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We use an off - lattice bead - spring model of a self - avoiding polymer chain immersed in a 3-dimensional quenched random medium to study chain dynamics by means of a Monte - Carlo (MC) simulation. The chain center of mass mean-squared…

Soft Condensed Matter · Physics 2007-05-23 A. Milchev , V. G. Rostiashvili , T. A. Vilgis

We use an off-lattice microscopic model for solutions of equilibrium polymers (EP) in a lamellar shear flow generated by means of a self-consistent external field between parallel hard walls. The individual conformations of the chains are…

Soft Condensed Matter · Physics 2009-10-31 A. Milchev , J. P. Wittmer , D. P. Landau

We present data of Monte Carlo simulations for monodisperse linear polymer chains in dense melts with degrees of polymerization between N=16 and N=512. The aim of this study is to investigate the crossover from Rouse-like dynamics for short…

Soft Condensed Matter · Physics 2009-10-31 T. Kreer , J. Baschnagel , M. Mueller , K. Binder

We use Monte Carlo simulations to study polymer melts consisting of fully flexible and moderately stiff chains in the bond fluctuation model at a volume fraction $0.5$. In order to reduce the local density fluctuations, we test a…

Soft Condensed Matter · Physics 2015-06-24 Hsiao-Ping Hsu

The localization length for isotopically disordered harmonic one-dimensional chains is calculated for arbitrary impurity concentration and scattering cross section. The localization length depends on the scattering cross section of a single…

Disordered Systems and Neural Networks · Physics 2009-11-10 K. A. Snyder , T. R. Kirkpatrick

Whether a system is to be considered complex or not depends on how one searches for correlations. We propose a general scheme for calculation of entropies in lattice systems that has high flexibility in how correlations are successively…

Statistical Mechanics · Physics 2015-06-18 Torbjørn Helvik , Kristian Lindgren

The excitonic luminescence of an isolated polydiacetylene polymer chain in its monomer matrix is studied by micro-photoluminescence. These chains behave as perfect 1D semiconducting wires with the expected 1/$\sqrt{E}$ density of states…

Materials Science · Physics 2007-05-23 F. Dubin

Ladder polymers, known for their rigid, ladder-like structures, exhibit exceptional thermal stability and mechanical strength, positioning them as candidates for advanced applications. However, accurately determining their structure from…

Soft Condensed Matter · Physics 2025-05-23 Lijie Ding , Chi-Huan Tung , Zhiqiang Cao , Zekun Ye , Xiaodan Gu , Yan Xia , Wei-Ren Chen , Changwoo Do

Polymers in nonuniform flows undergo strong deformation, which in the presence of persistent stretching can result in the coil-stretch transition. This phenomenon has been characterized by using the formalism of nonequilibrium statistical…

Soft Condensed Matter · Physics 2023-05-24 Stefano Musacchio , Victor Steinberg , Dario Vincenzi

The adsorption of a single ideal polymer chain on energetically heterogeneous and rough surfaces is investigated using a variational procedure introduced by Garel and Orland (Phys. Rev. B 55 (1997), 226). The mean polymer size is calculated…

Statistical Mechanics · Physics 2009-10-31 Gregor Huber , Thomas A. Vilgis

Macroscopic mechanical properties of polymers are determined by their microscopic molecular chain distribution. Due to randomness of these molecular chains, probability theory has been used to find their micro-states and energy…

Statistical Mechanics · Physics 2023-08-23 Lixiang Yang

We make use of the previously developed formalism for a monomer ensemble and include angular dependence of the segments of the polymer chains thus described. In particular we show how to deal with stiffness when the polymer chain is…

Soft Condensed Matter · Physics 2015-06-24 K. K. Muller-Nedebock , H. L. Frisch , J. K. Percus

In this paper we study the shape characteristics of a polymer chain in a good solvent using a mesoscopic level of modelling. The dissipative particle dynamics simulations are performed in the $3D$ space at a range of chain lengths $N$. The…

Soft Condensed Matter · Physics 2016-11-24 Ostap Kalyuzhnyi , Jaroslav Ilnytskyi , Yurij Holovatch , Christian von Ferber

We study the permeability and selectivity (`permselectivity') of model membranes made of polydisperse polymer networks for molecular penetrant transport, using coarse-grained, implicit-solvent computer simulations. The permeability…

Soft Condensed Matter · Physics 2020-09-30 Won Kyu Kim , Richard Chudoba , Sebastian Milster , Rafael Roa , Matej Kanduc , Joachim Dzubiella

By tracking small particles in the bulk of an intensely turbulent flow, we show that even a very small concentration of long-chain polymers disrupts the usual turbulent energy cascade. The polymers affect scales much larger than their…

Fluid Dynamics · Physics 2007-12-31 Nicholas T. Ouellette , Haitao Xu , Eberhard Bodenschatz

Whereas entropy can induce phase behavior that is as rich as seen in energetic systems, microphase separation remains a very rare phenomenon in entropic systems. In this paper, we present a density functional approach to study the…

Soft Condensed Matter · Physics 2009-11-10 Paul P. F. Wessels , Bela M. Mulder

Trimers are chains formed by two lattice edges, and therefore three monomers. We consider trimers placed on the square lattice, the edges belonging to the same trimer are either colinear, forming a straight rod with unitary statistical…

Statistical Mechanics · Physics 2023-04-19 Pablo Serra , Wellington G. Dantas , Jürgen F. Stilck

A polymer chain pinned in space exerts a fluctuating force on the pin point in thermal equilibrium. The average of such fluctuating force is well understood from statistical mechanics as an entropic force, but little is known about the…

Statistical Mechanics · Physics 2015-07-22 James T. Waters , Harold D. Kim

We study dynamics of a Rouse polymer chain, which diffuses in a three-dimensional space under the constraint that one of its ends, referred to as the slip-link, may move only along a one-dimensional line containing randomly placed,…

Statistical Mechanics · Physics 2007-05-23 S. Nechaev , G. Oshanin , A. Blumen

The conditions of multi-phase equilibrium are solved for generic polydisperse systems. The case of multiple polydispersity is treated, where several properties (e.g. size, charge, shape) simultaneously vary from one particle to another. By…

Statistical Mechanics · Physics 2009-10-31 R. M. L. Evans
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