Related papers: Two geometrically frustrated magnets studied by ne…
We present neutron diffraction analysis of BaFe$_2$(As$_{1-x}$P$_x$)$_2$ over a wide temperature (10 to 300 K) and compositional ($0.11 \leq x \leq 0.79$) range, including the normal state, the magnetically ordered state, and the…
The magnetic ground state of oxynitride pyrochlore Lu$_2$Mo$_2$O$_{5-y}$N$_2$, a candidate compound for the quantum spin liquid ($S=1/2$, Mo$^{5+}$), was studied by muon spin rotation/relaxation experiment. In contrast to Lu$_2$Mo$_2$O$_7$…
YBaCo4O7 belongs to a new class of geometrically frustrated magnets like the pyrochlores, in which Co-spins occupy corners of tetrahedra. The structure can be viewed as an alternating stacking of Kagome and triangular layers. Exactly half…
The singlet ground state magnetism in pyrochlore osmates Y$_2$Os$_2$O$_7$ and Ho$_2$Os$_2$O$_7$ is studied by DC and AC susceptibility, specific heat, and neutron powder diffraction measurements. Despite the expected non-magnetic singlet in…
Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative…
The frustrated magnet has been regarded as a system that could be a promising host material for the quantum spin liquid (QSL). However, it is difficult to determine the spin configuration and the corresponding mechanism in this system,…
The magnetic pyrochlore oxide materials of general chemical formula R2Ti2O7 and R2Sn2O7 (R = rare earth) display a host of interesting physical behaviours depending on the flavour of rare earth ion. These properties depend on the value of…
Crystal and magnetic structures of $R_2$Ni$_2$In ($R$ = Tb and Ho) have been studied by powder neutron diffraction at low temperatures. The compounds crystallize in an orthorhombic crystal structure of the Mn$_2$AlB$_2$-type. At low…
Two B-site ordered double perovskites, La2LiMoO6 and Ba2YMoO6, based on the S = 1/2 ion, Mo5+, have been investigated in the context of geometric magnetic frustration. Powder neutron diffraction, heat capacity, susceptibility, muon spin…
Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…
The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…
The rich phase diagrams of magnetically frustrated pyrochlores have maintained a high level of interest over the past 20 years. To experimentally explore these phase diagrams requires a means of tuning the relevant interactions. One…
We report an extensive study on the zero field ground state of a powder sample of the pyrochlore $\mathrm{Yb_2Ti_2O_7}$. A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK.…
High pressure neutron diffraction is employed to investigate the magnetic behavior of CaMn$_2$Bi$_2$ in extreme conditions. In contrast to antiferromagnetic ordering on Mn atoms reported at ambient pressure, our results reveal that at high…
Electronic and magnetic properties of molybdenum pyrochlores A2Mo2O7 are studied by the fully relativistic density-functional theory plus on-site repulsion (U) method, with focusing on the spin-glass insulating material Y2Mo2O7. We find…
We report a resonant inelastic X-ray scattering study on a single crystal of a non-stoichiometric pyrochlore iridate Tb$_{2+x}$Ir$_{2-x}$O$_{7-y}$ ($x \simeq 0.25$) that magnetically orders at $T_{\rm{N}}\simeq 50$ K. We find that the…
We have identified TbOF as a unique frustrated and mixed-anion lattice, hosting unconventional magnetism. By means of magnetization, specific heat and neutron diffraction measurements down to 90 mK, as well as DFT calculations, we present a…
Geometric frustration usually arises in systems that comprise magnetic moments (spins) which reside on the sites of a lattice made up of elementary triangular or tetrahedral units and which interact via antiferromagnetic nearest-neighbor…
By means of ac magnetic-susceptibility measurements, we find evidence for a new magnetic phase of Tb$_2$Ti$_2$O$_7$ below about 140 mK in zero magnetic field. In magnetic fields parallel to [111], this phase---exhibiting frequency- and…
Neutron diffraction studies have been carried out in the applied magnetic field H(//[011]) on a single crystal of pyrochlore ferromagnet Nd2Mo2O7, whose Hall resistivity(r_H) has been reported to have quite unusual magnetic field (H)- and…