Related papers: Non-linear response of single-molecule magnets: fi…
We present an experimental study of the {\em nonlinear} susceptibility of Mn$_{12}$ single-molecule magnets. We investigate both their thermal-equilibrium and dynamical nonlinear responses. The equilibrium results show the sensitivity of…
The nonlinear dynamical response of Mn$_{12}$ single-molecule magnets is experimentally found to be very large, quite insensitive to the spin-lattice coupling constant, and displaying peaks reversed with respect to classical…
The spin relaxation in the molecular magnet \Mn12 is investigated by a novel type of high-frequency magnetic spectroscopy. By reversing the external magnetic field the intensities of the $|\pm 10>\to |\pm 9>$ transitions within the ground…
We calculate the magnetisation relaxation in the short-time regime for an ensemble of nanomagnets in the presence of a low-frequency external AC biasing field, at temperatures lower than the magnetic anisotropy energy of the individual…
The magnetic relaxation and hysteresis of a system of single domain particles with dipolar interactions are studied by Monte Carlo simulations. We model the system by a chain of Heisenberg classical spins with randomly oriented easy-axis…
We have studied numerically the quantum-classical crossover in the escape-rate for an uniaxial spin system with an arbitrarily directed field. Using the simple quantum transition-state theory, we have obtained the boundary separating the…
Monte Carlo simulations are used to study the magnetic relaxation of a system of single domain particles with dipolar interactions modeled by a chain of Heisenberg classical spins. We show that the so-called $T\ln(t/\tau_0)$ method can be…
With decreasing particle size, different mechanisms dominate the thermally activated magnetization reversal in ferromagnetic particles. We investigate some of these mechanisms for the case of elongated, single-domain nanoparticles which we…
In a recent paper, cond-mat/0404041, J. Vanacken et al. reported experimental studies of crystals of Mn12-ac molecular nanomagnets in pulsed magnetic fields with sweep rates up to 4000 T/s. Steps in the magnetization curve were observed.…
We argue that to explain recent resonant tunneling experiments on crystals of Mn$_{12}$ and Fe$_8$, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-$T$, short-time relaxation…
Magnetization measurements of a truly axial symmetry Mn12-tBuAc molecular nanomagnet with a spin ground state of S = 10 show resonance tunneling. This compound has the same magnetic anisotropy as Mn12-Ac but the molecules are better…
Recent progress in experiment on quantum tunnelling of the magnetic moment in mesoscopic systems will be reviewed. The emphasis will be made on measurements of individual nanoparticles. These nanomagnets allow one to test the border between…
A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…
Nonexponential relaxation of magnetization at resonant tunneling points of nanoscale molecular magnets is interpreted to be an effect of fluctuating random field around the applied field. We demonstrate such relaxation in Langevin equation…
We study nonlinear response in quantum spin systems {near infinite-randomness critical points}. Nonlinear dynamical probes, such as two-dimensional (2D) coherent spectroscopy, can diagnose the nearly localized character of excitations in…
How nanoscale uniaxial magnets respond to an alternating field is studied by direct numerical calculation. A nontrivial oscillation of the magnetization is found, which is analyzed in terms of the non-adiabatic transition due to the time…
High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…
The relaxation mechanisms of a quantum nanomagnet are discussed in the frame of linear response theory. We use a spin Hamiltonian with a uniaxial potential barrier plus a Zeeman term. The spin, having arbitrary $S$, is coupled to a bosonic…
The crossover between thermally assisted and pure quantum tunneling has been studied in single crystals of high spin (S=10) uniaxial molecular magnet Mn12 using micro-Hall-effect magnetometry. Magnetic hysteresis and relaxation experiments…
A quantum Heisenberg model with anisotropic coupling and all-to-all interaction has been analyzed using the Bose-Einstein statistics. In Ref.\cite{jsp} the existence of a classical energy disconnection border (EDB) in the same kind of…