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With use of homogeneous model for magnetic sub-lattice of compound La1-x CaxMnO3 allowing for Heisenberg superexchange and double exchange between nearest neighbors the temperature dependence of spontaneous magnetization on a separate site…

Strongly Correlated Electrons · Physics 2007-05-23 B. V. Karpenko , L. D. Falkovskaya , A. V. Kuznetsov

Detailed measurements of the magnetic and transport properties of the two La1-xCaxMnO3 (x = 0.18, x = 0.20) single crystals straddling the compositional metal-insulator transition boundary (0.18 < xc < 0.22) are summarized. The analysis of…

Strongly Correlated Electrons · Physics 2009-01-15 Wanjun Jiang , X. Z. Zhou , K. Glazyrin , Y. Mukovskii , Gwyn Williams

The exchange interactions and magnetic structure in layered system CuMnO2 (mineral crednerite) and in nonstoichiometric system Cu1.04Mn0.96O2, with triangular layers distorted due to orbital ordering of the Mn3+ ions, are studied by…

Strongly Correlated Electrons · Physics 2014-01-21 A. V. Ushakov , S. V. Streltsov , D. I. Khomskii

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

Materials Science · Physics 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

We present a neutron and x-ray scattering investigation of Ca$_3$LiOsO$_6$, a material predicted to host magnetic ordering solely through an extended superexchange pathway involving two anions, an interaction mechanism that has undergone…

Strongly Correlated Electrons · Physics 2012-08-13 S. Calder , M. D. Lumsden , V. O. Garlea , J. -W. Kim , Y. G. Shi , H. L. Feng , K. Yamaura , A. D. Christianson

The magnetic properties of the molecular cluster Mn12Ac are due to the four Mn3+ ions which have spins S=3/2 and the eight Mn4+ ions with spins S=2. These spins are coupled by superexchange mechanism. We determine the four exchange…

Strongly Correlated Electrons · Physics 2009-11-07 N. Regnault , Th. Jolicoeur , R. Sessoli , D. Gatteschi , M. Verdaguer

Neutron and X-ray diffraction, magnetic susceptibility, and specific heat measurements have been used to investigate the magnetic and structural phase transitions of the spinel system Fe1+xCr2-xO4(0.0<=x<=1.0). The temperature versus Fe…

The electronic structure and magnetic properties of La_{1-x}A_{x}MnO_3 are investigated. It is assumed that, at the outermost layer, the environment of the Mn ions does not have cubic symmetry. The e_g orbitals are split and the double…

Strongly Correlated Electrons · Physics 2009-10-31 M. J. Calderon , L. Brey , F. Guinea

The effect of orbital degrees of freedom on the exchange interactions in the spin-1 quasi-one-dimensional antiferromagnet CaV2O4 is systematically studied. For this purpose a realistic low-energy model with the parameters derived from the…

Materials Science · Physics 2015-06-23 Z. V. Pchelkina , I. V. Solovyev

We have investigated the crystal structure and magnetic properties for polycrystalline samples of LaMn1-xFexO3+y, in the whole range x=0.0 to x=1.0, prepared by solid state reaction in air. All samples show the ORT-2 orthorhombic structure…

Strongly Correlated Electrons · Physics 2009-11-13 O. F. de Lima , J. A. H. Coaquira , R. L. de Almeida , L. B. de Carvalho , S. K. Malik

The electronic and magnetic structure, including the Heisenberg model exchange interaction parameters, was explored for the recently proposed novel cuprate Cu$_2$F$_5$. Using the DFT+U calculation, it is shown that the compound is formed by…

Strongly Correlated Electrons · Physics 2021-08-11 Dmitry M. Korotin , Dmitry Y. Novoselov , Vladimir I. Anisimov , Artem R. Oganov

The structure and magnetic properties of oligonuclear manganese complex [Mn(hfa)2cpo]2 (where hfa is hexafluoroacetylacetonate dehydrate and cpo is 4-cyanopyridine-N-oxide) are presented. In the unit cell, the dinuclear molecules are well…

The results of ac and dc magnetization and heat capacity measurements on the oxides, Ca$_3$Co$_{1+x}$Mn$_{1-x}$O$_6$, forming in a K$_4$CdCl$_6$-derived rhombohedral quasi-one-dimensional crystal structure, are reported. As far as…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

Two perovskite-derived materials, CaCu3Mn4O12 and CaCu3Ti4O12, have drawn much recent interest due to their magnetoresistive, dielectric, and magnetoelectronic characteristics. Here we present initial theoretical insights into each of these…

Materials Science · Physics 2007-05-23 M. D. Johannes , W. E. Pickett , R. Weht

The spin-wave spectrum in the metallic ferromagnetic lantha-num cubic manganites was investigated. The interactions with four coordination spheres (32 neighbors) were taken into ac-count. The Heisenberg superexchange between all manganese…

Strongly Correlated Electrons · Physics 2008-05-21 B. V. Karpenko , A. V. Kuznetzov

We investigate the magnetic structure of Mn3-xFexSn2 using neutron powder diffraction experiments and electronic structure calculations. These alloys crystallize in the orthorhombic Ni3Sn2 type of structure (Pnma) and comprise two…

Materials Science · Physics 2013-09-03 Q. Recour , V. Ban , Z. Gercsi , T. Mazet , M. Francois , B. Malaman

In this contribution we derive and discuss energy levels of the strongly-correlated d2 configuration of the V3+ ion (LaVO3) and of d4 configuration of the Mn3+ ion (LaMnO3) in the octahedral surroundings in the presence of the spin-orbit…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. Radwanski Z. Ropka

The recent development in the field of 2D magnetic materials urges reliable theoretical methodology for determination of magnetic properties. Among the available methods, ab initio four-state energy mapping based on Density Functional…

Mesoscale and Nanoscale Physics · Physics 2020-08-05 Denis Sabani , Cihan Bacaksiz , Milorad Milosevic

We describe the evolution of the static and dynamic spin correlations of La$_{1-x}$Ca$_x$MnO$_3$, for x=0.1, 0.125 and 0.2, where the system evolves from the canted magnetic state towards the insulating ferromagnetic state, approaching the…

Strongly Correlated Electrons · Physics 2019-08-17 G. Biotteau , M. Hennion , F. Moussa , L. Pinsard , A. Revcolevschi , Y. M. Mukovskii , D. Shulyatev

The crystal structure of hexagonal-Sr0.6Ba0.4MnO3 allows various competing superexchange interactions, leading to intriguing magnetic properties. Local structural changes modify overlapping between Mn and oxygen ions with temperature.…

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