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The crystallographic and magnetic phase diagram of the n=2 layered manganite La2-2xSr1+2xMn2O7 in the region x=>0.5 has been studied using temperature dependent neutron powder diffraction. The magnetic phase diagram reveals a progression of…

Materials Science · Physics 2009-10-31 C. D. Ling , J. E. Millburn , J. F. Mitchell , D. N. Argyriou J. Linton , H. N. Bordallo

It is argued that both transitions observed in 50%-doped manganites, at the N\'{e}el temperature ($T_{\rm N}$) and the so-called charge ordering temperature ($T_{\rm CO}$), are magnetic. $T_{\rm N}$ corresponds to the order-disorder…

Strongly Correlated Electrons · Physics 2007-05-23 I. V. Solovyev

The magnetic phase diagram of the colossal magnetoresistance (CMR) manganites is determined based on the Hamiltonian incorporating the double-exchange (DE) interaction between degenerate Mn $e_g$ orbitals and the antiferromagnetic (AF)…

Strongly Correlated Electrons · Physics 2009-11-07 Unjong Yu , Yookyung Jo , B. I. Min

Correlation between orbital structure and magnetic ordering in bilayered manganites is examined. A level separation between the $3d_{3z^2-r^2}$ and $3d_{x^2-y^2}$ orbitals in a Mn ion is calculated in the ionic model for a large number of…

Strongly Correlated Electrons · Physics 2009-10-31 S. Okamoto , S. Ishihara , S. Maekawa

We study theoretically the phase diagram of the double-layered perovskite manganites taking into account the orbital degeneracy, the strong Coulombic repulsion, and the coupling with the lattice deformation. Observed spin structural changes…

Strongly Correlated Electrons · Physics 2009-10-31 Ryo Maezono , Naoto Nagaosa

The mechanisms of magnetic and orbital interactions due to double exchange (DE) and superexchange (SE) in transition metal oxides with degenerate e_g orbitals are presented. Specifically, we study the effective spin-orbital models derived…

Strongly Correlated Electrons · Physics 2009-10-31 A. M. Oles , M. Cuoco , N. B. Perkins

A series of manganites Tb1-xHoxMnO3 (0<=x<=0.6) with orthorhombic structure are synthesized and detailed investigations on their multiferroicity are performed. Successive magnetic transitions upon temperature variation are evidenced for all…

Strongly Correlated Electrons · Physics 2010-04-19 C. L. Lu , S. Dong , K. F. Wang , J. -M. Liu

Motivated by recent experiments, we present a comprehensive theoretical study of the geometrically frustrated strongly correlated magnetic insulator Mn$_3$O$_4$ spinel oxide based on a microscopic Hamiltonian involving lattice, spin and…

Strongly Correlated Electrons · Physics 2017-08-23 Santanu Pal , Siddhartha Lal

We investigate the high temperature phase of layered manganites, and demonstrate that the charge-orbital phase transition without magnetic order in La$_{0.5}$Sr$_{1.5}$MnO$_4$ can be understood in terms of the density wave instability. The…

Strongly Correlated Electrons · Physics 2013-04-17 Zi-Jian Yao , Wei-Qiang Chen , Jin-Hua Gao , Hong-Min Jiang , Fu-Chun Zhang

A lightly doped perovskite mangantite La_{0.88}Sr_{0.12}MnO_3 exhibits a phase transition at T_{OO}=145 K from a ferromagnetic metal (T_C=172 K) to a novel ferromagnetic insulator.We identify that the key parameter in the transition is the…

Strongly Correlated Electrons · Physics 2019-08-17 Y. Endoh , K. Hirota , S. Ishihara , S. Okamoto , Y. Murakami , A. Nishizawa , T. Fukuda , H. Kimura , H. Nojiri , K. Kaneko , S. Maekawa

Correlation-induced spin-charge and spin-orbital coupling effects on spin dynamics in ferromagnetic manganites are calculated with realistic parameters in order to provide a quantitative comparison with experimental results for spin…

Strongly Correlated Electrons · Physics 2015-05-18 Dheeraj Kumar Singh , Bhaskar Kamble , Avinash Singh

The optical conductivity of the undoped PrMnO$_3$ manganite has been investigated in details at various temperatures between 300 and 4 K. Its low energy spectrum exhibits an optical gap, and is characterized by a single broad peak centered…

Strongly Correlated Electrons · Physics 2007-05-23 R. Sopracase , G. Gruener , C. Autret-Lambert , V. Ta Phuoc , V. Brize , J. C. Soret

In strongly correlated electronic systems, such as manganites, the global transport behavior depends sensitively on the spin ordering, whose alteration often requires a large external magnetic field. Here we show that the spin ordering in…

Strongly Correlated Electrons · Physics 2014-07-01 T. Z. Ward , Z. Gai , X. Y. Xu , H. W. Guo , L. F. Yin , J. Shen

We analyze the role of orbital degeneracy in possible magnetic and orbital instabilities by solving exactly a two-site molecule with two orbitals of either $e_g$ or $t_{2g}$ symmetry at quarter-filling. As a generic feature of both models…

Strongly Correlated Electrons · Physics 2007-05-23 Marcin Raczkowski , Raymond Fresard , Andrzej M. Oles

Photo-excitation in complex oxides1 transfers charge across semicovalent bonds, drastically perturbing spin and orbital orders2. Light may then be used in compounds like magnetoresistive manganites to control magnetism on nanometre…

We review some aspects related to orbital degrees of freedom in manganites. The Mn$^{3+}$ ions in these compounds have double orbital degeneracy and are strong Jahn-Teller ions, causing structural distortions and orbital ordering. We…

Strongly Correlated Electrons · Physics 2007-05-23 Jeroen van den Brink , Giniyat Khaliullin , Daniel Khomskii

We study the effects of temperature and magnetic field on a two-orbital Hubbard model within dynamical mean field theory. We focus on the quarter filled system, which is a special point in the phase diagram due to orbital degeneracy. At…

Strongly Correlated Electrons · Physics 2011-03-29 Robert Peters , Norio Kawakami , Thomas Pruschke

The competition of charge, orbital, and ferromagnetic interactions in layered manganites is investigated by magneto-Raman scattering spectroscopy. We find that the colossal magnetoresistance effect in the layered compounds results from the…

Strongly Correlated Electrons · Physics 2009-10-31 D. B. Romero , Y. Moritomo , J. F. Mitchell , H. D. Drew

Basic mechanisms controlling orbital order and orbital fluctuations in transition metal oxides are discussed. The lattice driven classical orbital picture, e.g. like in manganites LaMnO$_3$, is contrasted to the quantum behavior of orbitals…

Strongly Correlated Electrons · Physics 2009-11-11 Giniyat Khaliullin

We derive a spin-orbital model for insulating LaMnO_3 which fulfills the SU(2) symmetry of S=2 spins at Mn^{3+} ions. It includes the complete e_g and t_{2g} superexchange which follows from a realistic Mn^{2+} multiplet structure in cubic…

Strongly Correlated Electrons · Physics 2009-10-31 Louis Felix Feiner , Andrzej M. Oles