English
Related papers

Related papers: Orbital ordering in LaMnO$_3$: Electron-electron v…

200 papers

We consider a model of strongly correlated $e_g$ electrons interacting by superexchange orbital interactions in the ferromagnetic phase of LaMnO$_3$. It is found that the classical orbital order with alternating occupied $e_g$ orbitals has…

Strongly Correlated Electrons · Physics 2009-10-31 Jeroen van den Brink , Peter Horsch , Frank Mack , Andrzej M. Oles

Using the multi-band $d-p$ model and unrestricted Hartree-Fock approximation we investigate the electronic structure and spin-orbital order in three-dimensional VO$_3$ lattice. The main aim of this investigation is testing if simple $d-p$…

Strongly Correlated Electrons · Physics 2018-08-14 Krzysztof Rościszewski , Andrzej M. Oleś

We use the temperature of the structural phase transition to determine the Jahn-Teller (JT) coupling constant in the model derived for LaMnO$_3$ which includes both the superexchange between S=2 spins and the JT effect. We also investigate…

Strongly Correlated Electrons · Physics 2022-01-27 Olga Sikora , Andrzej M. Oles

CaMnO3 is a simple bi-partite antiferromagnet(AF) which can be continuously electron-doped up to LaMnO3. Electrons enter the doubly degenerate E_g subshell with spins aligned to the S=3/2 core of Mn^4+ (T_2g^3)$. We take the Hubbard and…

Strongly Correlated Electrons · Physics 2009-11-07 Yiing-Rei Chen , Philip B. Allen

The effects of lattice relaxation in LaTiO$_3$/SrTiO$_3$ superlattices are investigated using a combination of LDA$+U$ density functional theory, and Hartree-Fock effective Hamiltonian calculations. We find noticeable ($\sim 0.1$--0.2 \AA)…

Strongly Correlated Electrons · Physics 2021-04-06 Satoshi Okamoto , Andrew J. Millis , Nicola A. Spaldin

We present powder and single crystal X-ray diffraction data as evidence for a monoclinic distortion in the low spin (S=0) and intermediate spin state (S=1) of LaCoO3. The alternation of short and long bonds in the ab plane indicates the…

Strongly Correlated Electrons · Physics 2009-11-10 G. Maris , Y. Ren , V. Volotchaev , C. Zobel , T. Lorenz , T. T. M. Palstra

The collective behavior of correlated electrons in the VO$_2-$interface layer of LaVO$_3$/SrTiO$_3$ heterostructure is studied within a quarter-filled $t_{2g}$-orbital Hubbard model on a square lattice. We argue that the ground state is…

Strongly Correlated Electrons · Physics 2008-11-21 G. Jackeli , G. Khaliullin

We study how strain affects orbital ordering and magnetism at the interface between SrMnO$_3$ and LaMnO$_3$ from density-functional calculations and interpret the basic results in terms of a three-site Mn-O-Mn model. Magnetic interaction…

Materials Science · Physics 2010-03-10 B. R. K. Nanda , S. Satpathy

The origin of the "hidden" quadrupolar and unconventional magnetic low-temperature orders observed in the spin-orbit double perovskite Ba$_2$MgReO$_6$ defies explanation through standard experimental and theoretical techniques. Here we…

Strongly Correlated Electrons · Physics 2024-11-07 Dario Fiore Mosca , Cesare Franchini , Leonid V. Pourovskii

We investigate the highly frustrated spin and orbital superexchange interactions in cubic vanadates. The fluctuations of $t_{2g}$ orbitals trigger a {\it novel mechanism of ferromagnetic interactions} between spins S=1 of V$^{3+}$ ions…

Strongly Correlated Electrons · Physics 2009-11-07 G. Khaliullin , P. Horsch , A. M. Oles

The debate over the orbital order in layered triangular lattice system NaTiO$_2$ has been rekindled by the recent experiments of McQueen, et al. \cite{cava} on NaVO$_2$ ({\em Phys. Rev. Lett.} {\bf 101}, 166402 (2008)). In view of this, the…

Strongly Correlated Electrons · Physics 2015-05-30 Monika Dhariwal , T. Maitra , Ishwar Singh , S. Koley , A. Taraphder

The role of lattice distortion in the charge, orbital and spin ordering in half doped manganites has been investigated. For fixed magnetic ordering, we show that the cooperative lattice distortion stabilize the experimentally observed…

Strongly Correlated Electrons · Physics 2009-11-07 R. Y. Gu , C. S. Ting

We investigate spin-charge-orbital ordering in a Mn$^{3+}$/Mn$^{4+}$ mixed valence state on a hollandite-type lattice using unrestricted Hartree-Fock calculation on a multi-band Mn 3$d$-O 2$p$ lattice model. The calculations show that the…

Strongly Correlated Electrons · Physics 2013-02-19 Makoto Fukuzawa , Daiki Ootsuki , Takashi Mizokawa

We present evidence that the insulator to metal transition in (La,Ca)MnO3 near x~0.2 is driven by the suppression of coherent Jahn-Teller distortions, originating from d type orbital ordering. The orbital ordered state is characterised by…

Materials Science · Physics 2009-11-07 Bas B. Van Aken , Auke Meetsma , Y. Tomioka , Y. Tokura , Thomas T. M. Palstra

Single-site dynamical mean field theory is used to determine the magnetic and orbital-ordering phase diagram for a model of electrons moving on a lattice with three orbital states per site and with the fully rotationally invariant…

Strongly Correlated Electrons · Physics 2010-02-22 Ching-Kit Chan , Philipp Werner , Andrew J. Millis

Crystal lattice structure is present in stellar compact objects, such as white dwarf stars and in the crust of neutron stars. These structures can be described by a body-centered cubic crystal, which is formed by ions due to Coulombian…

Solar and Stellar Astrophysics · Physics 2022-12-20 S. V. C. Ramalho , S. B. Duarte , G. S. Vicente

The equilibrium structure and exchange constants of CaMnO$_3$ and LaMnO$_3$ have been investigated using total energy unrestricted Hartree-Fock (UHF) and localised orbital configuration interaction (CI) calculations on the bulk compounds…

Strongly Correlated Electrons · Physics 2009-11-07 M. Nicastro , C. H. Patterson

The standard way to find the orbital occupation of Jahn-Teller (JT) ions is to use structural data, with the assumption of a one-to-one correspondence between the orbital occupation and the associated JT distortion, e.g. in O6 octahedron.…

Strongly Correlated Electrons · Physics 2011-10-19 Hua Wu , C. F. Chang , O. Schumann , Z. Hu , J. C. Cezar , T. Burnus , N. Hollmann , N. B. Brookes , A. Tanaka , M. Braden , L. H. Tjeng , D. I. Khomskii

We investigate the frustrated magnetic interactions in cubic transition metal oxides with orbital degeneracy. The $e_g$ orbitals order easier and their ordering explains the $A$-type antiferromagnetic phase in KCuF$_3$ and LaMnO$_3$. In…

Strongly Correlated Electrons · Physics 2016-08-31 Andrzej M. Oles

The origin of the cooperative Jahn-Teller distortion and orbital-order in LaMnO3 is central to the physics of the manganites. The question is complicated by the simultaneous presence of tetragonal and GdFeO3-type distortions and the strong…

Strongly Correlated Electrons · Physics 2013-05-29 Eva Pavarini , Erik Koch