

We investigate polyelectrolyte brushes in the osmotic regime using both theoretical analysis and molecular dynamics simulation techniques. In the simulations at moderate Bjerrum length, we observe that the brush height varies weakly with…

Soft Condensed Matter · Physics 2007-05-23 Ali Naji , Roland R. Netz , Christian Seidel

Continuum Monte-Carlo simulations at constant pressure are performed on short chain molecules at surfaces. The rodlike chains, consisting of seven effective monomers, are attached at one end to a flat twodimensional substrate. It is found…

Condensed Matter · Physics 2007-05-23 R. Hilfer , F. M. Haas