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We report a theoretical investigation of a charged 180$^\circ$ domain wall in ferroelectric PbTiO$_3$, compensated by randomly distributed immobile charge defects. For this we utilize atomistic shell-model simulations and continuous…

Density functional theory calculations have been performed for the structural, electronic, magnetic and ferroelectric properties of a mixed-valence Fe(II)-Fe(III) formate framework [NH$_2$(CH$_3$)$_2$][Fe$^{\rm III}$Fe$^{\rm II}$(HCOO)$_6$]…

Materials Science · Physics 2019-10-15 Gang Tang , Wei Ren , Jiawang Hong , Alessandro Stroppa

Two-dimensional (2D) ferroelectrics, which is rare in nature, enable high-density non-volatile memory with low energy consumption. Here, we propose a theory of bilayer stacking ferroelectricity (BSF), in which, two stacked layers of the…

Materials Science · Physics 2023-04-19 Junyi Ji , Changsong Xu , H. J. Xiang

Domain walls in ferroelectrics exhibit a plethora of phases and functionalities not found in the bulk. The interplay of electrostatic, chemical, topological, and distortive inhomogeneities at the walls can be so complex, however, that this…

Mesoscale and Nanoscale Physics · Physics 2017-02-23 Gabriele De Luca , Marta D. Rossell , Jakob Schaab , Nathalie Viart , Manfred Fiebig , Morgan Trassin

Charge manipulation and fabrication of stable domain patterns in ferroelectric materials by scanning probe microscopy open up broad avenues for the development of tunable electronics. Harnessing the polarization energy and electrostatic…

Materials Science · Physics 2021-02-08 S. Kondovych , A. Gruverman , I. Luk'yanchuk

The interaction of electric field with charged domain walls in ferroelectrics is theoretically addressed. A general expression for the force acting per unit area of a charged domain wall carrying free charge is derived. It is shown that, in…

Materials Science · Physics 2012-01-31 Maxim Y. Gureev , Pavel Mokry , Alexander K. Tagantsev , Nava Setter

Pyroelectricity is a very promising phenomenon in three- and two-dimensional (2D) materials, but first-principles calculations have not so far been used to elucidate the underlying mechanisms. Here we report density-functional theory (DFT)…

Materials Science · Physics 2018-05-23 Jian Liu , Sokrates T. Pantelides

Ferroelectrets are piezoelectrically-active polymer foams that can convert externally applied loads into electric charge. Existing processing routes used to create pores of the desired geometry and degree of alignment appropriate for…

Applied Physics · Physics 2019-02-06 Yan Zhang , Chris R. Bowen , Sylvain Deville

The density functional theory (DFT) is used to investigate the mechanical properties of pure, fully hydrogenated, semi-hydrogenated, fully fluorinated, and semi-fluorinated germanene sheets, including Young's and bulk moduli, and plastic…

Materials Science · Physics 2021-04-07 M. Goli , S. M. Mozvashi , P. Aghdasi , Sh. Yousefi , R. Ansari

The polarization fatigue in (Pb0.97La0.02)(Zr0.95Ti0.05)O3 (PLZT) antiferroelectric thin films deposited onto silicon wafers is studied by investigating the effect of the peak/average/effective cycling voltage through varying the waveform…

A new experimental set-up controlled by computer has been made to measure the pyroelectric charge of ferroelectric materials with a relatively high conductivity at slow rates of temperature variation. It allowed us to obtain the…

Materials Science · Physics 2007-05-23 B. Noheda , N. Duan , N. Cereceda , J. A. Gonzalo

In biological and synthetic materials, many important processes involve charges that are present in a medium with spatially varying dielectric permittivity. To accurately understand the role of electrostatic interactions in such systems, it…

Soft Condensed Matter · Physics 2013-09-30 Vikram Jadhao , Francisco J. Solis , Monica Olvera de la Cruz

Due to their low surface mass density, two-dimensional materials with a strong piezoelectric response are interesting for nanoelectromechanical systems with high force sensitivity. Unlike graphene, the two sublattices in a monolayer of…

Mesoscale and Nanoscale Physics · Physics 2016-08-05 Matthias Droth , Guido Burkard , Vitor M. Pereira

The discovery of two-dimensional (2D) materials possessing switchable spontaneous polarization with atomic thickness opens up exciting opportunities to realize ultrathin, high-density electronic devices with potential applications ranging…

Materials Science · Physics 2020-11-04 Jiawei Huang , Sang-Hoon Lee , Andrew Supka , Young-Woo Son , Shi Liu

An electric-field-induced phase transition and pattern formation in a binary dielectric fluid layer are studied using a coarse-grained free energy functional. The electrostatic part of the free energy is a nonlinear functional of the…

Soft Condensed Matter · Physics 2007-05-23 M. D. Johnson , X. Duan , Brett Riley , Aniket Bhattacharya , Weili Luo

In this paper, the theoretical analysis for a hollow thick-walled functionally graded piezoelectric cylinder subjected to electric and mechanical loads are developed. The cylinder consists of two materials (PZT4 and PVDF) and the volume…

Other Condensed Matter · Physics 2018-11-14 Han Wang , Libiao Xin , Guansuo Dui

We performed density functional theory (DFT) calculations on epitaxially strained hafnia. We demonstrate the stabilization of the ferroelectric ($Pca2_{1}$) phase from the antiferroelectric ($Pbcn$) in bulk hafnia in the presence of…

Materials Science · Physics 2023-02-07 Aldo Raeliarijaona , R. E. Cohen

We investigate the properties of oxygen-functionalized carbides of lanthanide elements with the composition M2CO2 (M=Gd, Tb,Dy) that form two-dimensional (2D) structures. Our ab initio calculations reveal that oxygen termination turns M2C…

Materials Science · Physics 2024-06-04 Lin Han , Wencong Sun , Pingwei Liu , Xianqing Lin , Dan Liu , David Tomanek

The dynamics of phase field crystal (PFC) modeling is derived from dynamical density functional theory (DDFT), for both single-component and binary systems. The derivation is based on a truncation up to the three-point direct correlation…

Materials Science · Physics 2015-05-19 Zhi-Feng Huang , K. R. Elder , Nikolas Provatas

Combining ferroelectricity with other properties such as visible light absorption or long-range magnetic order requires the discovery of new families of ferroelectric materials. Here, through the analysis of a high-throughput database of…