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Nanoscale polymeric thin films are widely used in diverse applications such as energy devices, flexible electronics and biosensors, where a satisfactory mechanical performance is of vital importance to realize their full functionality. It…

Soft Condensed Matter · Physics 2022-06-29 Zhengyang Zhang , Pei Bai , Yuhan Xiao , Yunlong Guo , Yanming Wang

We use molecular dynamics simulations to study the static properties of a single linear multiblock copolymer chain under poor solvent conditions varying the block length $N$, the number of blocks $n$, and the solvent quality by variation of…

Soft Condensed Matter · Physics 2015-03-19 N. G. Fytas , P. E. Theodorakis

We present a long-wavelength approximation to the Navier-Stokes Cahn-Hilliard equations to describe phase separation in thin films. The equations we derive underscore the coupled behaviour of free-surface variations and phase separation. We…

Soft Condensed Matter · Physics 2015-05-14 Lennon O Naraigh , Jean-Luc Thiffeault

We study random copolymers consisted of two kinds of monomers with attraction between similar kinds. The mean field analysis of this system indicates a continuous phase transition into a phase with periodic microdomain structure. It is…

Condensed Matter · Physics 2009-10-22 A. M. Gutin , C. D. Sfatos , E. I. Shakhnovich

We investigate the ordered morphologies occurring in thin-films diblock copolymer. For temperatures above the order-disorder transition and for an arbitrary two-dimensional surface pattern, we use a Ginzburg-Landau expansion of the free…

Soft Condensed Matter · Physics 2007-05-23 Yoav Tsori , David Andelman

The phase behavior of linear dendritic triblock copolymer melts(AB2C4) is studied by self-consistent-field theory (SCFT) in order to find the effects of branching on the phase behavior of ABC linear triblock copolymer melts. We focus on a…

Soft Condensed Matter · Physics 2023-09-19 Danyang Chen , Xiaowei Ning

The derivation of density functional energies from the random phase approximation of self-consistent mean field theory is generalized and applied to a binary blend of diblock copolymers and homopolymers. A nonlocal transformation is…

Soft Condensed Matter · Physics 2023-07-04 Sulin Wang , Yuan Chen , Zengqiang Tan , Keith Promislow

Two ring polymers close to each other in space may be either in a segregated phase if there is a strong repulsion between monomers in the polymers, or intermingle in a mixed phase if there is a strong attractive force between the monomers.…

Soft Condensed Matter · Physics 2022-11-23 EJ Janse van Rensburg , E Orlandini , MC Tesi , SG Whittington

Formation of the intermediate phase patterns in the thin-film co-deposition process is simulated using the Stochastic Kinetic Mean-Field method and Monte Carlo. Three basic morphologies of the 2D sections are distinguished: (1) spots…

Materials Science · Physics 2024-12-05 Serhii Abakumov , Andriy Gusak

When systems that can undergo phase separation between two coexisting phases in the bulk are confined in thin film geometry between parallel walls, the phase behavior can be profoundly modified. These phenomena shall be described and…

Soft Condensed Matter · Physics 2008-04-17 Kurt Binder , Juergen Horbach , Richard Vink , Andres De Virgiliis

We examine the structural and dynamic properties of confined binary hard-sphere mixtures designed to mimic realizable colloidal thin films. Using computer simulations, governed by either Newtonian or overdamped Langevin dynamics, together…

Soft Condensed Matter · Physics 2015-05-01 Jonathan A. Bollinger , Avni Jain , James Carmer , Thomas M. Truskett

Artificial antiferromagnets and synthetic metamagnets have attracted much attention recently due to their potential for many different applications. Under some simplifying assumptions these systems can be modeled by thin Ising metamagnetic…

Statistical Mechanics · Physics 2011-10-18 Yen-Liang Chou , Michel Pleimling

We examine the phase transition of polymer adsorption as well as the underlying kinetics of polymer binding from dilute solutions on a structureless solid surface. The emphasis is put on the properties of regular multiblock copolymers,…

Soft Condensed Matter · Physics 2009-09-03 A. Milchev , V. Rostiashvili , S. Bhattacharya , T. Vilgis

A mean field rate theory description of the homo- and co-polymerization of $f$-functional molecules is developed, which contains the formation of short cyclic structures inside the network. The predictions of this model are compared with…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang , Konrad Schwenke , Jens-Uwe Sommer

Homogeneous face-centered cubic (fcc) polycrystalline CoCrFeNi films were deposited at room temperature on (0001)alpha-Al2O3 (c-sapphire). Phase and morphological stability of 200 to 670 nm thick films were investigated between 973 K and…

Block copolymer melts self-assemble in the bulk into a variety of nanostructures, making them perfect candidates to template the position of nanoparticles. The morphological changes of block copolymers are studied in the presence of a…

Soft Condensed Matter · Physics 2019-10-31 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga

Experiments of particle-laden inclined film flow [Zhou, Dupuy, Bertozzi, and Hosoi, Phys. Rev. Lett. 94 (2005)] have displayed different settling behaviors depending on the particle concentration $\phi$ and angle of inclination $\theta$, in…

Fluid Dynamics · Physics 2009-11-13 Benjamin P. Cook

A phase-field description of brittle fracture is employed in the reported four-point bending analyses of monolithic and laminated glass plates. Our aims are: (i) to compare different phase-field fracture formulations applied to thin glass…

Computational Engineering, Finance, and Science · Computer Science 2020-12-30 Jaroslav Schmidt , Alena Zemanová , Jan Zeman , Michal Šejnoha

We apply self consistent field theory to twist grain boundaries of block copolymer melts. The distribution of monomers throughout the grain boundary is obtained as well as the grain boundary free energy per unit area as a function of twist…

Soft Condensed Matter · Physics 2009-10-31 Daniel Duque , Michael Schick

We study the effects of chirality at the segment scale on the thermodynamics of block copolymer melts using self consistent field theory. In linear diblock melts where segments of one block prefer a twisted, or cholesteric, texture, we show…

Soft Condensed Matter · Physics 2015-06-11 Wei Zhao , Thomas P. Russell , Gregory M. Grason
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