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High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

Several rare earth magnetic pyrochlore materials are well modeled by a spin-1/2 quantum Hamiltonian with anisotropic exchange parameters Js. For the Er2Ti2O7 material, the Js were recently determined from high-field inelastic neutron…

Strongly Correlated Electrons · Physics 2014-04-11 J. Oitmaa , R. R. P. Singh , A. G. R. Day , B. V. Bagheri , M. J. P. Gingras

Magnetic resonance spectra of EuTiO3 in both bulk and thin film form were taken at temperatures from 3-350 K and microwave frequencies from 9.2-9.8 and 34 GHz. In the paramagnetic phase, magnetic resonance spectra are determined by magnetic…

Materials Science · Physics 2017-03-08 V. V. Laguta , S. Kamba , M. Maryško , B. Andrzejewski , M. Kachlík , K. Maca , J. H. Lee , D. G. Schlom

The frustrated pyrochlore antiferromagnet Gd$_{2}$Ti$_{2}$O$_{7}$ has an unusual partially-ordered magnetic structure at the lowest measurable temperatures. This structure is currently believed to involve four magnetic propagation vectors…

Using muon-spin-relaxation measurements we show that the pyrochlore compound Gd2Ti2O7, in its magnetically orderered phase below ~ 1 K, displays persistent spin dynamics down to temperatures as low as 20 mK. The characteristics of the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Yaouanc , P. Dalmas de Reotier , V. Glazkov , C. Marin , P. Bonville , J. A. Hodges , P. C. M. Gubbens , S. Sakarya , C. Baines

We report the response of electrical resistivity $\rho$ to the application of magnetic fields (H) up to 140 kOe in the temperature interval 1.8-300 K for the compound, Gd7Rh3, ordering antiferromagnetically below 150 K. We find that there…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , E. V. Sampathkumaran

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin

The electron paramagnetic resonance is used to measure the single-ion anisotropy of Gd3+ ions in the pyrochlore structure of (Y{1-x}Gdx)2Ti2O7. A rather strong easy-plane type anisotropy is found. The anisotropy constant D is comparable to…

Strongly Correlated Electrons · Physics 2007-05-23 V. N. Glazkov , M. E. Zhitomirsky , A. I. Smirnov , H. -A. Krug von Nidda , A. Loidl , C. Marin , J. -P. Sanchez

We report high resolution single crystal x-ray diffraction measurements of the frustrated pyrochlore magnet Tb2Ti2O7, collected using a novel low temperature pulsed magnet system. This instrument allows characterization of structural…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , Z. Islam , J. P. Clancy , K. A. Ross , H. Nojiri , Y. H. Matsuda , H. A. Dabkowska , A. D. Dabkowski , B. D. Gaulin

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

The infrared phonon spectrum of the spinel CdCr2O4 is measured as a function temperature from 6 K to 300K. The triply degenerate Cr phonons soften in the paramagnetic phase as temperature is lowered below 100 K and then split into a singlet…

Materials Science · Physics 2009-11-13 R. Valdés Aguilar , A. B. Sushkov , Y. J. Choi , S-W. Cheong , H. D. Drew

The gadolinium pyrochlores, Gd$_2B_2$O$_7$, are amongst the best realizations of antiferromagnetically coupled Heisenberg spins on a pyrochlore lattice. We present a magnetic characterization of Gd$_2$Pt$_2$O$_7$, a unique member of this…

Strongly Correlated Electrons · Physics 2016-10-18 A. M. Hallas , A. Z. Sharma , Y. Cai , T. J. Munsie , M. N. Wilson , M. Tachibana , C. R. Wiebe , G. M. Luke

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

We report synchrotron radiation diffraction and muon spin rotation (muSR) measurements on the frustrated pyrochlore magnet Tb2Ti2O7. The powder diffraction study of a crushed crystal fragment does not reveal any structural change down to 4…

Strongly Correlated Electrons · Physics 2014-12-22 P. Dalmas de Reotier , A. Yaouanc , A. Bertin , C. Marin , S. Vanishri , D. Sheptyakov , A. Cervellino , B. Roessli , C. Baines

We present an elaborate electron-spin resonance study of the low-energy dynamics and magnetization in the ordered phase of the magnetically frustrated spinel ZnCr$_2$O$_4$. We observe several resonance modes corresponding to different…

Strongly Correlated Electrons · Physics 2010-11-29 V. N. Glazkov , A. M. Farutin , V. Tsurkan , H. -A. Krug von Nidda , A. Loidl

A quasi-one dimensional antiferromagnet with a strong reduction of the ordered spin component, BaCu2Si2O7, is studied by the magnetic resonance technique in a wide field and frequency range. Besides of conventional spin-flop transition at…

Strongly Correlated Electrons · Physics 2009-11-11 V. N. Glazkov , A. I. Smirnov , A. Revcolevschi , G. Dhalenne

Longitudinal-field muon spin relaxation experiments have been carried out in the paramagnetic state of single-crystal Gd_2Ti_2O_7 just above the phase transition at T_m = 1.0 K. At high applied fields the exponential relaxation time T_1 is…

Strongly Correlated Electrons · Physics 2009-11-11 D. E. MacLaughlin , M. S. Rose , J. E. Anderson , Lei Shu , R. H. Heffner , T. Kimura , G. D. Morris , O. O. Bernal

The rare earth pyrochlore material Gd2Ti2O7 is considered to be an ideal model frustrated Heisenberg antiferromagnet with additional dipolar interactions. For this system there are several untested theoretical predictions of the ground…

Condensed Matter · Physics 2009-11-07 J. D. M. Champion , A. S. Wills , T. Fennell , S. T. Bramwell , J. S. Gardner , M. A. Green

In the Heisenberg antiferromagnet $Gd_2Ti_2O_7$, the exchange interactions are geometrically frustrated by the pyrochlore lattice structure. This ESR study reveals a strong temperature dependent anisotropy with respect to a [111] body…

Strongly Correlated Electrons · Physics 2016-08-16 A. K. Hassan , L. P. Lévy , C. Darie , P. Strobel

Altermagnetism, known for its non-relativistic spin-split band structures with yet compensated moments, is being intensively investigated. Discovering new altermagnetic materials with characteristics suitable for practical use remains an…