English

Charge and spin order on the triangular lattice -- Na$_x$CoO$_2$ at $x=0.5$

Strongly Correlated Electrons 2007-06-13 v3

Abstract

The nature of electronic states due to strong correlation and geometric frustration on the triangular lattice is investigated in connection to the unconventional insulating state of Nax_xCoO2_2 at x=0.5x=0.5. We study an extended Hubbard model using a spatially unrestricted Gutzwiller approximation. We find a new class of charge and spin ordered states at x=1/3x=1/3 and x=0.5x=0.5 where antiferromagnetic (AF) frustration is alleviated via weak charge inhomogeneity. At x=0.5x=0.5, we show that the 3a×2a\sqrt{3}a\times2a off-plane Na dopant order induces weak 3a×1a\sqrt{3}a\times1a charge order in the Co layer. The symmetry breaking enables successive 3a×1a\sqrt{3}a\times1a AF and 2a×2a2a\times2a charge/spin ordering transitions at low temperatures. The Fermi surface is truncated by the 2a×2a2a\times2a hexagonal zone boundary into small electron and hole pockets. We study the phase structure and compare to recent experiments.

Keywords

Cite

@article{arxiv.cond-mat/0608068,
  title  = {Charge and spin order on the triangular lattice -- Na$_x$CoO$_2$ at $x=0.5$},
  author = {Sen Zhou and Ziqiang Wang},
  journal= {arXiv preprint arXiv:cond-mat/0608068},
  year   = {2007}
}

Comments

4 pages, 4 figures, revtex4 file