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The magnetic structure of the edge sharing cuprate compound Li2CuO2 has been investigated by means of ab initio electronic structure calculations. The first and second neighbor in-chain magnetic interactions are calculated to be -142 K and…

Materials Science · Physics 2007-05-23 Coen de Graaf , Iberio de P. R. Moreira , Francesc Illas , Oscar Iglesias , Amilcar Labarta

The dc resistivity, magnetoresistance and magnetic susceptibility of La(1-x)SrxCoO3 compounds have been investigated in the temperature range of 4K to 300K for magnetic fields up to 7 T. In the doping range studied (0.05 - x - 0.25) the…

Condensed Matter · Physics 2009-10-28 Vladimir Golovanov , Laszlo Mihaly , A. R. Moodenbaugh

The structure and magnetic properties of Mn1+xV2-xO4 (0<x<=1), a complex frustrated system, were investigated by heat capacity, magnetization, x-ray diffraction, and neutron diffraction measurements. For x<=0.3, a cubic-to-tetragonal (c >…

Strongly Correlated Electrons · Physics 2020-10-07 J. L. Jiao , H. P. Zhang , Q. Huang , W. Wang , G. Wang , Q. Ren , R. Sinclair , G. T. Lin , A. Huq , H. Cao , H. D. Zhou , M. Z. Li , J. Ma

The crystal structure and magnetic properties of the spin-1 triangular-lattice antiferromagnet Ba$_2$La$_2$NiTe$_2$O$_{12}$ are reported. Its crystal structure is trigonal $R\bar{3}$, which is the same as that of Ba$_2$La$_2$NiW$_2$O$_{12}$…

Strongly Correlated Electrons · Physics 2019-08-28 Mutsuki Saito , Masari Watanabe , Nobuyuki Kurita , Akira Matsuo , Koichi Kindo , Maxim Avdeev , Harald O. Jeschke , Hidekazu Tanaka

The spin-chain compounds, Ca3CuIrO6 and Ca3CuRhO6, crystallizing in a K4CdCl6-derived monoclinic structure, are investigated by ac and dc magnetization, isothermal remnant magnetization as well as heat capacity measurements. The results…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , E. V. Sampathkumaran

The ordered magnetic states of MnWO4 at low temperatures were examined by evaluating the spin exchange interactions between the Mn2+ ions of MnWO4 on the basis of first principles density functional calculations and by performing classical…

The recent synthesis of the chromium selenide compound LiCrSe$_2$ constitutes a valuable addition to the ensemble of two-dimensional triangular lattice antiferromagnets (2D-TLA). In this work we present the very first comprehensive study of…

The structural, electronic, and magnetic properties of La2-xBaxCoMnO6 (0.25 =< x =< 1.0) compounds were investigated employing x-ray powder diffraction and magnetometry. The crystal structure evolves from orthorhombic Pnma to rhombohedral…

Materials Science · Physics 2023-03-07 H. Fabrelli , A. G. Silva , M. Boldrin , L. Bufaiçal , E. M. Bittar

Neutron spectroscopy was applied to study the magnetic interactions of orbitally degenerate Co$^{2+}$ on a host MgO rocksalt lattice where no long range spin or orbital order exists. The paramagnetic nature of the substituted monoxide…

We derived simple rules for the sign of superexchange interaction based on the multielectron calculations of the superexchange interaction in the transition metal oxides that are valid both below and above spin crossover under high…

Materials Science · Physics 2020-03-18 Vladimir A. Gavrichkov , Semyon I. Polukeev , Sergey G. Ovchinnikov

The puzzle of 3D magnetic interactions in the structurally 2D layered oxide Na$_{x}$CoO$_2$ is addressed using first principles calculations and analysis of the exchange mechanisms. The calculations agree with recent neutron results,…

Strongly Correlated Electrons · Physics 2007-05-23 M. D. Johannes , I. I. Mazin , D. J. Singh

A comprehensive theoretical and experimental study is presented of the magnetic susceptibility versus temperature \chi(T) of spin S = 1/2 two- and three-leg Heisenberg ladders and ladder oxide compounds. Extensive quantum Monte Carlo…

The delicate balance between spin-orbit coupling, Coulomb repulsion and crystalline electric field interactions observed in Ir-based oxides is usually manifested as exotic magnetic behavior. Here we investigate the evolution of the exchange…

Evidence for multiple magnetic transitions and unconventional spin exchange interactions in the ilmenite insulator MnTiO3 is provided via neutron scattering. On cooling, while G-type antiferromagnetic (AFM) order sets in first at 63 K with…

Strongly Correlated Electrons · Physics 2026-03-09 Srimal Rathnayaka , Luke Daemen , Despina Louca

We present a method of extracting the exchange parameters of the classical Heisenberg model from first-principles calculations of spin-spiral total energies based on density functional theory. The exchange parameters of the transition-metal…

Materials Science · Physics 2015-06-17 Adam Jacobsson , Biplab Sanyal , Marjana Lezaic , Stefan Blügel

Spin-crossover compounds, which are characterized by magnetic ions showing low-spin and high-spin states at thermally accessible energies, are ubiquitous in nature. We here focus on the effect of an exchange interaction on the collective…

Statistical Mechanics · Physics 2009-11-13 Carsten Timm , Charles J. Pye

The electronic structure and magnetic properties of CaCr$\mathrm{O}_3$ have been calculated by two methods, including hybrid-exchange density-function theory and density-functional theory + $U$. The computed densities of states from both of…

Strongly Correlated Electrons · Physics 2015-05-13 Wei Wu

We report the crystal structure, magnetization measurements, and band-structure calculations for the spin-1/2 quantum magnet CaCu2(SeO3)2Cl2. The magnetic behavior of this compound is well reproduced by a uniform spin-1/2 chain model with…

Magnetic molecules are a class of compounds that is also investigated in view of their magnetocaloric properties. The isothermal entropy change and the adiabatic temperature change are key figures of merit for magnetocaloric performance.…

Chemical Physics · Physics 2026-02-23 D. Westerbeck , J. Schnack

We have studied the phase diagram of La$_{1-x}$Ca$_{x}$MnO$_{3}$ for $0.5\leq x\leq 0.9$ using neutron powder diffraction and magnetization measurements. At 300 K all samples are paramagnetic and single phase with crystallographic symmetry…

Strongly Correlated Electrons · Physics 2009-11-07 M. Pissas , G. Kallias