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V 3$d$ charge and orbital states in V$_2$OPO$_4$ have been investigated by means of x-ray absorption spectroscopy (XAS). The electronic structure of V$_2$OPO$_4$ is very unique in that the charge transfer between V$^{2+}$ and V$^{3+}$ in…

Strongly Correlated Electrons · Physics 2020-06-09 Kota Murota , Elise Pachoud , J. Paul Attfield , Robert Glaum , Ronny Sutarto , Kou Takubo , Daniel I. Khomskii , Takashi Mizokawa

Effects of possible orbital order in magnetic properties of two-dimensional spin gap system for CaV$_4$O$_9$ are investigated theoretically. After analyzing experimental data, we show that single orbital models assumed in the literature are…

Strongly Correlated Electrons · Physics 2009-10-30 Nobuyuki Katoh , Masatoshi Imada

We present the refinement of the crystal structure of charge-ordered LuFe2O4, based on single-crystal x-ray diffraction data. The arrangement of the different Fe-valence states, determined with bond-valence-sum analysis, corresponds to a…

Strongly Correlated Electrons · Physics 2012-05-04 J. de Groot , T. Mueller , R. A. Rosenberg , D. J. Keavney , Z. Islam , J. -W. Kim , M. Angst

The local structure of La2-xSrxCuO4, for 0 < x < 0.30, has been investigated using the atomic pair distribution function (PDF) analysis of neutron powder diffraction data. The local octahedral tilts are studied to look for evidence of [110]…

Superconductivity · Physics 2009-10-31 E. S. Bozin , S. J. L. Billinge , G. H. Kwei , H. Takagi

Charge transfer between metal nanoparticles and the supported TiO2 surface is primarily important for catalytic applications as it greatly affects the catalytic activity and the thermal stability of the deposited nanoparticles on the…

Materials Science · Physics 2013-12-24 Cai Yongqing , Bai Zhaoqiang , Chintalapati Sandhya , Zeng Qingfeng , Feng Yuan Ping

Ionic liquids form intricate microstructures, both in the bulk and near charged surfaces. In this Letter, we show that, given the ionic positions from molecular simulations, the ionic charges minimize a "spin-glass" Hamiltonian for…

Chemical Physics · Physics 2019-05-29 Amir Levy , Michael McEldrew , Martin Z. Bazant

The weakly interacting S=1/2 dimers system Sr3Cr2O8 has been investigated by powder neutron diffraction and inelastic neutron scattering. Our data reveal a structural phase transition below room temperature corresponding to an…

Materials Science · Physics 2008-07-10 L. C. Chapon , C. Stock , P. G. Radaelli , C. Martin

We examine the role of charge, structural, and spin degrees of freedom in the previously poorly understood phase transition in the 5$d^1$ transition-metal double perovskite Cs$_2$TaCl$_6$, using a combination of computational and…

The spin-one-half Falicov-Kimball model with spin-dependent on-site interaction between localized ($f$) and itinerant ($d$) electrons is studied by small-cluster exact-diagonalization calculations and a well-controlled approximative method…

Strongly Correlated Electrons · Physics 2008-05-28 Hana Cencarikova , Pavol Farkasovsky , Natalia Tomasovicov , Martin Zonda

We have performed ab initio calculations within the LDA+U method in the multilayered system (LaMnO$_3$)$_{2n}$ / (SrMnO$_3$)$_n$. Our results suggest a charge-ordered state that alternates Mn$^{3+}$ and Mn$^{4+}$ cations in a checkerboard…

Strongly Correlated Electrons · Physics 2016-04-25 Victor Pardo , Antia S. Botana , Daniel Baldomir

We performed low-bias STM measurements on underdoped Bi2212 crystals, and confirmed that a two-dimensional (2D) superstructure with a periodicity of four lattice constants (4a) is formed within the Cu-O plane at T<Tc. This 4a X 4a…

Superconductivity · Physics 2007-05-23 N. Momono , A. Hashimoto , Y. Kobatake , M. Oda , M. Ido

The candidate magnetoelectric Pb3Mn7O15 has a structure consisting of 1/3 filled Kagome layers linked by ribbons of edge-sharing octahedra in the stacking direction. Previous reports have indicated a complex hexagonal-orthorhombic…

Strongly Correlated Electrons · Physics 2012-04-18 Simon A. J. Kimber

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

Strong resonant enhancements of the charge-order and spin-order superstructure-diffraction intensities in La1.8Sr0.2NiO4 are observed when x-ray energies in the vicinity of the Ni L2,3 absorption edges are used. The pronounced photon-energy…

The competition between long-range and short-range interactions among holes moving in an antiferromagnet (AF), is studied within a model derived from the spin density wave picture of layered transition metal oxides. A novel numerical…

We report a high-resolution neutron diffraction study on the orbitally-degenerate spin-1/2 hexagonal antiferromagnet AgNiO2. A structural transition to a tripled unit cell with expanded and contracted NiO6 octahedra indicates root(3) x…

Strongly Correlated Electrons · Physics 2009-11-13 E. Wawrzynska , R. Coldea , E. M. Wheeler , I. I. Mazin , M. D. Johannes , T. Sorgel , M. Jansen , R. M. Ibberson , P. G. Radaelli

The nature of electronic states due to strong correlation and geometric frustration on the triangular lattice is investigated in connection to the unconventional insulating state of Na$_x$CoO$_2$ at $x=0.5$. We study an extended Hubbard…

Strongly Correlated Electrons · Physics 2007-06-13 Sen Zhou , Ziqiang Wang

Using first principle band structure calculations, we critically examine results of resonant x-ray scattering experiments which is believed to directly probe charge and orbital ordering. Considering the specific case of La0.5Sr1.5MnO4, we…

Strongly Correlated Electrons · Physics 2015-06-24 Priya Mahadevan , K. Terakura , D. D. Sarma

Motivated by the co-existing charge and spin order found in strongly correlated ladder systems, we study an effective pseudospin model on a coupled two-leg ladder. A bosonisation analysis yields a rich phase diagram showing Wigner/Peierls…

Strongly Correlated Electrons · Physics 2007-05-23 Siddhartha Lal , Mukul S. Laad

It was recently discovered that the low temperature, charge ordered phase of 1T-TiSe2 has a chiral character. This unexpected chirality in a system described by a scalar order parameter could be explained in a model where the emergence of…