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Transport through molecular devices with strong coupling to a single vibrational mode is considered in the case where the vibration is damped by coupling to the environment. We focus on the weak tunneling limit, for which a rate equation…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Stephan Braig , Karsten Flensberg

The voltage dependence of nanoelectromechanical effects in a system where the quantized mechanical vibrations of a quantum dot are coupled to coherent tunneling of electrons through a single level in the dot is studied. It is found that…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 D. Fedorets

We employ the time-dependent non-crossing approximation to investigate the joint effect of strong electron-electron and electron-phonon interaction on the instantaneous conductance of a single molecule transistor which is abruply moved into…

Strongly Correlated Electrons · Physics 2010-10-19 Ali Goker

The electron transport in a 1D conductor with an isolated local defect such as an impurity or a non-adiabatic contact is studied theoretically. New regime of conduction in correlated 1D systems is predicted beyond the well-known regime of…

Strongly Correlated Electrons · Physics 2015-10-01 S. N. Artemenko , P. P. Aseev , D. S. Shapiro , R. R. Vakhitov

The symmetry properties of transport beyond the linear regime in chaotic quantum dots are investigated experimentally. A component of differential conductance that is antisymmetric in both applied source-drain bias V and magnetic field B,…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 D. M. Zumbuhl , C. M. Marcus , M. P. Hanson , A. C. Gossard

We propose a mechanism which allows one to control the transmission of single electrons through a molecular junction. The principle utilizes the emergence of transmission sidebands when molecular vibrational modes are coupled to the…

Mesoscale and Nanoscale Physics · Physics 2010-03-26 Thomas Olsen , Jakob Schiøtz

We theoretically analyze correlation effects on the transport properties of a benzene molecule that are mediated by interactions between the motion of the nuclei and the transmitted charge. We focus on the lowest-lying molecular vibrational…

Mesoscale and Nanoscale Physics · Physics 2013-08-09 Michael Knap , Enrico Arrigoni , Wolfgang von der Linden

The description of spontaneous symmetry breaking that underlies the connection between classically ordered objects in the thermodynamic limit and their individual quantum mechanical building blocks is one of the cornerstones of modern…

Other Condensed Matter · Physics 2010-04-29 Jasper van Wezel

We describe single electron tunneling through molecular structures under the influence of nano-mechanical excitations. We develop a full quantum mechanical model, which includes charging effects and dissipation, and apply it to the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Daniel Boese , Herbert Schoeller

We present an atomistic theory of electronic transport through single organic molecules that reproduces the important features of the current-voltage characteristics observed in recent experiments. We trace these features to their origin in…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Heurich , J. C. Cuevas , W. Wenzel , G. Schoen

Single-molecule electronics has been envisioned as the ultimate goal in the miniaturisation of electronic circuits. While the aim of incorporating single-molecule junctions into modern technology still proves elusive, recent developments in…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

We investigate how vibration affects molecular photoemission dynamics, through simulations on two-dimension asymmetric model molecules including the electronic and nuclear motions in a fully correlated way. We show that a slight anisotropy…

Chemical Physics · Physics 2024-02-14 Antoine Desrier , Morgan Berkane , Camille Lévêque , Richard Taïeb , Jérémie Caillat

Electron-hole pairs in organic photovoltaics dissociate efficiently despite their Coulomb-binding energy exceeding thermal energy at room temperature. The electronic states involved in charge separation couple to structured vibrational…

Mesoscale and Nanoscale Physics · Physics 2023-08-15 Alejandro D. Somoza , Nicola Lorenzoni , James Lim , Susana F. Huelga , Martin B. Plenio

Understanding how the mechanism of charge transport through molecular tunnel junctions depends on temperature is crucial to control electronic function in molecular electronic devices. With just a few systems investigated as a function of…

Mesoscale and Nanoscale Physics · Physics 2016-05-27 Alvar R. Garrigues , Lejia Wang , Enrique del Barco , Christian A. Nijhuis

Spontaneous breaking of continuous time translation symmetry into a discrete one is related to time crystal formation. While the phenomenon is not possible in the ground state of a time-independent many-body system, it can occur in an…

Quantum Gases · Physics 2018-08-21 Arkadiusz Kosior , Andrzej Syrwid , Krzysztof Sacha

We report on dynamical quantum transport simulations for realistic molecular devices based on an approximate formulation of time-dependent Density Functional Theory with open boundary conditions. The method allows for the computation of…

Mesoscale and Nanoscale Physics · Physics 2013-09-16 Christian Oppenländer , Björn Korff , Thomas A. Niehaus

We investigate the non-equilibrium transport properties of a disordered molecular nanowire. The nanowire is regarded as a quasi-one-dimensional organic crystal composed of self-assembled molecules. One orbital and a single random energy are…

Mesoscale and Nanoscale Physics · Physics 2017-06-07 P. Thiessen , E. Diaz , R. A. Roemer , F. Dominguez-Adame

We calculate the zero temperature conductance and characteristic correlation functions of a molecule with a center of mass (CM) motion which modulates couplings to the leads. In the first model studied, the CM vibrational mode is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Mravlje , A. Ramsak , T. Rejec

We discuss general properties of discrete time quantum symmetry breaking in degenerate parametric oscillators. Recent experiments in superconducting quantum circuit with Josephson junction nonlinearities give rise to new properties of…

Quantum Physics · Physics 2019-09-20 Feng-Xiao Sun , Qiongyi He , Qihuang Gong , Run Yan Teh , Margaret D. Reid , Peter D. Drummond

Tunnel transport of interacting spin-polarized electrons through a single-level vibrating quantum dot in external magnetic field is studied. By using density matrix method, the current-voltage characteristics and the dependence of…

Mesoscale and Nanoscale Physics · Physics 2021-03-23 A. D. Shkop , O. M. Bahrova , S. I. Kulinich , I. V. Krive
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