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We study the diffusion-driven kinetics of phase separation of a symmetric binary mixture (AB), confined in a thin-film geometry between two parallel walls. We consider cases where (a) both walls preferentially attract the same component…

Soft Condensed Matter · Physics 2009-11-11 Subir K. Das , Sanjay Puri , Juergen Horbach , Kurt Binder

Inspired by recent experiments, we present a phase-field model of microphase separation in an elastomer swollen with a solvent. The imbalance between the molecular scale of demixing and the mesoscopic scale beyond which elasticity operates…

Soft Condensed Matter · Physics 2025-09-05 Manu Mannattil , Haim Diamant , David Andelman

Superconducting properties of thin films can be vastly different from those of bulk materials. Seminal work has shown the critical temperature Tc of elemental superconductors decreases with decreasing film thickness when the normal-state…

We report results of density-functional theory calculations on the structural, magnetic, and electronic properties of (1x1)-structures of Co on Cu(001) for coverages up to two monolayers. In particular we discuss the tendency towards phase…

Materials Science · Physics 2009-10-31 R. Pentcheva , M. Scheffler

The interfacial profile between coexisting phases of a binary mixture (A,B) in a thin film of thickness D and lateral linear dimensions L depends sensitively on both linear dimensions and on the nature of boundary conditions and statistical…

Statistical Mechanics · Physics 2009-10-30 Andreas Werner , Friederike Schmid , Marcus Mueller , Kurt Binder

In this paper the evolution of a binary mixture in a thin-film geometry with a wall at the top and bottom is considered. By bringing the mixture into its miscibility gap so that no spinodal decomposition occurs in the bulk, a slight…

Dimension-reduction homogenization results for thin films have been obtained under hypotheses of periodicity or almost-periodicity of the energies in the directions of the mid-plane of the film. In this note we consider thin films, obtained…

Analysis of PDEs · Mathematics 2022-12-22 Irene Anello , Andrea Braides , Fabrizio Caragiulo

We report molecular dynamics simulation results on the equilibrium properties of polymer thin films adsorbed onto flat and curved substrates. We first systematically determine the contact angle of polymer droplets on flat substrates as a…

Soft Condensed Matter · Physics 2023-12-15 Gabriel Catalini , Nicolás A. García , Daniel A. Vega , Arash Nikoubashman

The glass transition temperature and its connection to statistical properties of confined and free-standing polymer films of varying thickness containing unentangled to highly entangled bead-spring chains are studied by molecular dynamics…

Soft Condensed Matter · Physics 2023-09-21 Hsiao-Ping Hsu , Kurt Kremer

We investigate the segregation pattern formations of strongly and weakly fluctuated Brownian particle mixtures, which are confined in spherical containers with finite volumes. We consider systems where the container restricts the motions of…

Soft Condensed Matter · Physics 2015-06-19 Akinori Awazu

Microphase separated structure consisting of the periodic alternation of the layers of stretched homopolymer chains surrounded by perpendicularly oriented oligomeric tails is studied for both, strongly bonded (ionic) systems and weakly…

Statistical Mechanics · Physics 2007-05-23 A. Olemskoi , I. Krakovsky , A. Savelyev

Conformational properties of polymer melts confined between two hard structureless walls are investigated by Monte Carlo simulation of the bond-fluctuation model. Parallel and perpendicular components of chain extension, bond-bond…

Soft Condensed Matter · Physics 2009-11-10 A. Cavallo , M. Müller , J. P. Wittmer , A. Johner , K. Binder

We enumerate all minimal energy packings (MEPs) for small single linear and ring polymers composed of spherical monomers with contact attractions and hard-core repulsions, and compare them to corresponding results for monomer packings. We…

Soft Condensed Matter · Physics 2015-05-18 Robert S. Hoy , Corey S. O'Hern

Monte Carlo simulations in the grand canonical ensemble were used to obtain critical parameters and conditions leading to microphase separation for block copolymers with solvophilic and solvophobic segments. Solvent selectivity was…

Soft Condensed Matter · Physics 2024-09-13 Athanassios Z. Panagiotopoulos

We study the interplay between wetting and miscibility of a symmetric polymer mixture via MC simulations and SCF calculations. The film surfaces interact with the monomers via short ranged potentials and the wetting transition is of first…

Soft Condensed Matter · Physics 2007-05-23 Marcus Mueller , Kurt Binder

The phase behaviour of blends of ABC triblock and ac diblock copolymers is examined using self-consistent field theory. Several equilibrium lamellar structures are observed, depending on the volume fraction of the diblocks, phi_2, the…

Soft Condensed Matter · Physics 2009-11-07 Robert A. Wickham , An-Chang Shi

In the present work, we study morphologies arising due to competing substrate interaction, electric field and confinement effects on a symmetric diblock copolymer. We employ a coarse grained non-local Cahn-Hilliard phenomenological model…

Materials Science · Physics 2016-04-06 Arnab Mukherjee , Rajdip Mukherjee , Kumar Ankit , Avisor Bhattacharya , Britta Nestler

Stationary phase plays a crucial role in the operation of a protein chromatography column. Conventional resins composed of acrylic polymers and their derivatives contribute to heterogeneity of the packing of stationary phase inside these…

Soft Condensed Matter · Physics 2023-11-14 Raghu K. Moorthy , Serena D'Souza , P. Sunthar , Santosh B. Noronha

We consider here a blend made of two types of polymers, $A$ and $B$, of different chemical nature. At high temperature the homogeneous mixture is cross-linked. As the temperature is lowered, the two species try to segregate but are kept…

Condensed Matter · Physics 2015-06-25 Edilson Vargas , Marcia C. Barbosa

We analyze a (1+1)-dimension directed random walk model of a polymer dipped in a medium constituted by two immiscible solvents separated by a flat interface. The polymer chain is heterogeneous in the sense that a single monomer may…

Probability · Mathematics 2007-05-23 Erwin Bolthausen , Giambattista Giacomin