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The question of stability against diffusional mixing at the prototypical LaAlO3/SrTiO3(001) interface is explored using a multi-faceted experimental and theoretical approach. We combine analytical methods with a range of sensitivities to…

The rich electron correlations and highly coherent transport in reconfigurable devices sketched by a conductive atomic force microscope tip at the LaAlO3/SrTiO3 interface have enabled the oxide platform an ideal playground for studying…

Mesoscale and Nanoscale Physics · Physics 2023-06-19 Dawei Qiu , Mengke Ha , Qing Xiao , Zhiyuan Qin , Danqing Liu , Changjian Ma , Guanglei Cheng , Jiangfeng Du

Nanoscale channels realized at the conducting interface between LaAlO$_{3}$ and SrTiO$_{3}$ provide a perfect playground to explore the effect of dimensionality on the electronic properties of complex oxides. Here we compare the electric…

The emergent superconductivity at the LaAlO3/KTaO3 interfaces exhibits a mysterious dependence on the KTaO3 crystallographic orientations. Here we show, by soft X-ray angle-resolved photoemission spectroscopy, that the interfacial…

Infinite-layer nickelate thin films materialize an intriguing new platform for high-temperature unconventional superconductivity, with LaNiO$_2$/SrTiO$_3$ as reference setup. We discuss the relative stability of the elementary interfaces of…

Superconductivity · Physics 2020-08-03 F. Bernardini , A. Cano

The structure and interface characteristics of (LaVO3)6m(SrVO3)m superlattices deposited on (100)-SrTiO3 (STO) substrate were studied using Transmission Electron Microscopy (TEM). Cross-section TEM studies revealed that both LaVO3 (LVO) and…

Materials Science · Physics 2015-05-20 P. Boullay , A. David , W. C. Sheets , U. Lüders , W. Prellier , H. Tan , J. Verbeeck , G. Van Tendeloo , C. Gatel , G. Vincze , Z. Radi

In pursuit of creating cuprate-like electronic and orbital structures, artificial heterostructures based on LaNiO$_3$ have inspired a wealth of exciting experimental and theoretical results. However, to date there is a very limited…

Strongly Correlated Electrons · Physics 2016-02-17 Yanwei Cao , Xiaoran Liu , M. Kareev , D. Choudhury , S. Middey , D. Meyers , J. -W. Kim , P. Ryan , J. W. Freeland , J. Chakhalian

Perovskite oxides are promising for energy and quantum technologies, but wide-gap hosts such as NaAlO3 suffer from deep-UV absorption and limited carrier transport. Using first-principles GGA+U+SOC calculations, we investigate Eu3+-, Gd3+-,…

Materials Science · Physics 2025-10-10 Muhammad Imran , Sikander Azam , Qaiser Rafiq , Amin Ur Rahman

The time-resolved photoconductance of amorphous and crystalline LaAlO$_3$/SrTiO$_3$ interfaces, both hosting an interfacial 2-dimensional electron gas, is investigated under irradiation by variable-wavelengths, visible or ultraviolet…

Interfaces can differ from their parent compounds in terms of charge, spin, and orbital orders and are fertile ground for emergent phenomena, strongly correlated physics, and device applications. Here, we discover that ferroelectric order…

Superconductivity · Physics 2025-06-19 M. D. Dong , X. B. Cheng , M. Zhang , J. Wu

The effect of growth conditions on the structural and electronic properties of the polar/non-polar LaCrO$_3$/SrTiO$_3$ (LCO/STO) interface has been investigated. The interface is either insulating or metallic depending on growth conditions.…

Materials Science · Physics 2019-06-04 A. H. Al-Tawhid , J. R. Frick , D. B. Dougherty , D. P. Kumah

Nanoscale control of the quasi-two-dimensional electron gas at the LaAlO3/SrTiO3 (LAO/STO) interface by a conductive probe tip has triggered the development of a number of electronic devices. While the spatial distribution of the…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Zhanzhi Jiang , Xiaoyu Wu , Hyungwoo Lee , Jung-Woo Lee , Jianan Li , Guanglei Cheng , Chang-Beom Eom , Jeremy Levy , Keji Lai

We investigate the electronic, ferroelectric and magnetic properties of KTaO3/PbTiO3 interfaces by using conventional density functional theory (DFT) and advanced DFT such as hybrid functional HSE06. We show that doped holes in valence…

Materials Science · Physics 2014-07-04 Yi Yang , Chen-Sheng Lin , Jin-Feng Chen , Lei Hu , Wen-Dan Cheng

The interface of complex oxide heterostructures sets the stage for various electronic and magnetic phenomena. Many of these collective effects originate from the precise structural arrangement at the interface that in turn governs local…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Max Burian , Bill Francesco Pedrini , Nazaret Ortiz Hernandez , Hiroki Ueda , C. A. F. Vaz , Milan Radovic , Urs Staub

The two dimensional electron gas formed between the two band insulators SrTiO3 and LaAlO3 exhibits a variety of interesting physical properties which make it an appealing material for use in future spintronics and/or quantum computing…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 D. Rakhmilevitch , M. Ben Shalom , M. Eshkol , A. Tsukernik , A. Palevski , Y. Dagan

Atomically sharp oxide heterostructures exhibit a range of novel physical phenomena that do not occur in the parent bulk compounds. The most prominent example is the appearance of highly conducting and superconducting states at the…

The highly conductive two-dimensional electron gas formed at the interface between insulating SrTiO$_3$ and LaAlO$_3$ shows low-temperature superconductivity coexisting with inhomogeneous ferromagnetism. The Rashba spin-orbit interaction…

Superconductivity · Physics 2013-12-30 N. Mohanta , A. Taraphder

We report first-principles density-functional pseudopotential calculations on the atomic structures, electronic properties, and band offsets of BaO/BaTiO$_3$ and SrO/SrTiO$_3$ nanosized heterojunctions grown on top of a silicon substrate.…

Materials Science · Physics 2009-11-07 Javier Junquera , Magali Zimmer , Pablo Ordejon , Philippe Ghosez

We address the fundamental issue of growth of perovskite ultra-thin films under the condition of a strong polar mismatch at the heterointerface exemplified by the growth of a correlated metal LaNiO$_3$ on the band insulator SrTiO$_3$ along…

Strongly Correlated Electrons · Physics 2014-12-23 S. Middey , P. Rivero , D. Meyers , M. Kareev , X. Liu , Y. Cao , J. W. Freeland , S. Barraza-Lopez , J. Chakhalian

Recently a metallic state was discovered at the interface between insulating oxides, most notably LaAlO3 and SrTiO3. Properties of this two-dimensional electron gas (2DEG) have attracted significant interest due to its potential…

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